Literature DB >> 33173234

Interstellar nitrile anions: Detection of C3N- and C5N- in TMC-1.

J Cernicharo1, N Marcelino1, J R Pardo1, M Agúndez1, B Tercero2,3, P de Vicente2, C Cabezas1, C Bermúdez1.   

Abstract

We report on the first detection of n class="Chemical">pan class="Chemical">C3N- and class="Chemical">n>an class="Chemical">C5N- towards the cold dark core TMC-1 in the Taurus region, using the Yebes 40 m telescope. The observed C3N/C3N- and C5N/C5N- abundance ratios are ~140 and ~2, respectively; that is similar to those found in the circumstellar envelope of the carbon-rich star IRC +10216. Although the formation mechanisms for the neutrals are different in interstellar (ion-neutral reactions) and circumstellar clouds (photodissociation and radical-neutral reactions), the similarity of the C3N/C3N- and C5N/C5N- abundance ratios strongly suggests a common chemical path for the formation of these anions in interstellar and circumstellar clouds. We discuss the role of radiative electronic attachment, reactions between N atoms and carbon chain anions C n -, and that of H- reactions with HC3N and HC5N as possible routes to form C n N-. The detection of C5N- in TMC-1 gives strong support for assigning to this anion the lines found in IRC +10216, as it excludes the possibility of a metal-bearing species, or a vibrationally excited state. New sets of rotational parameters have been derived from the observed frequencies in TMC-1 and IRC +10216 for C5N- and the neutral radical C5N.

Entities:  

Keywords:  Astrochemistry; ISM: individual (TMC-1); ISM: molecules; line: identification; molecular data

Year:  2020        PMID: 33173234      PMCID: PMC7116340          DOI: 10.1051/0004-6361/202039231

Source DB:  PubMed          Journal:  Astron Astrophys        ISSN: 0004-6361            Impact factor:   5.802


  7 in total

1.  Is interstellar detection of higher members of the linear radicals CnCH and CnN feasible?

Authors:  F Pauzat; Y Ellinger; A D McLean
Journal:  Astrophys J       Date:  1991-03-01       Impact factor: 5.874

2.  Low-Temperature Reactivity of C2n+1N(-) Anions with Polar Molecules.

Authors:  Baptiste Joalland; Nour Jamal-Eddine; Jacek Kłos; François Lique; Yann Trolez; Jean-Claude Guillemin; Sophie Carles; Ludovic Biennier
Journal:  J Phys Chem Lett       Date:  2016-07-19       Impact factor: 6.475

3.  The rotational spectrum of CN-.

Authors:  C A Gottlieb; S Brünken; M C McCarthy; P Thaddeus
Journal:  J Chem Phys       Date:  2007-05-21       Impact factor: 3.488

4.  Chemistry of dark clouds: databases, networks, and models.

Authors:  Marcelino Agúndez; Valentine Wakelam
Journal:  Chem Rev       Date:  2013-10-07       Impact factor: 60.622

5.  Negative Ions in Space.

Authors:  Thomas J Millar; Catherine Walsh; Thomas A Field
Journal:  Chem Rev       Date:  2017-01-23       Impact factor: 60.622

6.  Carbon chains of type C2n+1N(-) (n=2-6): A theoretical study of potential interstellar anions.

Authors:  Peter Botschwina; Rainer Oswald
Journal:  J Chem Phys       Date:  2008-07-28       Impact factor: 3.488

7.  Extended negative glow and "hollow anode" discharges for submillimeter-wave observation of CN-, C2H-, and C4H-.

Authors:  T Amano
Journal:  J Chem Phys       Date:  2008-12-28       Impact factor: 3.488

  7 in total
  4 in total

1.  Discovery of HC4NC in TMC-1: A study of the isomers of HC3N, HC5N, and HC7N.

Authors:  J Cernicharo; N Marcelino; M Agúndez; C Bermúdez; C Cabezas; B Tercero; J R Pardo
Journal:  Astron Astrophys       Date:  2020-10-07       Impact factor: 5.802

2.  Laboratory microwave spectroscopy of the doubly deuterated cyanomethyl radical, D2CCN.

Authors:  Carlos Cabezas; Yasuki Endo; José Cernicharo
Journal:  J Mol Spectrosc       Date:  2021-03-12       Impact factor: 1.507

3.  Rotational Spectra of Unsaturated Carbon Chains Produced by Pyrolysis: The Case of Propadienone, Cyanovinylacetylene, and Allenylacetylene.

Authors:  Alessio Melli; Mattia Melosso; Luca Bizzocchi; Silvia Alessandrini; Ningjing Jiang; Francesca Tonolo; Salvatore Boi; Giorgia Castellan; Carlotta Sapienza; Jean-Claude Guillemin; Luca Dore; Cristina Puzzarini
Journal:  J Phys Chem A       Date:  2022-08-31       Impact factor: 2.944

Review 4.  Sources of Nitrogen-, Sulfur-, and Phosphorus-Containing Feedstocks for Prebiotic Chemistry in the Planetary Environment.

Authors:  Zoe R Todd
Journal:  Life (Basel)       Date:  2022-08-19
  4 in total

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