Literature DB >> 28499080

Efficient Electrocatalytic Reduction of CO2 by Nitrogen-Doped Nanoporous Carbon/Carbon Nanotube Membranes: A Step Towards the Electrochemical CO2 Refinery.

Hong Wang1, Jia Jia1, Pengfei Song2, Qiang Wang3, Debao Li3, Shixiong Min4, Chenxi Qian1, Lu Wang1, Young Feng Li1, Chun Ma5, Tom Wu5, Jiayin Yuan6,7, Markus Antonietti6, Geoffrey A Ozin1.   

Abstract

Herein we introduce a straightforward, low cost, scalable, and technologically relevant method to manufacture an all-carbon, electroactive, nitrogen-doped nanoporous-carbon/carbon-nanotube composite membrane, dubbed "HNCM/CNT". The membrane is demonstrated to function as a binder-free, high-performance gas diffusion electrode for the electrocatalytic reduction of CO2 to formate. The Faradaic efficiency (FE) for the production of formate is 81 %. Furthermore, the robust structural and electrochemical properties of the membrane endow it with excellent long-term stability.
© 2017 Wiley-VCH Verlag GmbH & Co. KGaA, Weinheim.

Entities:  

Keywords:  CO2 reduction; carbon nanotubes; hierarchical carbon; membranes; nitrogen doping

Year:  2017        PMID： 28499080     DOI： 10.1002/anie.201703720

Source DB:  PubMed          Journal:  Angew Chem Int Ed Engl        ISSN： 1433-7851            Impact factor:   15.336


  8 in total

Review 1.  Porous Polyelectrolytes: The Interplay of Charge and Pores for New Functionalities.

Authors:  Weiyi Zhang; Qiang Zhao; Jiayin Yuan
Journal:  Angew Chem Int Ed Engl       Date:  2018-04-26       Impact factor: 15.336

2.  Structural defects on converted bismuth oxide nanotubes enable highly active electrocatalysis of carbon dioxide reduction.

Authors:  Qiufang Gong; Pan Ding; Mingquan Xu; Xiaorong Zhu; Maoyu Wang; Jun Deng; Qing Ma; Na Han; Yong Zhu; Jun Lu; Zhenxing Feng; Yafei Li; Wu Zhou; Yanguang Li
Journal:  Nat Commun       Date:  2019-06-26       Impact factor: 14.919

3.  Electronic synergism of pyridinic- and graphitic-nitrogen on N-doped carbons for the oxygen reduction reaction.

Authors:  Xiaomei Ning; Yuhang Li; Jingyan Ming; Qiang Wang; Hongjuan Wang; Yonghai Cao; Feng Peng; Yanhui Yang; Hao Yu
Journal:  Chem Sci       Date:  2018-12-13       Impact factor: 9.825

4.  Morphological Attributes Govern Carbon Dioxide Reduction on N-Doped Carbon Electrodes.

Authors:  Dorottya Hursán; Angelika A Samu; László Janovák; Kateryna Artyushkova; Tristan Asset; Plamen Atanassov; Csaba Janáky
Journal:  Joule       Date:  2019-07-17

5.  Heterostructure Engineering of a Reverse Water Gas Shift Photocatalyst.

Authors:  Hong Wang; Jia Jia; Lu Wang; Keith Butler; Rui Song; Gilberto Casillas; Le He; Nazir P Kherani; Doug D Perovic; Liqiang Jing; Aron Walsh; Roland Dittmeyer; Geoffrey A Ozin
Journal:  Adv Sci (Weinh)       Date:  2019-10-04       Impact factor: 16.806

6.  Online Monitoring of Electrochemical Carbon Corrosion in Alkaline Electrolytes by Differential Electrochemical Mass Spectrometry.

Authors:  Sandra Möller; Stefan Barwe; Justus Masa; Daniela Wintrich; Sabine Seisel; Helmut Baltruschat; Wolfgang Schuhmann
Journal:  Angew Chem Int Ed Engl       Date:  2019-12-04       Impact factor: 15.336

Review 7.  Heteroatom-Doped Metal-Free Carbon Nanomaterials as Potential Electrocatalysts.

Authors:  Jayeeta Chattopadhyay; Tara Sankar Pathak; Daewon Pak
Journal:  Molecules       Date:  2022-01-20       Impact factor: 4.411

8.  Cu x Ni y alloy nanoparticles embedded in a nitrogen-carbon network for efficient conversion of carbon dioxide.

Authors:  Dongxing Tan; Jianling Zhang; Xiuyan Cheng; Xiuniang Tan; Jinbiao Shi; Bingxing Zhang; Buxing Han; Lirong Zheng; Jing Zhang
Journal:  Chem Sci       Date:  2019-03-15       Impact factor: 9.825
  8 in total

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