Literature DB >> 33953436

Microwave-Assisted Synthesis of Organometallic Rhenium (I) Pentylcarbonato Complexes: New Synthon for Carboxylato, Sulfonato and Chlorido Complexes.

Angela J Winstead1, Khayra Alabrash1, Brent V Powell1, Sabreea J Parnell1, Tiara V Hinton1, Tijesunimi Odebode1, Jiangnan Peng1, Jeanette A Krause2, Peter Y Zavalij3, Santosh K Mandal1.   

Abstract

Tricarbonylrhenium(I)(α-diimine) complexes are of importance because of their strong cytotoxic and fluorescence properties. Syntheses of such complexes were achieved through a two-step process. First, the n class="Chemical">pentylcarbonato complexes, fac-(CO)3(α-diimine)ReOC(O)OC5H11 were synthesized through a microwave-assisted reaction of Re2(CO)10, α-diimine, 1-pentanol and CO2 in a few hours. Second, the pentylcarbonato complexes are treated with carboxylic, sulfonic and halo acids to obtain the corresponding carboxylato, sulfonato and halido complexes. This is the first example of conversion of Re2(CO)10 into a rhenium carbonyl complex through microwave-assisted reaction.

Entities:  

Keywords:  Rhenium decacarbonyl; carboxylate; chloride; microwave-assisted; pentyl carbonate; sulfonate; α-diimines

Year:  2021        PMID: 33953436      PMCID: PMC8095682          DOI: 10.1016/j.jorganchem.2021.121718

Source DB:  PubMed          Journal:  J Organomet Chem        ISSN: 0022-328X            Impact factor:   2.369


  8 in total

1.  DNA binding and cytotoxicity of ruthenium(II) and rhenium(I) complexes of 2-amino-4-phenylamino-6-(2-pyridyl)-1,3,5-triazine.

Authors:  Dik-Lung Ma; Chi-Ming Che; Fung-Ming Siu; Mengsu Yang; Kwok-Yin Wong
Journal:  Inorg Chem       Date:  2007-02-05       Impact factor: 5.165

2.  Unprecedented anticancer activities of organorhenium sulfonato and carboxylato complexes against hormone-dependent MCF-7 and hormone-independent triple-negative MDA-MB-231 breast cancer cells.

Authors:  Paul T Wilder; David J Weber; Angela Winstead; Sabreea Parnell; Tiara V Hinton; Monet Stevenson; Dipak Giri; Samira Azemati; Pola Olczak; Brent V Powell; Tijesunimi Odebode; Solomon Tadesse; Yongchao Zhang; Saroj K Pramanik; James M Wachira; Sujan Ghimire; Pumtiwitt McCarthy; Alexis Barfield; Hirendra N Banerjee; Chao Chen; James A Golen; Arnold L Rheingold; Jeanette A Krause; Douglas M Ho; Peter Y Zavalij; Roosevelt Shaw; Santosh K Mandal
Journal:  Mol Cell Biochem       Date:  2017-09-14       Impact factor: 3.396

3.  Microwave-assisted synthesis of tricarbonyl rhenacarboranes: steric and electronic effects on the 1,2 --> 1,7 carborane cage isomerization.

Authors:  Andrea F Armstrong; John F Valliant
Journal:  Inorg Chem       Date:  2007-02-16       Impact factor: 5.165

4.  Microwave-assisted synthesis of organometallic complexes of ⁹⁹mTc(CO)₃ and Re(CO)₃: its application to radiopharmaceuticals.

Authors:  Hiroyuki Kimura; Daisuke Mori; Naoya Harada; Masahiro Ono; Yoshiro Ohmomo; Tetsuya Kajimoto; Hidekazu Kawashima; Hideo Saji
Journal:  Chem Pharm Bull (Tokyo)       Date:  2012       Impact factor: 1.645

5.  Microwave-assisted synthesis of 3,1,2- and 2,1,8-Re(I) and 99mTc(I)-metallocarborane complexes.

Authors:  Andrew E C Green; Patrick W Causey; Anika S Louie; Andrea F Armstrong; Laura E Harrington; John F Valliant
Journal:  Inorg Chem       Date:  2006-07-24       Impact factor: 5.165

6.  Chloro-fac-tricarbonylrhenium(I) complexes of asymmetric azines derived from 6-acetyl-1,3,7-trimethylpteridine-2,4(1H,3H)-dione with hydrazine and aromatic aldehydes: preparation, structural characterization and biological activity against several human tumor cell lines.

Authors:  Inmaculada Picón-Ferrer; Francisco Hueso-Ureña; Nuria A Illán-Cabeza; Sonia B Jiménez-Pulido; José M Martínez-Martos; María J Ramírez-Expósito; Miguel N Moreno-Carretero
Journal:  J Inorg Biochem       Date:  2008-10-10       Impact factor: 4.155

7.  Expedient multi-step synthesis of organometallic complexes of Tc and Re in high effective specific activity. A new platform for the production of molecular imaging and therapy agents.

Authors:  Patrick W Causey; Travis R Besanger; Paul Schaffer; John F Valliant
Journal:  Inorg Chem       Date:  2008-08-19       Impact factor: 5.165

8.  Carbonic acid monoethyl ester as a pure solid and its conformational isomerism in the gas-phase.

Authors:  Jürgen Bernard; Eva-Maria Köck; Roland G Huber; Klaus R Liedl; Ludwig Call; Robert Schlögl; Hinrich Grothe; Thomas Loerting
Journal:  RSC Adv       Date:  2017-04-21       Impact factor: 3.361

  8 in total
  1 in total

Review 1.  Microwave-Assisted Synthesis: Can Transition Metal Complexes Take Advantage of This "Green" Method?

Authors:  Elisabetta Gabano; Mauro Ravera
Journal:  Molecules       Date:  2022-06-30       Impact factor: 4.927

  1 in total

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