Literature DB >> 31251067

Light Harvesting with Guide-Slide Superabsorbing Condensed-Matter Nanostructures.

W M Brown1, E M Gauger1.   

Abstract

We establish design principles for light-harvesting antennae whose energy capture scales superlinearly with system size. Controlling the absorber dipole orientations produces sets of "guide-slide" states that promote steady-state superabsorbing characteristics in noisy condensed-matter nanostructures. Inspired by natural photosynthetic complexes, we discuss the example of ringlike dipole arrangements and show that, in our setup, vibrational relaxation enhances rather than impedes performance. Remarkably, the superabsorption effect proves to be robust to O(5%) disorder simultaneously for all relevant system parameters, showing promise for experimental exploration across a broad range of platforms.

Year:  2019        PMID: 31251067     DOI: 10.1021/acs.jpclett.9b01349

Source DB:  PubMed          Journal:  J Phys Chem Lett        ISSN: 1948-7185            Impact factor:   6.475


  2 in total

1.  Structure-based Hamiltonian model for IsiA uncovers a highly robust pigment-protein complex.

Authors:  Hanan Schoffman; William M Brown; Yossi Paltiel; Nir Keren; Erik M Gauger
Journal:  J R Soc Interface       Date:  2020-08-26       Impact factor: 4.118

2.  Superabsorption in an organic microcavity: Toward a quantum battery.

Authors:  James Q Quach; Kirsty E McGhee; Lucia Ganzer; Dominic M Rouse; Brendon W Lovett; Erik M Gauger; Jonathan Keeling; Giulio Cerullo; David G Lidzey; Tersilla Virgili
Journal:  Sci Adv       Date:  2022-01-14       Impact factor: 14.136

  2 in total

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