Literature DB >> 12900500

Coarse-grained microscopic model of glass formers.

Juan P Garrahan1, David Chandler.   

Abstract

We introduce a coarse-grained model for atomic glass formers. Its elements are physically motivated local microscopic dynamical rules parameterized by observables. Results of the model are established and used to interpret the measured behaviors of supercooled fluids approaching glass transitions. The model predicts the presence of a crossover from hierarchical super-Arrhenius dynamics at short length scales to diffusive Arrhenius dynamics at large length scales. This prediction distinguishes our model from other theories of glass formers and can be tested by experiment.

Year:  2003        PMID: 12900500      PMCID: PMC187830          DOI: 10.1073/pnas.1233719100

Source DB:  PubMed          Journal:  Proc Natl Acad Sci U S A        ISSN: 0027-8424            Impact factor:   11.205


  8 in total

1.  A thermodynamic connection to the fragility of glass-forming liquids.

Authors:  L M Martinez; C A Angell
Journal:  Nature       Date:  2001-04-05       Impact factor: 49.962

2.  Supercooled liquids and the glass transition.

Authors:  P G Debenedetti; F H Stillinger
Journal:  Nature       Date:  2001-03-08       Impact factor: 49.962

3.  Fragilities of liquids predicted from the random first order transition theory of glasses.

Authors:  X Xia; P G Wolynes
Journal:  Proc Natl Acad Sci U S A       Date:  2000-03-28       Impact factor: 11.205

4.  Spatially heterogeneous dynamics in supercooled liquids.

Authors:  M D Ediger
Journal:  Annu Rev Phys Chem       Date:  2000       Impact factor: 12.703

5.  Geometrical explanation and scaling of dynamical heterogeneities in glass forming systems.

Authors:  Juan P Garrahan; David Chandler
Journal:  Phys Rev Lett       Date:  2002-07-01       Impact factor: 9.161

6.  Elastic and viscoelastic properties of amorphous selenium and identification of the phase transition between ring and chain structures.

Authors: 
Journal:  Phys Rev B Condens Matter       Date:  1993-09-01

7.  Viscous flow in supercooled liquids analyzed in terms of transport theory for random media with energetic disorder.

Authors: 
Journal:  Phys Rev Lett       Date:  1987-02-23       Impact factor: 9.161

8.  Formation of glasses from liquids and biopolymers.

Authors:  C A Angell
Journal:  Science       Date:  1995-03-31       Impact factor: 47.728

  8 in total
  14 in total

1.  Testing "microscopic" theories of glass-forming liquids.

Authors:  L Berthier; G Tarjus
Journal:  Eur Phys J E Soft Matter       Date:  2011-09-23       Impact factor: 1.890

2.  The role of the dynamic crossover temperature and the arrest in glass-forming fluids.

Authors:  F Mallamace; C Corsaro; H E Stanley; S-H Chen
Journal:  Eur Phys J E Soft Matter       Date:  2011-09-23       Impact factor: 1.890

3.  Finite-temperature critical point of a glass transition.

Authors:  Yael S Elmatad; Robert L Jack; David Chandler; Juan P Garrahan
Journal:  Proc Natl Acad Sci U S A       Date:  2010-07-02       Impact factor: 11.205

4.  Transport properties of glass-forming liquids suggest that dynamic crossover temperature is as important as the glass transition temperature.

Authors:  Francesco Mallamace; Caterina Branca; Carmelo Corsaro; Nancy Leone; Jeroen Spooren; Sow-Hsin Chen; H Eugene Stanley
Journal:  Proc Natl Acad Sci U S A       Date:  2010-12-08       Impact factor: 11.205

5.  Relation between the Widom line and the dynamic crossover in systems with a liquid-liquid phase transition.

Authors:  Limei Xu; Pradeep Kumar; S V Buldyrev; S-H Chen; P H Poole; F Sciortino; H E Stanley
Journal:  Proc Natl Acad Sci U S A       Date:  2005-11-02       Impact factor: 11.205

6.  Molecular dynamics studies of heterogeneous dynamics and dynamic crossover in supercooled atomic liquids.

Authors:  Hans C Andersen
Journal:  Proc Natl Acad Sci U S A       Date:  2005-05-03       Impact factor: 11.205

7.  Space-time thermodynamics of the glass transition.

Authors:  Mauro Merolle; Juan P Garrahan; David Chandler
Journal:  Proc Natl Acad Sci U S A       Date:  2005-07-25       Impact factor: 11.205

8.  Dimensional study of the caging order parameter at the glass transition.

Authors:  Patrick Charbonneau; Atsushi Ikeda; Giorgio Parisi; Francesco Zamponi
Journal:  Proc Natl Acad Sci U S A       Date:  2012-08-13       Impact factor: 11.205

9.  Fragile-to-strong crossover in supercooled liquids remains elusive.

Authors:  Yael Sarah Elmatad
Journal:  Proc Natl Acad Sci U S A       Date:  2011-06-16       Impact factor: 11.205

10.  Critical-like behaviour of glass-forming liquids.

Authors:  Hajime Tanaka; Takeshi Kawasaki; Hiroshi Shintani; Keiji Watanabe
Journal:  Nat Mater       Date:  2010-02-21       Impact factor: 43.841

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