Literature DB >> 19706396

Spatial dimension and the dynamics of supercooled liquids.

Joel D Eaves1, David R Reichman.   

Abstract

Inspired by recent theories that apply ideas from critical phenomena to the glass transition, we have simulated an atomistic model of a supercooled liquid in three and four spatial dimensions. At the appropriate temperatures and density, dynamic density correlation functions in three and four spatial dimensions correspond nearly exactly. Dynamic heterogeneity, quantified through the breakdown of the Stokes-Einstein relationship, is weaker in four dimensions than in three. We discuss this in the context of recent theories for dynamical heterogeneity. Because dimensionality is a crucially important variable, our work adds a stringent test for emerging theories of glassy dynamics.

Mesh:

Year:  2009        PMID: 19706396      PMCID: PMC2741223          DOI: 10.1073/pnas.0902888106

Source DB:  PubMed          Journal:  Proc Natl Acad Sci U S A        ISSN: 0027-8424            Impact factor:   11.205


  29 in total

1.  Spatially heterogeneous dynamics in supercooled liquids.

Authors:  M D Ediger
Journal:  Annu Rev Phys Chem       Date:  2000       Impact factor: 12.703

2.  Nature of the spin glass state.

Authors:  M Palassini; A P Young
Journal:  Phys Rev Lett       Date:  2000-10-02       Impact factor: 9.161

3.  Time and length scales in supercooled liquids.

Authors:  Ludovic Berthier
Journal:  Phys Rev E Stat Nonlin Soft Matter Phys       Date:  2004-02-27

4.  On the Adam-Gibbs-Kirkpatrick-Thirumalai-Wolynes scenario for the viscosity increase in glasses.

Authors:  Jean-Philippe Bouchaud; Giulio Biroli
Journal:  J Chem Phys       Date:  2004-10-15       Impact factor: 3.488

5.  Tests of an approximate scaling principle for dynamics of classical fluids.

Authors:  Thomas Young; Hans C Andersen
Journal:  J Phys Chem B       Date:  2005-02-24       Impact factor: 2.991

6.  Inhomogeneous mode-coupling theory and growing dynamic length in supercooled liquids.

Authors:  Giulio Biroli; Jean-Philippe Bouchaud; Kunimasa Miyazaki; David R Reichman
Journal:  Phys Rev Lett       Date:  2006-11-06       Impact factor: 9.161

7.  Activated hopping and dynamical fluctuation effects in hard sphere suspensions and fluids.

Authors:  Erica J Saltzman; Kenneth S Schweizer
Journal:  J Chem Phys       Date:  2006-07-28       Impact factor: 3.488

8.  Search for a correlation length in a simulation of the glass transition.

Authors: 
Journal:  Phys Rev B Condens Matter       Date:  1991-04-01

9.  Translation-rotation paradox for diffusion in fragile glass-forming liquids.

Authors: 
Journal:  Phys Rev E Stat Phys Plasmas Fluids Relat Interdiscip Topics       Date:  1994-09

10.  Kinetic structure of a two-dimensional liquid.

Authors: 
Journal:  Phys Rev E Stat Phys Plasmas Fluids Relat Interdiscip Topics       Date:  1995-08
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  6 in total

1.  When Brownian diffusion is not Gaussian.

Authors:  Bo Wang; James Kuo; Sung Chul Bae; Steve Granick
Journal:  Nat Mater       Date:  2012-05-22       Impact factor: 43.841

2.  Liquids and structural glasses special feature: liquids: condensed, disordered, and sometimes complex.

Authors:  David Chandler
Journal:  Proc Natl Acad Sci U S A       Date:  2009-09-08       Impact factor: 11.205

3.  Diffusing diffusivity: Rotational diffusion in two and three dimensions.

Authors:  Rohit Jain; K L Sebastian
Journal:  J Chem Phys       Date:  2017-06-07       Impact factor: 3.488

4.  Hopping and the Stokes-Einstein relation breakdown in simple glass formers.

Authors:  Patrick Charbonneau; Yuliang Jin; Giorgio Parisi; Francesco Zamponi
Journal:  Proc Natl Acad Sci U S A       Date:  2014-10-06       Impact factor: 11.205

5.  Escape rate and diffusion of a Stochastically Driven particle.

Authors:  Antonio Piscitelli; Massimo Pica Ciamarra
Journal:  Sci Rep       Date:  2017-01-25       Impact factor: 4.379

6.  A Novel Physical Mechanism to Model Brownian Yet Non-Gaussian Diffusion: Theory and Application.

Authors:  Francisco E Alban-Chacón; Erick A Lamilla-Rubio; Manuel S Alvarez-Alvarado
Journal:  Materials (Basel)       Date:  2022-08-23       Impact factor: 3.748

  6 in total

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