Literature DB >> 22522933

Spin-orbital separation in the quasi-one-dimensional Mott insulator Sr2CuO3.

J Schlappa1, K Wohlfeld, K J Zhou, M Mourigal, M W Haverkort, V N Strocov, L Hozoi, C Monney, S Nishimoto, S Singh, A Revcolevschi, J-S Caux, L Patthey, H M Rønnow, J van den Brink, T Schmitt.   

Abstract

When viewed as an elementary particle, the electron has spin and charge. When binding to the atomic nucleus, it also acquires an angular momentum quantum number corresponding to the quantized atomic orbital it occupies. Even if electrons in solids form bands and delocalize from the nuclei, in Mott insulators they retain their three fundamental quantum numbers: spin, charge and orbital. The hallmark of one-dimensional physics is a breaking up of the elementary electron into its separate degrees of freedom. The separation of the electron into independent quasi-particles that carry either spin (spinons) or charge (holons) was first observed fifteen years ago. Here we report observation of the separation of the orbital degree of freedom (orbiton) using resonant inelastic X-ray scattering on the one-dimensional Mott insulator Sr2CuO3. We resolve an orbiton separating itself from spinons and propagating through the lattice as a distinct quasi-particle with a substantial dispersion in energy over momentum, of about 0.2 electronvolts, over nearly one Brillouin zone.

Entities:  

Year:  2012        PMID: 22522933     DOI: 10.1038/nature10974

Source DB:  PubMed          Journal:  Nature        ISSN: 0028-0836            Impact factor:   49.962


  15 in total

1.  Fractionalization in the cuprates: detecting the topological order.

Authors:  T Senthil; M P Fisher
Journal:  Phys Rev Lett       Date:  2001-01-08       Impact factor: 9.161

2.  Observation of Spin-Charge Separation in One-Dimensional SrCuO2.

Authors: 
Journal:  Phys Rev Lett       Date:  1996-11-04       Impact factor: 9.161

3.  Experimental quest for orbital waves.

Authors:  M Grüninger; R Rückamp; M Windt; P Reutler; C Zobel; T Lorenz; A Freimuth; A Revcolevschi
Journal:  Nature       Date:  2002-07-04       Impact factor: 49.962

4.  Intrinsic coupling of orbital excitations to spin fluctuations in Mott insulators.

Authors:  Krzysztof Wohlfeld; Maria Daghofer; Satoshi Nishimoto; Giniyat Khaliullin; Jeroen van den Brink
Journal:  Phys Rev Lett       Date:  2011-09-29       Impact factor: 9.161

5.  Two-spinon and orbital excitations of the spin-Peierls system TiOCl.

Authors:  S Glawion; J Heidler; M W Haverkort; L C Duda; T Schmitt; V N Strocov; C Monney; K J Zhou; A Ruff; M Sing; R Claessen
Journal:  Phys Rev Lett       Date:  2011-09-01       Impact factor: 9.161

6.  Magnetic excitations and phase separation in the underdoped La2-xSrxCuO4 superconductor measured by resonant inelastic X-ray scattering.

Authors:  L Braicovich; J van den Brink; V Bisogni; M Moretti Sala; L J P Ament; N B Brookes; G M De Luca; M Salluzzo; T Schmitt; V N Strocov; G Ghiringhelli
Journal:  Phys Rev Lett       Date:  2010-02-19       Impact factor: 9.161

7.  The Resonating Valence Bond State in La2CuO4 and Superconductivity.

Authors:  P W Anderson
Journal:  Science       Date:  1987-03-06       Impact factor: 47.728

8.  Theoretical demonstration of how the dispersion of magnetic excitations in cuprate compounds can be determined using resonant inelastic X-ray scattering.

Authors:  Luuk J P Ament; Giacomo Ghiringhelli; Marco Moretti Sala; Lucio Braicovich; Jeroen van den Brink
Journal:  Phys Rev Lett       Date:  2009-09-11       Impact factor: 9.161

9.  Theory of resonant inelastic x-ray scattering by collective magnetic excitations.

Authors:  M W Haverkort
Journal:  Phys Rev Lett       Date:  2010-10-15       Impact factor: 9.161

10.  Ab Initio determination of Cu 3d orbital energies in layered copper oxides.

Authors:  Liviu Hozoi; Liudmila Siurakshina; Peter Fulde; Jeroen van den Brink
Journal:  Sci Rep       Date:  2011-08-16       Impact factor: 4.379

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  19 in total

1.  Solid-state physics: Electrons do the split.

Authors:  Ralph Claessen
Journal:  Nature       Date:  2012-04-18       Impact factor: 49.962

2.  Stimulated X-ray emission for materials science.

Authors:  M Beye; S Schreck; F Sorgenfrei; C Trabant; N Pontius; C Schüßler-Langeheine; W Wurth; A Föhlisch
Journal:  Nature       Date:  2013-08-21       Impact factor: 49.962

3.  L-edge spectroscopy of dilute, radiation-sensitive systems using a transition-edge-sensor array.

Authors:  Charles J Titus; Michael L Baker; Sang Jun Lee; Hsiao-Mei Cho; William B Doriese; Joseph W Fowler; Kelly Gaffney; Johnathon D Gard; Gene C Hilton; Chris Kenney; Jason Knight; Dale Li; Ronald Marks; Michael P Minitti; Kelsey M Morgan; Galen C O'Neil; Carl D Reintsema; Daniel R Schmidt; Dimosthenis Sokaras; Daniel S Swetz; Joel N Ullom; Tsu-Chien Weng; Christopher Williams; Betty A Young; Kent D Irwin; Edward I Solomon; Dennis Nordlund
Journal:  J Chem Phys       Date:  2017-12-07       Impact factor: 3.488

4.  Persistent high-energy spin excitations in iron-pnictide superconductors.

Authors:  Ke-Jin Zhou; Yao-Bo Huang; Claude Monney; Xi Dai; Vladimir N Strocov; Nan-Lin Wang; Zhi-Guo Chen; Chenglin Zhang; Pengcheng Dai; Luc Patthey; Jeroen van den Brink; Hong Ding; Thorsten Schmitt
Journal:  Nat Commun       Date:  2013       Impact factor: 14.919

5.  Spin excitations in a single La2CuO4 layer.

Authors:  M P M Dean; R S Springell; C Monney; K J Zhou; J Pereiro; I Božović; B Dalla Piazza; H M Rønnow; E Morenzoni; J van den Brink; T Schmitt; J P Hill
Journal:  Nat Mater       Date:  2012-09-02       Impact factor: 43.841

6.  Self-doping processes between planes and chains in the metal-to-superconductor transition of YBa2Cu3O6.9.

Authors:  M Magnuson; T Schmitt; V N Strocov; J Schlappa; A S Kalabukhov; L-C Duda
Journal:  Sci Rep       Date:  2014-11-12       Impact factor: 4.379

7.  Prospects of high-resolution resonant X-ray inelastic scattering studies on solid materials, liquids and gases at diffraction-limited storage rings.

Authors:  Thorsten Schmitt; Frank M F de Groot; Jan Erik Rubensson
Journal:  J Synchrotron Radiat       Date:  2014-08-31       Impact factor: 2.616

8.  Raman and fluorescence characteristics of resonant inelastic X-ray scattering from doped superconducting cuprates.

Authors:  H Y Huang; C J Jia; Z Y Chen; K Wohlfeld; B Moritz; T P Devereaux; W B Wu; J Okamoto; W S Lee; M Hashimoto; Y He; Z X Shen; Y Yoshida; H Eisaki; C Y Mou; C T Chen; D J Huang
Journal:  Sci Rep       Date:  2016-01-22       Impact factor: 4.379

9.  Improving the energy resolution of bent crystal X-ray spectrometers with position-sensitive detectors.

Authors:  Ari Pekka Honkanen; Roberto Verbeni; Laura Simonelli; Marco Moretti Sala; Ali Al-Zein; Michael Krisch; Giulio Monaco; Simo Huotari
Journal:  J Synchrotron Radiat       Date:  2014-06-12       Impact factor: 2.616

10.  Quenched Magnon excitations by oxygen sublattice reconstruction in (SrCuO2)n/(SrTiO3)2 superlattices.

Authors:  M Dantz; J Pelliciari; D Samal; V Bisogni; Y Huang; P Olalde-Velasco; V N Strocov; G Koster; T Schmitt
Journal:  Sci Rep       Date:  2016-09-12       Impact factor: 4.379

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