Literature DB >> 30166450

Franck-Condon picture of incoherent neutron scattering.

Gerald R Kneller1,2.   

Abstract

A spectroscopic interpretation of incoherent neutron scattering experiments is presented which is based on Franck-Condon-type probabilities for scattering-induced transitions between quantum states of the target. The resulting expressions for the scattering functions enable an energy landscape-oriented analysis of neutron scattering spectra as well as a physical interpretation of Van Hove's space-time correlation functions in the quantum regime that accounts for the scattering kinematics. They suggest moreover a combined analysis of quasielastic and elastic scattering that become inseparable for complex systems with slow power-law relaxation.

Keywords:  Van Hove theory; complex systems; energy landscapes; neutron scattering theory; quasielastic neutron scattering

Year:  2018        PMID： 30166450      PMCID： PMC6156675          DOI： 10.1073/pnas.1718720115

Source DB:  PubMed          Journal:  Proc Natl Acad Sci U S A        ISSN： 0027-8424            Impact factor:   11.205


  9 in total

Review 1.  Protein dynamics studied by neutron scattering.

Authors:  Frank Gabel; Dominique Bicout; Ursula Lehnert; Moeava Tehei; Martin Weik; Giuseppe Zaccai
Journal:  Q Rev Biophys       Date:  2002-11       Impact factor: 5.318

2.  The energy landscapes and motions of proteins.

Authors:  H Frauenfelder; S G Sligar; P G Wolynes
Journal:  Science       Date:  1991-12-13       Impact factor: 47.728

3.  Dynamics and the free-energy landscape of proteins, explored with the Mössbauer effect and quasi-elastic neutron scattering.

Authors:  Hans Frauenfelder; Robert D Young; Paul W Fenimore
Journal:  J Phys Chem B       Date:  2013-09-12       Impact factor: 2.991

4.  The temperature dependence of internal molecular motions in hydrated and dry alpha-amylase: the role of hydration water in the dynamical transition of proteins.

Authors:  J Fitter
Journal:  Biophys J       Date:  1999-02       Impact factor: 4.033

5.  The role of momentum transfer during incoherent neutron scattering is explained by the energy landscape model.

Authors:  Hans Frauenfelder; Robert D Young; Paul W Fenimore
Journal:  Proc Natl Acad Sci U S A       Date:  2017-05-01       Impact factor: 11.205

6.  A wave-mechanical model of incoherent quasielastic scattering in complex systems.

Authors:  Hans Frauenfelder; Paul W Fenimore; Robert D Young
Journal:  Proc Natl Acad Sci U S A       Date:  2014-08-18       Impact factor: 11.205

7.  Asymptotic neutron scattering laws for anomalously diffusing quantum particles.

Authors:  Gerald R Kneller
Journal:  J Chem Phys       Date:  2016-07-28       Impact factor: 3.488

8.  Reply to Wuttke: Our reinterpretation of QENS does not violate scattering theory.

Authors:  Hans Frauenfelder; Robert D Young; Paul W Fenimore
Journal:  Proc Natl Acad Sci U S A       Date:  2017-09-20       Impact factor: 11.205

9.  No case against scattering theory.

Authors:  Joachim Wuttke
Journal:  Proc Natl Acad Sci U S A       Date:  2017-09-20       Impact factor: 11.205
  9 in total
  2 in total

1.  Time domain versus energy domain neutron scattering analysis of protein dynamics.

Authors:  Wolfgang Doster
Journal:  Proc Natl Acad Sci U S A       Date:  2019-04-12       Impact factor: 11.205

2.  Reply to Doster: Franck-Condon and Van Hove formulation of quasielastic neutron scattering from complex systems.

Authors:  Gerald R Kneller
Journal:  Proc Natl Acad Sci U S A       Date:  2019-04-12       Impact factor: 11.205
  2 in total

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