Literature DB >> 35030030

Superabsorption in an organic microcavity: Toward a quantum battery.

James Q Quach1, Kirsty E McGhee2, Lucia Ganzer3, Dominic M Rouse4, Brendon W Lovett4, Erik M Gauger5, Jonathan Keeling4, Giulio Cerullo3, David G Lidzey2, Tersilla Virgili3.   

Abstract

The rate at which matter emits or absorbs light can be modified by its environment, as markedly exemplified by the widely studied phenomenon of superradiance. The reverse process, superabsorption, is harder to demonstrate because of the challenges of probing ultrafast processes and has only been seen for small numbers of atoms. Its central idea—superextensive scaling of absorption, meaning larger systems absorb faster—is also the key idea underpinning quantum batteries. Here, we implement experimentally a paradigmatic model of a quantum battery, constructed of a microcavity enclosing a molecular dye. Ultrafast optical spectroscopy allows us to observe charging dynamics at femtosecond resolution to demonstrate superextensive charging rates and storage capacity, in agreement with our theoretical modeling. We find that decoherence plays an important role in stabilizing energy storage. Our work opens future opportunities for harnessing collective effects in light-matter coupling for nanoscale energy capture, storage, and transport technologies.

Entities:  

Year:  2022        PMID: 35030030      PMCID: PMC8759743          DOI: 10.1126/sciadv.abk3160

Source DB:  PubMed          Journal:  Sci Adv        ISSN: 2375-2548            Impact factor:   14.136


  21 in total

1.  Superradiant rayleigh scattering from a bose-einstein condensate

Authors: 
Journal:  Science       Date:  1999-07-23       Impact factor: 47.728

2.  Time-resolved methods in biophysics. 4. Broadband pump-probe spectroscopy system with sub-20 fs temporal resolution for the study of energy transfer processes in photosynthesis.

Authors:  Giulio Cerullo; Cristian Manzoni; Larry Lüer; Dario Polli
Journal:  Photochem Photobiol Sci       Date:  2006-12-08       Impact factor: 3.982

3.  A quantum open system model of molecular battery charged by excitons.

Authors:  Robert Alicki
Journal:  J Chem Phys       Date:  2019-06-07       Impact factor: 3.488

4.  Extractable Work, the Role of Correlations, and Asymptotic Freedom in Quantum Batteries.

Authors:  Gian Marcello Andolina; Maximilian Keck; Andrea Mari; Michele Campisi; Vittorio Giovannetti; Marco Polini
Journal:  Phys Rev Lett       Date:  2019-02-01       Impact factor: 9.161

5.  Entanglement generation is not necessary for optimal work extraction.

Authors:  Karen V Hovhannisyan; Martí Perarnau-Llobet; Marcus Huber; Antonio Acín
Journal:  Phys Rev Lett       Date:  2013-12-09       Impact factor: 9.161

6.  High-Power Collective Charging of a Solid-State Quantum Battery.

Authors:  Dario Ferraro; Michele Campisi; Gian Marcello Andolina; Vittorio Pellegrini; Marco Polini
Journal:  Phys Rev Lett       Date:  2018-03-16       Impact factor: 9.161

Review 7.  Light Harvesting for Organic Photovoltaics.

Authors:  Gordon J Hedley; Arvydas Ruseckas; Ifor D W Samuel
Journal:  Chem Rev       Date:  2016-12-07       Impact factor: 60.622

8.  Superabsorption of light via quantum engineering.

Authors:  K D B Higgins; S C Benjamin; T M Stace; G J Milburn; B W Lovett; E M Gauger
Journal:  Nat Commun       Date:  2014-08-22       Impact factor: 14.919

9.  An exciton-polariton laser based on biologically produced fluorescent protein.

Authors:  Christof P Dietrich; Anja Steude; Laura Tropf; Marcel Schubert; Nils M Kronenberg; Kai Ostermann; Sven Höfling; Malte C Gather
Journal:  Sci Adv       Date:  2016-08-19       Impact factor: 14.136

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  1 in total

1.  Efficiency Fluctuations in a Quantum Battery Charged by a Repeated Interaction Process.

Authors:  Felipe Barra
Journal:  Entropy (Basel)       Date:  2022-06-13       Impact factor: 2.738

  1 in total

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