| Literature DB >> 20366830 |
François Sausset1, Gilles Tarjus.
Abstract
We investigate the characteristic length scales associated with the glass transition phenomenon. By studying an atomic glass-forming liquid in negatively curved space, for which the local order is well identified and the amount of frustration opposing the spatial extension of this order is tunable, we provide insight into the structural origin of the main characteristics of the dynamics leading to glass formation. We find that the structural length and the correlation length characterizing the increasing heterogeneity of the dynamics grow together as temperature decreases. However, the system eventually enters a regime in which the former saturates as a result of frustration whereas dynamic correlations keep building up.Year: 2010 PMID: 20366830 DOI: 10.1103/PhysRevLett.104.065701
Source DB: PubMed Journal: Phys Rev Lett ISSN: 0031-9007 Impact factor: 9.161