Literature DB >> 35338141

High-speed 4D neutron computed tomography for quantifying water dynamics in polymer electrolyte fuel cells.

Ralf F Ziesche1,2,3,4, Jennifer Hack1, Lara Rasha1, Maximilian Maier1, Chun Tan1,2, Thomas M M Heenan1,2, Henning Markötter5,6,7, Nikolay Kardjilov5, Ingo Manke5, Winfried Kockelmann4, Dan J L Brett1,2, Paul R Shearing8,9.   

Abstract

In recent years, low-temperature polymer electrolyte fuel cells have become an increasingly important pillar in a zero-carbon strategy for curbing climate change, with their potential to power multiscale stationary and mobile applications. The performance improvement is a particular focus of research and engineering roadmaps, with water management being one of the major areas of interest for development. Appropriate characterisation tools for mapping the evolution, motion and removal of water are of high importance to tackle shortcomings. This article demonstrates the development of a 4D high-speed neutron imaging technique, which enables a quantitative analysis of the local water evolution. 4D visualisation allows the time-resolved studies of droplet formation in the flow fields and water quantification in various cell parts. Performance parameters for water management are identified that offer a method of cell classification, which will, in turn, support computer modelling and the engineering of next-generation flow field designs.
© 2022. The Author(s).

Entities:  

Year:  2022        PMID: 35338141      PMCID: PMC8956593          DOI: 10.1038/s41467-022-29313-5

Source DB:  PubMed          Journal:  Nat Commun        ISSN: 2041-1723            Impact factor:   17.694


  7 in total

1.  Investigation of the role of the micro-porous layer in polymer electrolyte fuel cells with hydrogen deuterium contrast neutron radiography.

Authors:  Kyu Taek Cho; Matthew M Mench
Journal:  Phys Chem Chem Phys       Date:  2012-02-15       Impact factor: 3.676

2.  The ASTRA Toolbox: A platform for advanced algorithm development in electron tomography.

Authors:  Wim van Aarle; Willem Jan Palenstijn; Jan De Beenhouwer; Thomas Altantzis; Sara Bals; K Joost Batenburg; Jan Sijbers
Journal:  Ultramicroscopy       Date:  2015-05-06       Impact factor: 2.689

3.  Fast and flexible X-ray tomography using the ASTRA toolbox.

Authors:  Wim van Aarle; Willem Jan Palenstijn; Jeroen Cant; Eline Janssens; Folkert Bleichrodt; Andrei Dabravolski; Jan De Beenhouwer; K Joost Batenburg; Jan Sijbers
Journal:  Opt Express       Date:  2016-10-31       Impact factor: 3.894

4.  In Operando Quantification of Three-Dimensional Water Distribution in Nanoporous Carbon-Based Layers in Polymer Electrolyte Membrane Fuel Cells.

Authors:  Saad S Alrwashdeh; Ingo Manke; Henning Markötter; Merle Klages; Martin Göbel; Jan Haußmann; Joachim Scholta; John Banhart
Journal:  ACS Nano       Date:  2017-05-30       Impact factor: 15.881

5.  Polymer electrolyte fuel cell performance degradation at different synchrotron beam intensities.

Authors:  Jens Eller; Felix N Büchi
Journal:  J Synchrotron Radiat       Date:  2013-11-02       Impact factor: 2.616

6.  Capturing 3D Water Flow in Rooted Soil by Ultra-fast Neutron Tomography.

Authors:  Christian Tötzke; Nikolay Kardjilov; Ingo Manke; Sascha E Oswald
Journal:  Sci Rep       Date:  2017-07-21       Impact factor: 4.379

7.  Ror2 signaling regulates Golgi structure and transport through IFT20 for tumor invasiveness.

Authors:  Michiru Nishita; Seung-Yeol Park; Tadashi Nishio; Koki Kamizaki; ZhiChao Wang; Kota Tamada; Toru Takumi; Ryuju Hashimoto; Hiroki Otani; Gregory J Pazour; Victor W Hsu; Yasuhiro Minami
Journal:  Sci Rep       Date:  2017-01-26       Impact factor: 4.379

  7 in total

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