| Literature DB >> 24082108 |
Anuj Girdhar1, Chaitanya Sathe, Klaus Schulten, Jean-Pierre Leburton.
Abstract
By using the nonequilibrium Green's function technique, we show that the shape of the edge, the carrier concentration, and the position and size of a nanopore in graphene nanoribbons can strongly affect its electronic conductance as well as its sensitivity to external charges. This technique, combined with a self-consistent Poisson-Boltzmann formalism to account for ion charge screening in solution, is able to detect the rotational and positional conformation of a DNA strand inside the nanopore. In particular, we show that a graphene membrane with quantum point contact geometry exhibits greater electrical sensitivity than a uniform armchair geometry provided that the carrier concentration is tuned to enhance charge detection. We propose a membrane design that contains an electrical gate in a configuration similar to a field-effect transistor for a graphene-based DNA sensing device.Entities:
Keywords: bio-molecule; simulation; solid-state membrane; transport
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Year: 2013 PMID: 24082108 PMCID: PMC3801026 DOI: 10.1073/pnas.1308885110
Source DB: PubMed Journal: Proc Natl Acad Sci U S A ISSN: 0027-8424 Impact factor: 11.205