Literature DB >> 17155642

Inhomogeneous mode-coupling theory and growing dynamic length in supercooled liquids.

Giulio Biroli1, Jean-Philippe Bouchaud, Kunimasa Miyazaki, David R Reichman.   

Abstract

We extend mode-coupling theory (MCT) to inhomogeneous situations, relevant for supercooled liquid in an external field. We compute the response of the dynamical structure factor to a static inhomogeneous external potential and provide the first direct evidence that the standard formulation of MCT is associated with a diverging length scale. We find that the so-called cages are, in fact, extended objects. Although close to the transition the dynamic length grows as |T-T(c)|(-1/4) in both the beta and alpha regimes, our results suggest that the fractal dimension of correlated clusters is larger in the alpha regime. We derive inhomogeneous MCT equations valid to second order in gradients.

Entities:  

Year:  2006        PMID: 17155642     DOI: 10.1103/PhysRevLett.97.195701

Source DB:  PubMed          Journal:  Phys Rev Lett        ISSN: 0031-9007            Impact factor:   9.161


  14 in total

1.  Growing length and time scales in glass-forming liquids.

Authors:  Smarajit Karmakar; Chandan Dasgupta; Srikanth Sastry
Journal:  Proc Natl Acad Sci U S A       Date:  2009-02-20       Impact factor: 11.205

2.  Spatiotemporal structures in aging and rejuvenating glasses.

Authors:  Peter G Wolynes
Journal:  Proc Natl Acad Sci U S A       Date:  2009-02-02       Impact factor: 11.205

3.  Kinetic theories of dynamics and persistent caging in a one-dimensional lattice gas.

Authors:  Steven M Abel; Ying-Lung Steve Tse; Hans C Andersenb
Journal:  Proc Natl Acad Sci U S A       Date:  2009-06-29       Impact factor: 11.205

4.  Spatial dimension and the dynamics of supercooled liquids.

Authors:  Joel D Eaves; David R Reichman
Journal:  Proc Natl Acad Sci U S A       Date:  2009-08-24       Impact factor: 11.205

5.  Dynamical theory of shear bands in structural glasses.

Authors:  Apiwat Wisitsorasak; Peter G Wolynes
Journal:  Proc Natl Acad Sci U S A       Date:  2017-01-20       Impact factor: 11.205

6.  Bond orientational order in liquids: Towards a unified description of water-like anomalies, liquid-liquid transition, glass transition, and crystallization: Bond orientational order in liquids.

Authors:  Hajime Tanaka
Journal:  Eur Phys J E Soft Matter       Date:  2012-10-31       Impact factor: 1.890

7.  The relationship of dynamical heterogeneity to the Adam-Gibbs and random first-order transition theories of glass formation.

Authors:  Francis W Starr; Jack F Douglas; Srikanth Sastry
Journal:  J Chem Phys       Date:  2013-03-28       Impact factor: 3.488

8.  New conserved structural fields for supercooled liquids.

Authors:  Jean Farago; Alexander Semenov; Stefan Frey; Jörg Baschnagel
Journal:  Eur Phys J E Soft Matter       Date:  2014-06-06       Impact factor: 1.890

9.  Random pinning glass model.

Authors:  Smarajit Karmakar; Giorgio Parisi
Journal:  Proc Natl Acad Sci U S A       Date:  2013-02-04       Impact factor: 11.205

10.  Quantitative field theory of the glass transition.

Authors:  Silvio Franz; Hugo Jacquin; Giorgio Parisi; Pierfrancesco Urbani; Francesco Zamponi
Journal:  Proc Natl Acad Sci U S A       Date:  2012-10-29       Impact factor: 11.205

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