Literature DB >> 21045823

A microscopic view on the Mott transition in chromium-doped V(2)O(3).

S Lupi1, L Baldassarre, B Mansart, A Perucchi, A Barinov, P Dudin, E Papalazarou, F Rodolakis, J-P Rueff, J-P Itié, S Ravy, D Nicoletti, P Postorino, P Hansmann, N Parragh, A Toschi, T Saha-Dasgupta, O K Andersen, G Sangiovanni, K Held, M Marsi.   

Abstract

V(2)O(3) is the prototype system for the Mott transition, one of the most fundamental phenomena of electronic correlation. Temperature, doping or pressure induce a metal-to-insulator transition (MIT) between a paramagnetic metal (PM) and a paramagnetic insulator. This or related MITs have a high technological potential, among others, for intelligent windows and field effect transistors. However the spatial scale on which such transitions develop is not known in spite of their importance for research and applications. Here we unveil for the first time the MIT in Cr-doped V(2)O(3) with submicron lateral resolution: with decreasing temperature, microscopic domains become metallic and coexist with an insulating background. This explains why the associated PM phase is actually a poor metal. The phase separation can be associated with a thermodynamic instability near the transition. This instability is reduced by pressure, that promotes a genuine Mott transition to an eventually homogeneous metallic state.

Entities:  

Year:  2010        PMID: 21045823     DOI: 10.1038/ncomms1109

Source DB:  PubMed          Journal:  Nat Commun        ISSN: 2041-1723            Impact factor:   14.919


  13 in total

1.  Cerium volume collapse: results from the merger of dynamical mean-field theory and local density approximation.

Authors:  K Held; A K McMahan; R T Scalettar
Journal:  Phys Rev Lett       Date:  2001-12-13       Impact factor: 9.161

2.  Prominent quasiparticle peak in the photoemission spectrum of the metallic phase of V2O3.

Authors:  S-K Mo; J D Denlinger; H-D Kim; J-H Park; J W Allen; A Sekiyama; A Yamasaki; K Kadono; S Suga; Y Saitoh; T Muro; P Metcalf; G Keller; K Held; V Eyert; V I Anisimov; D Vollhardt
Journal:  Phys Rev Lett       Date:  2003-05-08       Impact factor: 9.161

3.  Lattice contraction driven insulator-metal transition in the d=

Authors: 
Journal:  Phys Rev Lett       Date:  1994-09-12       Impact factor: 9.161

4.  Inequivalent routes across the Mott transition in V2O3 explored by X-ray absorption.

Authors:  F Rodolakis; P Hansmann; J-P Rueff; A Toschi; M W Haverkort; G Sangiovanni; A Tanaka; T Saha-Dasgupta; O K Andersen; K Held; M Sikora; I Alliot; J-P Itié; F Baudelet; P Wzietek; P Metcalf; M Marsi
Journal:  Phys Rev Lett       Date:  2010-01-25       Impact factor: 9.161

5.  Strain-induced bond buckling and its role in insulating properties of Cr-doped V2O3.

Authors:  A I Frenkel; D M Pease; J I Budnick; P Metcalf; E A Stern; P Shanthakumar; T Huang
Journal:  Phys Rev Lett       Date:  2006-11-09       Impact factor: 9.161

6.  Quasiparticles at the Mott transition in V2O3: wave vector dependence and surface attenuation.

Authors:  F Rodolakis; B Mansart; E Papalazarou; S Gorovikov; P Vilmercati; L Petaccia; A Goldoni; J P Rueff; S Lupi; P Metcalf; M Marsi
Journal:  Phys Rev Lett       Date:  2009-02-11       Impact factor: 9.161

7.  Surface dead layer for quasiparticles near a mott transition.

Authors:  Giovanni Borghi; Michele Fabrizio; Erio Tosatti
Journal:  Phys Rev Lett       Date:  2009-02-11       Impact factor: 9.161

8.  Multi-orbital effects in optical properties of vanadium sesquioxide.

Authors:  Jan M Tomczak; Silke Biermann
Journal:  J Phys Condens Matter       Date:  2009-01-20       Impact factor: 2.333

9.  Mott-hubbard metal-insulator transition in paramagnetic V2O3: an LDA+DMFT(QMC) study.

Authors:  K Held; G Keller; V Eyert; D Vollhardt; V I Anisimov
Journal:  Phys Rev Lett       Date:  2001-06-04       Impact factor: 9.161

10.  Universality and critical behavior at the Mott transition.

Authors:  P Limelette; A Georges; D Jérome; P Wzietek; P Metcalf; J M Honig
Journal:  Science       Date:  2003-10-03       Impact factor: 47.728

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  9 in total

1.  Charge-ordering transition in iron oxide Fe4O5 involving competing dimer and trimer formation.

Authors:  Sergey V Ovsyannikov; Maxim Bykov; Elena Bykova; Denis P Kozlenko; Alexander A Tsirlin; Alexander E Karkin; Vladimir V Shchennikov; Sergey E Kichanov; Huiyang Gou; Artem M Abakumov; Ricardo Egoavil; Johan Verbeeck; Catherine McCammon; Vadim Dyadkin; Dmitry Chernyshov; Sander van Smaalen; Leonid S Dubrovinsky
Journal:  Nat Chem       Date:  2016-04-04       Impact factor: 24.427

2.  Nanoscale self-organization and metastable non-thermal metallicity in Mott insulators.

Authors:  Andrea Ronchi; Paolo Franceschini; Andrea De Poli; Pía Homm; Ann Fitzpatrick; Francesco Maccherozzi; Gabriele Ferrini; Francesco Banfi; Sarnjeet S Dhesi; Mariela Menghini; Michele Fabrizio; Jean-Pierre Locquet; Claudio Giannetti
Journal:  Nat Commun       Date:  2022-06-28       Impact factor: 17.694

3.  The strength of electron electron correlation in Cs3C60.

Authors:  L Baldassarre; A Perucchi; M Mitrano; D Nicoletti; C Marini; D Pontiroli; M Mazzani; M Aramini; M Riccó; G Giovannetti; M Capone; S Lupi
Journal:  Sci Rep       Date:  2015-10-15       Impact factor: 4.379

4.  Memristive and neuromorphic behavior in a Li(x)CoO2 nanobattery.

Authors:  V H Mai; A Moradpour; P Auban Senzier; C Pasquier; K Wang; M J Rozenberg; J Giapintzakis; C N Mihailescu; C M Orfanidou; E Svoukis; A Breza; Ch B Lioutas; S Franger; A Revcolevschi; T Maroutian; P Lecoeur; P Aubert; G Agnus; R Salot; P A Albouy; R Weil; D Alamarguy; K March; F Jomard; P Chrétien; O Schneegans
Journal:  Sci Rep       Date:  2015-01-14       Impact factor: 4.379

5.  Soft X-ray angle-resolved photoemission with micro-positioning techniques for metallic V₂O₃.

Authors:  Hidenori Fujiwara; Takayuki Kiss; Yuki K Wakabayashi; Yoshito Nishitani; Takeo Mori; Yuki Nakata; Satoshi Kitayama; Kazuaki Fukushima; Shinji Ikeda; Hiroto Fuchimoto; Yosuke Minowa; Sung-Kwan Mo; Jonathan D Denlinger; James W Allen; Patricia Metcalf; Masaki Imai; Kazuyoshi Yoshimura; Shigemasa Suga; Takayuki Muro; Akira Sekiyama
Journal:  J Synchrotron Radiat       Date:  2015-04-14       Impact factor: 2.616

6.  Volume-wise destruction of the antiferromagnetic Mott insulating state through quantum tuning.

Authors:  Benjamin A Frandsen; Lian Liu; Sky C Cheung; Zurab Guguchia; Rustem Khasanov; Elvezio Morenzoni; Timothy J S Munsie; Alannah M Hallas; Murray N Wilson; Yipeng Cai; Graeme M Luke; Bijuan Chen; Wenmin Li; Changqing Jin; Cui Ding; Shengli Guo; Fanlong Ning; Takashi U Ito; Wataru Higemoto; Simon J L Billinge; Shoya Sakamoto; Atsushi Fujimori; Taito Murakami; Hiroshi Kageyama; Jose Antonio Alonso; Gabriel Kotliar; Masatoshi Imada; Yasutomo J Uemura
Journal:  Nat Commun       Date:  2016-08-17       Impact factor: 14.919

7.  Ultrafast evolution and transient phases of a prototype out-of-equilibrium Mott-Hubbard material.

Authors:  G Lantz; B Mansart; D Grieger; D Boschetto; N Nilforoushan; E Papalazarou; N Moisan; L Perfetti; V L R Jacques; D Le Bolloc'h; C Laulhé; S Ravy; J-P Rueff; T E Glover; M P Hertlein; Z Hussain; S Song; M Chollet; M Fabrizio; M Marsi
Journal:  Nat Commun       Date:  2017-01-09       Impact factor: 14.919

8.  Imaging the itinerant-to-localized transmutation of electrons across the metal-to-insulator transition in V2O3.

Authors:  Maximilian Thees; Min-Han Lee; Rosa Luca Bouwmeester; Pedro H Rezende-Gonçalves; Emma David; Alexandre Zimmers; Franck Fortuna; Emmanouil Frantzeskakis; Nicolas M Vargas; Yoav Kalcheim; Patrick Le Fèvre; Koji Horiba; Hiroshi Kumigashira; Silke Biermann; Juan Trastoy; Marcelo J Rozenberg; Ivan K Schuller; Andrés F Santander-Syro
Journal:  Sci Adv       Date:  2021-11-03       Impact factor: 14.136

9.  Infrared evidence of a Slater metal-insulator transition in NaOsO₃.

Authors:  I Lo Vecchio; A Perucchi; P Di Pietro; O Limaj; U Schade; Y Sun; M Arai; K Yamaura; S Lupi
Journal:  Sci Rep       Date:  2013-10-21       Impact factor: 4.379

  9 in total

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