Literature DB >> 22887645

Redox self-sufficient biocatalyst network for the amination of primary alcohols.

Johann H Sattler1, Michael Fuchs, Katharina Tauber, Francesco G Mutti, Kurt Faber, Jan Pfeffer, Thomas Haas, Wolfgang Kroutil.   

Abstract

Driving the machinery: A biocatalytic redox-neutral cascade for the preparation of terminal primary amines from primary alcohols at the expense of ammonia has been established in a one-pot one-step method. Applying this artificial biocatalyst network, long-chain 1,ω-alkanediols were converted into diamines, which are building blocks for polymers, in up to 99 % conversion.
Copyright © 2012 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.

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Year:  2012        PMID： 22887645     DOI： 10.1002/anie.201204683

Source DB:  PubMed          Journal:  Angew Chem Int Ed Engl        ISSN： 1433-7851            Impact factor:   15.336


  23 in total

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3.  In vitro biocatalytic pathway design: orthogonal network for the quantitative and stereospecific amination of alcohols.

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Review 4.  Borrowing Hydrogen for Organic Synthesis.

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5.  Asymmetric Preparation of prim-, sec-, and tert-Amines Employing Selected Biocatalysts.

Authors:  Wolfgang Kroutil; Eva-Maria Fischereder; Christine S Fuchs; Horst Lechner; Francesco G Mutti; Desiree Pressnitz; Aashrita Rajagopalan; Johann H Sattler; Robert C Simon; Elina Siirola
Journal:  Org Process Res Dev       Date:  2013-04-22       Impact factor: 3.317

6.  Cofactor Specificity Engineering of Streptococcus mutans NADH Oxidase 2 for NAD(P)(+) Regeneration in Biocatalytic Oxidations.

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7.  Biocatalytic hydrogen-borrowing cascades.

Authors:  Tanja Knaus; Francesco G Mutti
Journal:  Chim Oggi       Date:  2017 Sep/Oct

8.  Conversion of alcohols to enantiopure amines through dual-enzyme hydrogen-borrowing cascades.

Authors:  Francesco G Mutti; Tanja Knaus; Nigel S Scrutton; Michael Breuer; Nicholas J Turner
Journal:  Science       Date:  2015-09-25       Impact factor: 47.728

9.  Biocatalytic access to betazole using a one-pot multienzymatic system in continuous flow.

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Review 10.  Synthetic biology for the directed evolution of protein biocatalysts: navigating sequence space intelligently.

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Journal:  Chem Soc Rev       Date:  2015-03-07       Impact factor: 54.564
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