Literature DB >> 33399586

ROBL-II at ESRF: a synchrotron toolbox for actinide research.

Andreas C Scheinost1, Juergen Claussner2, Joerg Exner1, Manuel Feig1, Stefan Findeisen2, Christoph Hennig1, Kristina O Kvashnina1, Damien Naudet1, Damien Prieur1, Andre Rossberg1, Moritz Schmidt3, Canrong Qiu3, Patrick Colomp4, Cedric Cohen4, Eric Dettona4, Vadim Dyadkin5, Thorsten Stumpf3.   

Abstract

ROBL-II provides four different experimental stations to investigate actinide and other alpha- and beta-emitting radionuclides at the new EBS storage ring of ESRF within an energy range of 3 to 35 keV. The XAFS station consists of a highly automatized, high sample throughput installation in a glovebox, to measure EXAFS and conventional XANES of samples routinely at temperatures down to 10 K, and with a detection limit in the sub-p.p.m. range. The XES station with its five bent-crystal analyzer, Johann-type setup with Rowland circles of 1.0 and 0.5 m radii provides high-energy resolution fluorescence detection (HERFD) for XANES, XES, and RIXS measurements, covering both actinide L and M edges together with other elements accessible in the 3 to 20 keV energy range. The six-circle heavy duty goniometer of XRD-1 is equipped for both high-resolution powder diffraction as well as surface-sensitive CTR and RAXR techniques. Single crystal diffraction, powder diffraction with high temporal resolution, as well as X-ray tomography experiments can be performed at a Pilatus 2M detector stage (XRD-2). Elaborate radioprotection features enable a safe and easy exchange of samples between the four different stations to allow the combination of several methods for an unprecedented level of information on radioactive samples for both fundamental and applied actinide and environmental research. open access.

Entities:  

Keywords:  CTR; EXAFS; HERFD-XANES; RAXR; RIXS; XANES; XAS; XES; XRD; actinides; surface diffraction

Year:  2021        PMID: 33399586     DOI: 10.1107/S1600577520014265

Source DB:  PubMed          Journal:  J Synchrotron Radiat        ISSN: 0909-0495            Impact factor:   2.616


  6 in total

1.  Application of multi-edge HERFD-XAS to assess the uranium valence electronic structure in potassium uranate (KUO3).

Authors:  René Bes; Gregory Leinders; Kristina Kvashnina
Journal:  J Synchrotron Radiat       Date:  2022-01-01       Impact factor: 2.616

2.  Implementation of cryogenic tender X-ray HR-XANES spectroscopy at the ACT station of the CAT-ACT beamline at the KIT Light Source.

Authors:  Bianca Schacherl; Tim Prüssmann; Kathy Dardenne; Kirsten Hardock; Volker Krepper; Jörg Rothe; Tonya Vitova; Horst Geckeis
Journal:  J Synchrotron Radiat       Date:  2022-01-01       Impact factor: 2.616

Review 3.  High-energy resolution X-ray spectroscopy at actinide M4,5 and ligand K edges: what we know, what we want to know, and what we can know.

Authors:  Kristina O Kvashnina; Sergei M Butorin
Journal:  Chem Commun (Camb)       Date:  2022-01-04       Impact factor: 6.222

4.  Refinement of anomalous dispersion correction parameters in single-crystal structure determinations.

Authors:  Florian Meurer; Oleg V Dolomanov; Christoph Hennig; Norbert Peyerimhoff; Florian Kleemiss; Horst Puschmann; Michael Bodensteiner
Journal:  IUCrJ       Date:  2022-07-20       Impact factor: 5.588

5.  Pbx(OH)y cluster formation and anomalous thermal behaviour in STI framework-type zeolites.

Authors:  Georgia Cametti; Diana P Roos; Damien Prieur; Andreas C Scheinost; Sergey V Churakov
Journal:  Sci Rep       Date:  2022-09-24       Impact factor: 4.996

6.  Oxidation of Micro- and Nanograined UO2 Pellets by In Situ Synchrotron X-ray Diffraction.

Authors:  Emanuele De Bona; Karin Popa; Olaf Walter; Marco Cologna; Christoph Hennig; Andreas C Scheinost; Damien Prieur
Journal:  Inorg Chem       Date:  2022-01-19       Impact factor: 5.165

  6 in total

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