| Literature DB >> 25375708 |
Simon Schreck1, Martin Beye2, Jonas A Sellberg3, Trevor McQueen4, Hartawan Laksmono5, Brian Kennedy2, Sebastian Eckert2, Daniel Schlesinger6, Dennis Nordlund7, Hirohito Ogasawara7, Raymond G Sierra5, Vegard H Segtnan8, Katharina Kubicek9, William F Schlotter10, Georgi L Dakovski10, Stefan P Moeller10, Uwe Bergmann10, Simone Techert11, Lars G M Pettersson6, Philippe Wernet2, Michael J Bogan5, Yoshihisa Harada12, Anders Nilsson13, Alexander Föhlisch1.
Abstract
We report on oxygen K-edge soft x-ray emission spectroscopy from a liquid water jet at the Linac Coherent Light Source. We observe significant changes in the spectral content when tuning over a wide range of incident x-ray fluences. In addition the total emission yield decreases at high fluences. These modifications result from reabsorption of x-ray emission by valence-excited molecules generated by the Auger cascade. Our observations have major implications for future x-ray emission studies at intense x-ray sources. We highlight the importance of the x-ray pulse length with respect to the core-hole lifetime.Entities:
Mesh:
Year: 2014 PMID: 25375708 DOI: 10.1103/PhysRevLett.113.153002
Source DB: PubMed Journal: Phys Rev Lett ISSN: 0031-9007 Impact factor: 9.161