| Literature DB >> 26038545 |
Abstract
The possible role of growing static order in the dynamical slowing down toward the glass transition has recently attracted considerable attention. On the basis of random first-order transition theory, a new method to measure the static correlation length of amorphous order, called "point-to-set" (PTS) length, has been proposed and used to show that the dynamic length grows much faster than the static length. Here, we study the nature of the PTS length, using a polydisperse hard-disk system, which is a model that is known to exhibit a growing hexatic order upon densification. We show that the PTS correlation length is decoupled from the steeper increase of the correlation length of hexatic order and dynamic heterogeneity, while closely mirroring the decay length of two-body density correlations. Our results thus provide a clear example that other forms of order can play an important role in the slowing down of the dynamics, casting a serious doubt on the order-agnostic nature of the PTS length and its relevance to slow dynamics, provided that a polydisperse hard-disk system is a typical glass former.Keywords: glass transition; hexatic order; pinning; slow dynamics; structural length scales
Year: 2015 PMID: 26038545 PMCID: PMC4460450 DOI: 10.1073/pnas.1501911112
Source DB: PubMed Journal: Proc Natl Acad Sci U S A ISSN: 0027-8424 Impact factor: 11.205