| Literature DB >> 28145598 |
Dawei Di1, Le Yang1, Johannes M Richter1, Lorenzo Meraldi1, Rashid M Altamimi2, Ahmed Y Alyamani2, Dan Credgington1, Kevin P Musselman3, Judith L MacManus-Driscoll4, Richard H Friend1.
Abstract
Solution-processed polymer organic light-emitting diodes (OLEDs) doped with triplet-triplet annihilation (TTA)-upconversion molecules, including 9,10-diphenylanthracene, perylene, rubrene and TIPS-pentacene, are reported. The fraction of triplet-generated electroluminescence approaches the theoretical limit. Record-high efficiencies in solution-processed OLEDs based on these materials are achieved. Unprecedented solid-state TTA-upconversion quantum yield of 23% (TTA-upconversion reaction efficiency of 70%) at electrical excitation well below one-sun equivalent is observed.Entities:
Keywords: molecularly doped polymer OLEDs; singlet exciton fission; solid-state TTA upconversion; solution-processing; triplet exciton fusion
Year: 2017 PMID: 28145598 DOI: 10.1002/adma.201605987
Source DB: PubMed Journal: Adv Mater ISSN: 0935-9648 Impact factor: 30.849