Literature DB >> 26382702

Creation of X-Ray Transparency of Matter by Stimulated Elastic Forward Scattering.

J Stöhr1, A Scherz2.   

Abstract

X-ray absorption by matter has long been described by the famous Beer-Lambert law. Here, we show how this fundamental law needs to be modified for high-intensity coherent x-ray pulses, now available at x-ray free electron lasers, due to the onset of stimulated elastic forward scattering. We present an analytical expression for the modified polarization-dependent Beer-Lambert law for the case of resonant core-to-valence electronic transitions and incident transform limited x-ray pulses. Upon transmission through a solid, the resonant absorption and dichroic contrasts are found to vanish with increasing x-ray intensity, with the stimulation threshold lowered by orders of magnitude through a resonant superradiantlike effect. Our results have broad implications for the study of matter with x-ray lasers.

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Year:  2015        PMID: 26382702     DOI: 10.1103/PhysRevLett.115.107402

Source DB:  PubMed          Journal:  Phys Rev Lett        ISSN: 0031-9007            Impact factor:   9.161


  6 in total

1.  In situ single-shot diffractive fluence mapping for X-ray free-electron laser pulses.

Authors:  Michael Schneider; Christian M Günther; Bastian Pfau; Flavio Capotondi; Michele Manfredda; Marco Zangrando; Nicola Mahne; Lorenzo Raimondi; Emanuele Pedersoli; Denys Naumenko; Stefan Eisebitt
Journal:  Nat Commun       Date:  2018-01-15       Impact factor: 14.919

2.  Soft x-ray absorption spectroscopy of metalloproteins and high-valent metal-complexes at room temperature using free-electron lasers.

Authors:  Markus Kubin; Jan Kern; Sheraz Gul; Thomas Kroll; Ruchira Chatterjee; Heike Löchel; Franklin D Fuller; Raymond G Sierra; Wilson Quevedo; Christian Weniger; Jens Rehanek; Anatoly Firsov; Hartawan Laksmono; Clemens Weninger; Roberto Alonso-Mori; Dennis L Nordlund; Benedikt Lassalle-Kaiser; James M Glownia; Jacek Krzywinski; Stefan Moeller; Joshua J Turner; Michael P Minitti; Georgi L Dakovski; Sergey Koroidov; Anurag Kawde; Jacob S Kanady; Emily Y Tsui; Sandy Suseno; Zhiji Han; Ethan Hill; Taketo Taguchi; Andrew S Borovik; Theodor Agapie; Johannes Messinger; Alexei Erko; Alexander Föhlisch; Uwe Bergmann; Rolf Mitzner; Vittal K Yachandra; Junko Yano; Philippe Wernet
Journal:  Struct Dyn       Date:  2017-09-01       Impact factor: 2.920

Review 3.  Recent Development in X-Ray Imaging Technology: Future and Challenges.

Authors:  Xiangyu Ou; Xue Chen; Xianning Xu; Lili Xie; Xiaofeng Chen; Zhongzhu Hong; Hua Bai; Xiaowang Liu; Qiushui Chen; Lin Li; Huanghao Yang
Journal:  Research (Wash D C)       Date:  2021-12-26

4.  Resonantly Enhanced Difference-Frequency Generation in the Core X-ray Absorption of Molecules.

Authors:  Carles Serrat
Journal:  J Phys Chem A       Date:  2021-12-15       Impact factor: 2.781

5.  Saturable Absorption of Free-Electron Laser Radiation by Graphite near the Carbon K-Edge.

Authors:  Lars Hoffmann; Sasawat Jamnuch; Craig P Schwartz; Tobias Helk; Sumana L Raj; Hikaru Mizuno; Riccardo Mincigrucci; Laura Foglia; Emiliano Principi; Richard J Saykally; Walter S Drisdell; Shervin Fatehi; Tod A Pascal; Michael Zuerch
Journal:  J Phys Chem Lett       Date:  2022-09-27       Impact factor: 6.888

6.  Femtosecond X-ray induced changes of the electronic and magnetic response of solids from electron redistribution.

Authors:  Daniel J Higley; Alex H Reid; Zhao Chen; Loïc Le Guyader; Olav Hellwig; Alberto A Lutman; Tianmin Liu; Padraic Shafer; Tyler Chase; Georgi L Dakovski; Ankush Mitra; Edwin Yuan; Justine Schlappa; Hermann A Dürr; William F Schlotter; Joachim Stöhr
Journal:  Nat Commun       Date:  2019-11-21       Impact factor: 14.919

  6 in total

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