Literature DB >> 29219532

Does a Growing Static Length Scale Control the Glass Transition?

Matthieu Wyart1, Michael E Cates2.   

Abstract

Several theories of the glass transition propose that the structural relaxation time τ_{α} is controlled by a growing static length scale ξ that is determined by the free energy landscape but not by the local dynamic rules governing its exploration. We argue, based on recent simulations using particle-radius-swap dynamics, that only a modest factor in the increase in τ_{α} on approach to the glass transition may stem from the growth of a static length, with a vastly larger contribution attributable, instead, to a slowdown of local dynamics. This reinforces arguments that we base on the observed strong coupling of particle diffusion and density fluctuations in real glasses.

Year:  2017        PMID: 29219532     DOI: 10.1103/PhysRevLett.119.195501

Source DB:  PubMed          Journal:  Phys Rev Lett        ISSN: 0031-9007            Impact factor:   9.161


  4 in total

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Journal:  Proc Natl Acad Sci U S A       Date:  2020-02-24       Impact factor: 11.205

Review 2.  Fast Vibrational Modes and Slow Heterogeneous Dynamics in Polymers and Viscous Liquids.

Authors:  Francesco Puosi; Antonio Tripodo; Dino Leporini
Journal:  Int J Mol Sci       Date:  2019-11-14       Impact factor: 5.923

3.  Effective one-component model of binary mixture: molecular arrest induced by the spatially correlated stochastic dynamics.

Authors:  M Majka; P F Góra
Journal:  Sci Rep       Date:  2019-12-23       Impact factor: 4.379

4.  Revisiting the concept of activation in supercooled liquids.

Authors:  Marco Baity-Jesi; Giulio Biroli; David R Reichman
Journal:  Eur Phys J E Soft Matter       Date:  2021-06-14       Impact factor: 1.890

  4 in total

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