Literature DB >> 23679412

Decorrelation of the static and dynamic length scales in hard-sphere glass formers.

Patrick Charbonneau1, Gilles Tarjus.   

Abstract

We show that, in the equilibrium phase of glass-forming hard-sphere fluids in three dimensions, the static length scales tentatively associated with the dynamical slowdown and the dynamical length characterizing spatial heterogeneities in the dynamics unambiguously decorrelate. The former grow at a much slower rate than the latter when density increases. This observation is valid for the dynamical range that is accessible to computer simulations, which roughly corresponds to that accessible in colloidal experiments. We also find that, in this same range, no one-to-one correspondence between relaxation time and point-to-set correlation length exists. These results point to the coexistence of several relaxation mechanisms in the dynamically accessible regime of three-dimensional hard-sphere glass formers.

Year:  2013        PMID: 23679412     DOI: 10.1103/PhysRevE.87.042305

Source DB:  PubMed          Journal:  Phys Rev E Stat Nonlin Soft Matter Phys        ISSN: 1539-3755


  6 in total

1.  Dynamical facilitation governs glassy dynamics in suspensions of colloidal ellipsoids.

Authors:  Chandan K Mishra; K Hima Nagamanasa; Rajesh Ganapathy; A K Sood; Shreyas Gokhale
Journal:  Proc Natl Acad Sci U S A       Date:  2014-10-13       Impact factor: 11.205

2.  Assessing the role of static length scales behind glassy dynamics in polydisperse hard disks.

Authors:  John Russo; Hajime Tanaka
Journal:  Proc Natl Acad Sci U S A       Date:  2015-05-18       Impact factor: 11.205

3.  Configurational entropy measurements in extremely supercooled liquids that break the glass ceiling.

Authors:  Ludovic Berthier; Patrick Charbonneau; Daniele Coslovich; Andrea Ninarello; Misaki Ozawa; Sho Yaida
Journal:  Proc Natl Acad Sci U S A       Date:  2017-10-10       Impact factor: 11.205

4.  Mutual information reveals multiple structural relaxation mechanisms in a model glass former.

Authors:  Andrew J Dunleavy; Karoline Wiesner; Ryoichi Yamamoto; C Patrick Royall
Journal:  Nat Commun       Date:  2015-01-22       Impact factor: 14.919

5.  Neural Networks Reveal the Impact of the Vibrational Dynamics in the Prediction of the Long-Time Mobility of Molecular Glassformers.

Authors:  Antonio Tripodo; Gianfranco Cordella; Francesco Puosi; Marco Malvaldi; Dino Leporini
Journal:  Int J Mol Sci       Date:  2022-08-18       Impact factor: 6.208

6.  The role of local-geometrical-orders on the growth of dynamic-length-scales in glass-forming liquids.

Authors:  Kaikin Wong; Rithin P Krishnan; Changjiu Chen; Qing Du; Dehong Yu; Zhaoping Lu; K Samwer; Suresh M Chathoth
Journal:  Sci Rep       Date:  2018-01-31       Impact factor: 4.379

  6 in total

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