Literature DB >> 25328006

Room temperature quantum coherence in a potential molecular qubit.

Katharina Bader1, Dominik Dengler1, Samuel Lenz1, Burkhard Endeward2, Shang-Da Jiang3, Petr Neugebauer1, Joris van Slageren1.   

Abstract

The successful development of a quantum computer would change the world, and current internet encryption methods would cease to function. However, no working quantum computer that even begins to rival conventional computers has been developed yet, which is due to the lack of suitable quantum bits. A key characteristic of a quantum bit is the coherence time. Transition metal complexes are very promising quantum bits, owing to their facile surface deposition and their chemical tunability. However, reported quantum coherence times have been unimpressive. Here we report very long quantum coherence times for a transition metal complex of 68 μs at low temperature (qubit figure of merit QM=3,400) and 1 μs at room temperature, much higher than previously reported values for such systems. We show that this achievement is because of the rigidity of the lattice as well as removal of nuclear spins from the vicinity of the magnetic ion.

Entities:  

Year:  2014        PMID: 25328006     DOI: 10.1038/ncomms6304

Source DB:  PubMed          Journal:  Nat Commun        ISSN: 2041-1723            Impact factor:   14.919


  29 in total

1.  Enhancing coherence in molecular spin qubits via atomic clock transitions.

Authors:  Muhandis Shiddiq; Dorsa Komijani; Yan Duan; Alejandro Gaita-Ariño; Eugenio Coronado; Stephen Hill
Journal:  Nature       Date:  2016-03-17       Impact factor: 49.962

2.  Chemical control of spin-lattice relaxation to discover a room temperature molecular qubit.

Authors:  M Jeremy Amdur; Kathleen R Mullin; Michael J Waters; Danilo Puggioni; Michael K Wojnar; Mingqiang Gu; Lei Sun; Paul H Oyala; James M Rondinelli; Danna E Freedman
Journal:  Chem Sci       Date:  2022-05-17       Impact factor: 9.969

Review 3.  Molecular spins for quantum computation.

Authors:  A Gaita-Ariño; F Luis; S Hill; E Coronado
Journal:  Nat Chem       Date:  2019-04       Impact factor: 24.427

4.  Decoding the Ambiguous Electron Paramagnetic Resonance Signals in the Lytic Polysaccharide Monooxygenase from Photorhabdus luminescens.

Authors:  Rogelio J Gómez-Piñeiro; Maria Drosou; Sylvain Bertaina; Christophe Decroos; A Jalila Simaan; Dimitrios A Pantazis; Maylis Orio
Journal:  Inorg Chem       Date:  2022-05-12       Impact factor: 5.436

5.  Electron spin coherence near room temperature in magnetic quantum dots.

Authors:  Fabrizio Moro; Lyudmila Turyanska; James Wilman; Alistair J Fielding; Michael W Fay; Josef Granwehr; Amalia Patanè
Journal:  Sci Rep       Date:  2015-06-04       Impact factor: 4.379

6.  Millisecond Coherence Time in a Tunable Molecular Electronic Spin Qubit.

Authors:  Joseph M Zadrozny; Jens Niklas; Oleg G Poluektov; Danna E Freedman
Journal:  ACS Cent Sci       Date:  2015-12-02       Impact factor: 14.553

7.  A modular design of molecular qubits to implement universal quantum gates.

Authors:  Jesús Ferrando-Soria; Eufemio Moreno Pineda; Alessandro Chiesa; Antonio Fernandez; Samantha A Magee; Stefano Carretta; Paolo Santini; Iñigo J Vitorica-Yrezabal; Floriana Tuna; Grigore A Timco; Eric J L McInnes; Richard E P Winpenny
Journal:  Nat Commun       Date:  2016-04-25       Impact factor: 14.919

Review 8.  A Molecular Approach to Quantum Sensing.

Authors:  Chung-Jui Yu; Stephen von Kugelgen; Daniel W Laorenza; Danna E Freedman
Journal:  ACS Cent Sci       Date:  2021-04-20       Impact factor: 14.553

9.  Targeting molecular quantum memory with embedded error correction.

Authors:  Selena J Lockyer; Alessandro Chiesa; Grigore A Timco; Eric J L McInnes; Tom S Bennett; Inigo J Vitorica-Yrezebal; Stefano Carretta; Richard E P Winpenny
Journal:  Chem Sci       Date:  2021-06-02       Impact factor: 9.825

10.  Making hybrid [n]-rotaxanes as supramolecular arrays of molecular electron spin qubits.

Authors:  Antonio Fernandez; Jesus Ferrando-Soria; Eufemio Moreno Pineda; Floriana Tuna; Iñigo J Vitorica-Yrezabal; Christiane Knappke; Jakub Ujma; Christopher A Muryn; Grigore A Timco; Perdita E Barran; Arzhang Ardavan; Richard E P Winpenny
Journal:  Nat Commun       Date:  2016-01-08       Impact factor: 14.919

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