Literature DB >> 26038545

Assessing the role of static length scales behind glassy dynamics in polydisperse hard disks.

John Russo1, Hajime Tanaka1.   

Abstract

The possible role of growing static order in the dynamical slowing down toward the glass transition has recently attracted considerable attention. On the basis of random first-order transition theory, a new method to measure the static correlation length of amorphous order, called "point-to-set" (PTS) length, has been proposed and used to show that the dynamic length grows much faster than the static length. Here, we study the nature of the PTS length, using a polydisperse hard-disk system, which is a model that is known to exhibit a growing hexatic order upon densification. We show that the PTS correlation length is decoupled from the steeper increase of the correlation length of hexatic order and dynamic heterogeneity, while closely mirroring the decay length of two-body density correlations. Our results thus provide a clear example that other forms of order can play an important role in the slowing down of the dynamics, casting a serious doubt on the order-agnostic nature of the PTS length and its relevance to slow dynamics, provided that a polydisperse hard-disk system is a typical glass former.

Keywords:  glass transition; hexatic order; pinning; slow dynamics; structural length scales

Year:  2015        PMID: 26038545      PMCID: PMC4460450          DOI: 10.1073/pnas.1501911112

Source DB:  PubMed          Journal:  Proc Natl Acad Sci U S A        ISSN: 0027-8424            Impact factor:   11.205


  26 in total

1.  Geometrical frustration and static correlations in a simple glass former.

Authors:  Benoit Charbonneau; Patrick Charbonneau; Gilles Tarjus
Journal:  Phys Rev Lett       Date:  2012-01-18       Impact factor: 9.161

2.  Dynamic relaxation of a liquid cavity under amorphous boundary conditions.

Authors:  Andrea Cavagna; Tomás S Grigera; Paolo Verrocchio
Journal:  J Chem Phys       Date:  2012-05-28       Impact factor: 3.488

3.  Correlation between dynamic heterogeneity and medium-range order in two-dimensional glass-forming liquids.

Authors:  Takeshi Kawasaki; Takeaki Araki; Hajime Tanaka
Journal:  Phys Rev Lett       Date:  2007-11-20       Impact factor: 9.161

4.  Dynamical correlations in a glass former with randomly pinned particles.

Authors:  Robert L Jack; Christopher J Fullerton
Journal:  Phys Rev E Stat Nonlin Soft Matter Phys       Date:  2013-10-11

5.  Comparison of static length scales characterizing the glass transition.

Authors:  Giulio Biroli; Smarajit Karmakar; Itamar Procaccia
Journal:  Phys Rev Lett       Date:  2013-10-14       Impact factor: 9.161

6.  Growing point-to-set length scale correlates with growing relaxation times in model supercooled liquids.

Authors:  Glen M Hocky; Thomas E Markland; David R Reichman
Journal:  Phys Rev Lett       Date:  2012-06-01       Impact factor: 9.161

7.  Bond orientational order in liquids: Towards a unified description of water-like anomalies, liquid-liquid transition, glass transition, and crystallization: Bond orientational order in liquids.

Authors:  Hajime Tanaka
Journal:  Eur Phys J E Soft Matter       Date:  2012-10-31       Impact factor: 1.890

8.  Importance of many-body correlations in glass transition: an example from polydisperse hard spheres.

Authors:  Mathieu Leocmach; John Russo; Hajime Tanaka
Journal:  J Chem Phys       Date:  2013-03-28       Impact factor: 3.488

9.  Decorrelation of the static and dynamic length scales in hard-sphere glass formers.

Authors:  Patrick Charbonneau; Gilles Tarjus
Journal:  Phys Rev E Stat Nonlin Soft Matter Phys       Date:  2013-04-15

10.  Random pinning glass model.

Authors:  Smarajit Karmakar; Giorgio Parisi
Journal:  Proc Natl Acad Sci U S A       Date:  2013-02-04       Impact factor: 11.205

View more
  5 in total

1.  Growing timescales and lengthscales characterizing vibrations of amorphous solids.

Authors:  Ludovic Berthier; Patrick Charbonneau; Yuliang Jin; Giorgio Parisi; Beatriz Seoane; Francesco Zamponi
Journal:  Proc Natl Acad Sci U S A       Date:  2016-07-08       Impact factor: 11.205

2.  Measurements of growing surface tension of amorphous-amorphous interfaces on approaching the colloidal glass transition.

Authors:  Divya Ganapathi; K Hima Nagamanasa; A K Sood; Rajesh Ganapathy
Journal:  Nat Commun       Date:  2018-01-26       Impact factor: 14.919

3.  Differential Variance Analysis: a direct method to quantify and visualize dynamic heterogeneities.

Authors:  Raffaele Pastore; Giuseppe Pesce; Marco Caggioni
Journal:  Sci Rep       Date:  2017-03-14       Impact factor: 4.379

4.  Zero-temperature glass transition in two dimensions.

Authors:  Ludovic Berthier; Patrick Charbonneau; Andrea Ninarello; Misaki Ozawa; Sho Yaida
Journal:  Nat Commun       Date:  2019-04-03       Impact factor: 14.919

5.  Systems with Size and Energy Polydispersity: From Glasses to Mosaic Crystals.

Authors:  Itay Azizi; Yitzhak Rabin
Journal:  Entropy (Basel)       Date:  2020-05-19       Impact factor: 2.524

  5 in total

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