| Literature DB >> 31395782 |
Pengfei Yu1,2,3, Owen B Toon4,5, Charles G Bardeen6, Yunqian Zhu5, Karen H Rosenlof2, Robert W Portmann2, Troy D Thornberry7,2, Ru-Shan Gao2, Sean M Davis2, Eric T Wolf5,8, Joost de Gouw7,9, David A Peterson10, Michael D Fromm11, Alan Robock12.
Abstract
In 2017, western Canadian wildfires injected smoke into the stratosphere that was detectable by satellites for more than 8 months. The smoke plume rose from 12 to 23 kilometers within 2 months owing to solar heating of black carbon, extending the lifetime and latitudinal spread. Comparisons of model simulations to the rate of observed lofting indicate that 2% of the smoke mass was black carbon. The observed smoke lifetime in the stratosphere was 40% shorter than calculated with a standard model that does not consider photochemical loss of organic carbon. Photochemistry is represented by using an empirical ozone-organics reaction probability that matches the observed smoke decay. The observed rapid plume rise, latitudinal spread, and photochemical reactions provide new insights into potential global climate impacts from nuclear war.Entities:
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Year: 2019 PMID: 31395782 DOI: 10.1126/science.aax1748
Source DB: PubMed Journal: Science ISSN: 0036-8075 Impact factor: 47.728