Literature DB >> 32094180

Pinching a glass reveals key properties of its soft spots.

Corrado Rainone1, Eran Bouchbinder2, Edan Lerner3.   

Abstract

It is now well established that glasses feature quasilocalized nonphononic excitations-coined "soft spots"-, which follow a universal [Formula: see text] density of states in the limit of low frequencies ω. All glass-specific properties, such as the dependence on the preparation protocol or composition, are encapsulated in the nonuniversal prefactor of the universal [Formula: see text] law. The prefactor, however, is a composite quantity that incorporates information both about the number of quasilocalized nonphononic excitations and their characteristic stiffness, in an apparently inseparable manner. We show that by pinching a glass-i.e., by probing its response to force dipoles-one can disentangle and independently extract these two fundamental pieces of physical information. This analysis reveals that the number of quasilocalized nonphononic excitations follows a Boltzmann-like law in terms of the parent temperature from which the glass is quenched. The latter, sometimes termed the fictive (or effective) temperature, plays important roles in nonequilibrium thermodynamic approaches to the relaxation, flow, and deformation of glasses. The analysis also shows that the characteristic stiffness of quasilocalized nonphononic excitations can be related to their characteristic size, a long sought-for length scale. These results show that important physical information, which is relevant for various key questions in glass physics, can be obtained through pinching a glass.

Entities:  

Keywords:  density of states; elasticity; glasses

Year:  2020        PMID: 32094180      PMCID: PMC7071925          DOI: 10.1073/pnas.1919958117

Source DB:  PubMed          Journal:  Proc Natl Acad Sci U S A        ISSN: 0027-8424            Impact factor:   11.205


  42 in total

1.  On the Adam-Gibbs-Kirkpatrick-Thirumalai-Wolynes scenario for the viscosity increase in glasses.

Authors:  Jean-Philippe Bouchaud; Giulio Biroli
Journal:  J Chem Phys       Date:  2004-10-15       Impact factor: 3.488

2.  Low-frequency vibrations in a model glass.

Authors: 
Journal:  Phys Rev B Condens Matter       Date:  1996-05-01

3.  Dynamic heterogeneities, boson peak, and activation volume in glass-forming liquids.

Authors:  L Hong; V N Novikov; A P Sokolov
Journal:  Phys Rev E Stat Nonlin Soft Matter Phys       Date:  2011-06-30

4.  Local thermal energy as a structural indicator in glasses.

Authors:  Jacques Zylberg; Edan Lerner; Yohai Bar-Sinai; Eran Bouchbinder
Journal:  Proc Natl Acad Sci U S A       Date:  2017-06-27       Impact factor: 11.205

5.  Random critical point separates brittle and ductile yielding transitions in amorphous materials.

Authors:  Misaki Ozawa; Ludovic Berthier; Giulio Biroli; Alberto Rosso; Gilles Tarjus
Journal:  Proc Natl Acad Sci U S A       Date:  2018-06-11       Impact factor: 11.205

6.  A characteristic energy scale in glasses.

Authors:  Edan Lerner; Eran Bouchbinder
Journal:  J Chem Phys       Date:  2018-06-07       Impact factor: 3.488

7.  Breakdown of continuum elasticity in amorphous solids.

Authors:  Edan Lerner; Eric DeGiuli; Gustavo Düring; Matthieu Wyart
Journal:  Soft Matter       Date:  2014-07-28       Impact factor: 3.679

8.  Effect of instantaneous and continuous quenches on the density of vibrational modes in model glasses.

Authors:  Edan Lerner; Eran Bouchbinder
Journal:  Phys Rev E       Date:  2017-08-28       Impact factor: 2.529

9.  Universal spectrum of normal modes in low-temperature glasses.

Authors:  Silvio Franz; Giorgio Parisi; Pierfrancesco Urbani; Francesco Zamponi
Journal:  Proc Natl Acad Sci U S A       Date:  2015-11-11       Impact factor: 11.205

10.  Mechanical glass transition revealed by the fracture toughness of metallic glasses.

Authors:  Jittisa Ketkaew; Wen Chen; Hui Wang; Amit Datye; Meng Fan; Gabriela Pereira; Udo D Schwarz; Ze Liu; Rui Yamada; Wojciech Dmowski; Mark D Shattuck; Corey S O'Hern; Takeshi Egami; Eran Bouchbinder; Jan Schroers
Journal:  Nat Commun       Date:  2018-08-16       Impact factor: 14.919

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