Literature DB >> 12144405

Geometrical explanation and scaling of dynamical heterogeneities in glass forming systems.

Juan P Garrahan1, David Chandler.   

Abstract

We show how dynamical heterogeneities in glass forming systems emerge as a consequence of the existence of dynamical constraints, and we offer an interpretation of the glass transition as an entropy crisis in trajectory space (space-time) rather than in configuration space. To illustrate our general ideas, we analyze the one-dimensional (d = 1) Fredrickson-Andersen and East models. Dynamics of such dynamically constrained systems are shown to be isomorphic to the statics of ( d + 1)-dimensional dense mixtures of polydisperse noninterpenetrating domains. The domains coincide with arrested regions in trajectory space.

Year:  2002        PMID: 12144405     DOI: 10.1103/PhysRevLett.89.035704

Source DB:  PubMed          Journal:  Phys Rev Lett        ISSN: 0031-9007            Impact factor:   9.161


  10 in total

1.  Coarse-grained microscopic model of glass formers.

Authors:  Juan P Garrahan; David Chandler
Journal:  Proc Natl Acad Sci U S A       Date:  2003-08-04       Impact factor: 11.205

2.  Finite-temperature critical point of a glass transition.

Authors:  Yael S Elmatad; Robert L Jack; David Chandler; Juan P Garrahan
Journal:  Proc Natl Acad Sci U S A       Date:  2010-07-02       Impact factor: 11.205

3.  Transport properties of glass-forming liquids suggest that dynamic crossover temperature is as important as the glass transition temperature.

Authors:  Francesco Mallamace; Caterina Branca; Carmelo Corsaro; Nancy Leone; Jeroen Spooren; Sow-Hsin Chen; H Eugene Stanley
Journal:  Proc Natl Acad Sci U S A       Date:  2010-12-08       Impact factor: 11.205

4.  Dynamical facilitation governs glassy dynamics in suspensions of colloidal ellipsoids.

Authors:  Chandan K Mishra; K Hima Nagamanasa; Rajesh Ganapathy; A K Sood; Shreyas Gokhale
Journal:  Proc Natl Acad Sci U S A       Date:  2014-10-13       Impact factor: 11.205

5.  Space-time thermodynamics of the glass transition.

Authors:  Mauro Merolle; Juan P Garrahan; David Chandler
Journal:  Proc Natl Acad Sci U S A       Date:  2005-07-25       Impact factor: 11.205

6.  Spatial dimension and the dynamics of supercooled liquids.

Authors:  Joel D Eaves; David R Reichman
Journal:  Proc Natl Acad Sci U S A       Date:  2009-08-24       Impact factor: 11.205

7.  Molecular random tilings as glasses.

Authors:  Juan P Garrahan; Andrew Stannard; Matthew O Blunt; Peter H Beton
Journal:  Proc Natl Acad Sci U S A       Date:  2009-08-31       Impact factor: 11.205

8.  Biomolecular dynamics: order-disorder transitions and energy landscapes.

Authors:  Paul C Whitford; Karissa Y Sanbonmatsu; José N Onuchic
Journal:  Rep Prog Phys       Date:  2012-06-28

9.  Calorimetric glass transition in a mean-field theory approach.

Authors:  Manuel Sebastian Mariani; Giorgio Parisi; Corrado Rainone
Journal:  Proc Natl Acad Sci U S A       Date:  2015-02-09       Impact factor: 11.205

10.  Interplay between the static ordering and dynamical heterogeneities determining the dynamics of rotation and ordinary liquid phases in 1,6-anhydro-β-D-glucose.

Authors:  O Madejczyk; K Kaminski; E Kaminska; K Jurkiewicz; M Tarnacka; A Burian; M Paluch
Journal:  Sci Rep       Date:  2017-02-06       Impact factor: 4.379

  10 in total

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