Literature DB >> 15447415

Does the interaction potential determine both the fragility of a liquid and the vibrational properties of its glassy state?

Patrice Bordat1, Frédéric Affouard, Marc Descamps, K L Ngai.   

Abstract

By performing molecular dynamics simulations of binary Lennard-Jones systems with three different potentials, we show that the increase of anharmonicity and capacity for intermolecular coupling of the potential is the cause of (i) the increase of kinetic fragility and nonexponentiality in the liquid state, and (ii) the T(g)-scaled temperature dependence of the nonergodicity parameter determined by the vibrations at low temperatures in the glassy state. Naturally, these parameters correlate with each other, as observed experimentally by T. Scopigno et al. [Science 302, 849 (2003)]

Entities:  

Year:  2004        PMID: 15447415     DOI: 10.1103/PhysRevLett.93.105502

Source DB:  PubMed          Journal:  Phys Rev Lett        ISSN: 0031-9007            Impact factor:   9.161


  14 in total

1.  Interatomic repulsion softness directly controls the fragility of supercooled metallic melts.

Authors:  Johannes Krausser; Konrad H Samwer; Alessio Zaccone
Journal:  Proc Natl Acad Sci U S A       Date:  2015-10-26       Impact factor: 11.205

2.  The kinetic fragility of liquids as manifestation of the elastic softening.

Authors:  F Puosi; D Leporini
Journal:  Eur Phys J E Soft Matter       Date:  2015-08-13       Impact factor: 1.890

3.  Strength of the repulsive part of the interatomic potential determines fragility in metallic liquids.

Authors:  Christopher E Pueblo; Minhua Sun; K F Kelton
Journal:  Nat Mater       Date:  2017-07-10       Impact factor: 43.841

4.  A universal modified van der Waals equation of state. Part I: Polymer and mineral glass formers.

Authors:  Jacques Rault
Journal:  Eur Phys J E Soft Matter       Date:  2014-11-20       Impact factor: 1.890

5.  Vibrational scaling of the heterogeneous dynamics detected by mutual information.

Authors:  Antonio Tripodo; Francesco Puosi; Marco Malvaldi; Dino Leporini
Journal:  Eur Phys J E Soft Matter       Date:  2019-11-22       Impact factor: 1.890

6.  Dynamical behavior of microgels of interpenetrated polymer networks.

Authors:  Valentina Nigro; Roberta Angelini; Monica Bertoldo; Fabio Bruni; Maria Antonietta Ricci; Barbara Ruzicka
Journal:  Soft Matter       Date:  2017-08-02       Impact factor: 3.679

7.  Probing equilibrium glass flow up to exapoise viscosities.

Authors:  Eva Arianna Aurelia Pogna; Cristian Rodríguez-Tinoco; Giulio Cerullo; Carino Ferrante; Javier Rodríguez-Viejo; Tullio Scopigno
Journal:  Proc Natl Acad Sci U S A       Date:  2015-02-09       Impact factor: 11.205

8.  Glass-Forming Tendency of Molecular Liquids and the Strength of the Intermolecular Attractions.

Authors:  Kajetan Koperwas; Karolina Adrjanowicz; Zaneta Wojnarowska; Agnieszka Jedrzejowska; Justyna Knapik; Marian Paluch
Journal:  Sci Rep       Date:  2016-11-24       Impact factor: 4.379

9.  Plastic Deformation of Pressured Metallic Glass.

Authors:  Yun Cheng; Chuanxiao Peng; Zhenting Zhang; Pengfei Wang; Shengzhong Yuan; Li Wang
Journal:  Materials (Basel)       Date:  2017-11-27       Impact factor: 3.623

10.  Structural rearrangements governing Johari-Goldstein relaxations in metallic glasses.

Authors:  Hai-Bin Yu; Ranko Richert; Konrad Samwer
Journal:  Sci Adv       Date:  2017-11-17       Impact factor: 14.136

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