Literature DB >> 17758561

Hole-burning spectroscopy and relaxation dynamics of amorphous solids at low temperatures.

R Jankowiak, G J Small.   

Abstract

The magnitude and temperature dependence of most of the properties of amorphous solids are anomalous at very low temperatures ( less, similar1 Kelvin). Phonon-assisted tunneling of a distribution of glassy bistable configurations, or two-level systems, can account for these anomalies. A unified understanding of the low-temperature properties is required for an understanding of the glassy state. Persistent nonphotochemical hole burning of impurity optical transitions allows a glass state to be produced that is thermally inaccessible to the preburn state, and that allows the probing of tunneling dynamics on time scales that range between picoseconds and days. These data combined with recently obtained distribution functions for the two-level systems offer new insights into the tunneling dynamics.

Year:  1987        PMID: 17758561     DOI: 10.1126/science.237.4815.618

Source DB:  PubMed          Journal:  Science        ISSN: 0036-8075            Impact factor:   47.728


  12 in total

1.  Molecular probes: what is the range of their interaction with the environment?

Authors:  H Lesch; J Schlichter; J Friedrich; J M Vanderkooi
Journal:  Biophys J       Date:  2004-01       Impact factor: 4.033

2.  Aging dynamics in globular proteins: summary and analysis of experimental results and simulation by a modified trap model.

Authors:  Levente Herenyi; Krisztian Szigeti; Judit Fidy; Tamas Temesvari; Jorg Schlichter; Josef Friedrich
Journal:  Eur Biophys J       Date:  2003-09-03       Impact factor: 1.733

3.  Determination of the primary charge separation rate in isolated photosystem II reaction centers with 500-fs time resolution.

Authors:  M R Wasielewski; D G Johnson; M Seibert
Journal:  Proc Natl Acad Sci U S A       Date:  1989-01       Impact factor: 11.205

4.  Proteins--paradigms of complex systems.

Authors:  H Frauenfelder
Journal:  Experientia       Date:  1995-03-15

5.  Spectral hole burning of the primary electron donor state of Photosystem I.

Authors:  J K Gillie; P A Lyle; G J Small; J H Golbeck
Journal:  Photosynth Res       Date:  1989-12       Impact factor: 3.573

6.  Applications of spectral hole burning spectroscopies to antenna and reaction center complexes.

Authors:  N R Reddy; P A Lyle; G J Small
Journal:  Photosynth Res       Date:  1992-03       Impact factor: 3.573

7.  Aluminum phthalocyanine tetrasulfonate in MCF-10F, human breast epithelial cells: a hole burning study.

Authors:  N Milanovich; T Reinot; J M Hayes; G J Small
Journal:  Biophys J       Date:  1998-05       Impact factor: 4.033

8.  Engineering dissipation with phononic spectral hole burning.

Authors:  R O Behunin; P Kharel; W H Renninger; P T Rakich
Journal:  Nat Mater       Date:  2016-12-12       Impact factor: 43.841

Review 9.  Spectral hole burning: examples from photosynthesis.

Authors:  Robin Purchase; Silvia Völker
Journal:  Photosynth Res       Date:  2009 Aug-Sep       Impact factor: 3.573

10.  Determination of the primary charge separation rate in Photosystem II reaction centers at 15 K.

Authors:  M R Wasielewski; D G Johnson; C Preston; M Seibert
Journal:  Photosynth Res       Date:  1989-01       Impact factor: 3.573

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