Literature DB >> 22623524

Ideal glass transitions by random pinning.

Chiara Cammarota1, Giulio Biroli.   

Abstract

We study the effect of freezing the positions of a fraction c of particles from an equilibrium configuration of a supercooled liquid at a temperature T. We show that within the random first-order transition theory pinning particles leads to an ideal glass transition for a critical fraction c = c(K)(T) even for moderate supercooling; e.g., close to the Mode-Coupling transition temperature. First we derive the phase diagram in the T - c plane by mean field approximations. Then, by applying a real-space renormalization group method, we obtain the critical properties for |c - c(K)(T)| → 0, in particular the divergence of length and time scales, which are dominated by two zero-temperature fixed points. We also show that for c = c(K)(T) the typical distance between frozen particles is related to the static point-to-set length scale of the unconstrained liquid. We discuss what are the main differences when particles are frozen in other geometries and not from an equilibrium configuration. Finally, we explain why the glass transition induced by freezing particles provides a new and very promising avenue of research to probe the glassy state and ascertain, or disprove, the validity of the theories of the glass transition.

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Year:  2012        PMID: 22623524      PMCID: PMC3384138          DOI: 10.1073/pnas.1111582109

Source DB:  PubMed          Journal:  Proc Natl Acad Sci U S A        ISSN: 0027-8424            Impact factor:   11.205


  18 in total

1.  On the Adam-Gibbs-Kirkpatrick-Thirumalai-Wolynes scenario for the viscosity increase in glasses.

Authors:  Jean-Philippe Bouchaud; Giulio Biroli
Journal:  J Chem Phys       Date:  2004-10-15       Impact factor: 3.488

2.  Static point-to-set correlations in glass-forming liquids.

Authors:  Ludovic Berthier; Walter Kob
Journal:  Phys Rev E Stat Nonlin Soft Matter Phys       Date:  2012-01-03

3.  Random pinning in glassy spin models with plaquette interactions.

Authors:  Robert L Jack; Ludovic Berthier
Journal:  Phys Rev E Stat Nonlin Soft Matter Phys       Date:  2012-02-15

4.  Rounding of first-order phase transitions in systems with quenched disorder.

Authors: 
Journal:  Phys Rev Lett       Date:  1989-05-22       Impact factor: 9.161

5.  Growing static and dynamic length scales in a glass-forming liquid.

Authors:  François Sausset; Gilles Tarjus
Journal:  Phys Rev Lett       Date:  2010-02-10       Impact factor: 9.161

6.  Metastable states and space-time phase transitions in a spin-glass model.

Authors:  Robert L Jack; Juan P Garrahan
Journal:  Phys Rev E Stat Nonlin Soft Matter Phys       Date:  2010-01-08

7.  Constructing explicit magnetic analogies for the dynamics of glass forming liquids.

Authors:  Jacob D Stevenson; Aleksandra M Walczak; Randall W Hall; Peter G Wolynes
Journal:  J Chem Phys       Date:  2008-11-21       Impact factor: 3.488

8.  Growing length and time scales in glass-forming liquids.

Authors:  Smarajit Karmakar; Chandan Dasgupta; Srikanth Sastry
Journal:  Proc Natl Acad Sci U S A       Date:  2009-02-20       Impact factor: 11.205

9.  Scaling concepts for the dynamics of viscous liquids near an ideal glassy state.

Authors: 
Journal:  Phys Rev A Gen Phys       Date:  1989-07-15

10.  Renormalization group analysis of the random first-order transition.

Authors:  Chiara Cammarota; Giulio Biroli; Marco Tarzia; Gilles Tarjus
Journal:  Phys Rev Lett       Date:  2011-03-17       Impact factor: 9.161

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  17 in total

1.  Vanishing of configurational entropy may not imply an ideal glass transition in randomly pinned liquids.

Authors:  Saurish Chakrabarty; Smarajit Karmakar; Chandan Dasgupta
Journal:  Proc Natl Acad Sci U S A       Date:  2015-08-17       Impact factor: 11.205

2.  Reply to Chakrabarty et al.: Particles move even in ideal glasses.

Authors:  Misaki Ozawa; Walter Kob; Atsushi Ikeda; Kunimasa Miyazaki
Journal:  Proc Natl Acad Sci U S A       Date:  2015-08-17       Impact factor: 11.205

3.  Equilibrium phase diagram of a randomly pinned glass-former.

Authors:  Misaki Ozawa; Walter Kob; Atsushi Ikeda; Kunimasa Miyazaki
Journal:  Proc Natl Acad Sci U S A       Date:  2015-05-14       Impact factor: 11.205

4.  Assessing the role of static length scales behind glassy dynamics in polydisperse hard disks.

Authors:  John Russo; Hajime Tanaka
Journal:  Proc Natl Acad Sci U S A       Date:  2015-05-18       Impact factor: 11.205

5.  Probing the non-Debye low-frequency excitations in glasses through random pinning.

Authors:  Luca Angelani; Matteo Paoluzzi; Giorgio Parisi; Giancarlo Ruocco
Journal:  Proc Natl Acad Sci U S A       Date:  2018-08-13       Impact factor: 11.205

6.  Structured environments fundamentally alter dynamics and stability of ecological communities.

Authors:  Nick Vallespir Lowery; Tristan Ursell
Journal:  Proc Natl Acad Sci U S A       Date:  2018-12-28       Impact factor: 11.205

7.  Structural-dynamical transition in the Wahnström mixture.

Authors:  Francesco Turci; Thomas Speck; C Patrick Royall
Journal:  Eur Phys J E Soft Matter       Date:  2018-04-26       Impact factor: 1.890

8.  A topologically driven glass in ring polymers.

Authors:  Davide Michieletto; Matthew S Turner
Journal:  Proc Natl Acad Sci U S A       Date:  2016-04-26       Impact factor: 11.205

9.  Random pinning glass model.

Authors:  Smarajit Karmakar; Giorgio Parisi
Journal:  Proc Natl Acad Sci U S A       Date:  2013-02-04       Impact factor: 11.205

10.  Multidimensional stationary probability distribution for interacting active particles.

Authors:  Claudio Maggi; Umberto Marini Bettolo Marconi; Nicoletta Gnan; Roberto Di Leonardo
Journal:  Sci Rep       Date:  2015-05-29       Impact factor: 4.379

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