Literature DB >> 20373762

Tuning MOF CO2 adsorption properties via cation exchange.

Jihyun An1, Nathaniel L Rosi.   

Abstract

The pore volume and BET surface area of bio-MOF-1 (a), Zn(8)(ad)(4)(BPDC)(6)O.2Me(2)NH(2), is systematically modified via postsynthetic cation exchange with either tetramethylammonium, tetraethylammonium, or tetrabutylammonium cations to yield Zn(8)(ad)(4)(BPDC)(6)O.2Me(4)N (b), Zn(8)(ad)(4)(BPDC)(6)O.2Et(4)N (c), and Zn(8)(ad)(4)(BPDC)(6)O.2Bu(4)N (d), respectively. The impact that pore volume and BET surface area have on CO(2) capacity is evaluated, and it is found that materials with intermediate porosity (b and c) have the largest CO(2) capacities under the conditions studied.

Entities:  

Year:  2010        PMID： 20373762     DOI： 10.1021/ja1012992

Source DB:  PubMed          Journal:  J Am Chem Soc        ISSN： 0002-7863            Impact factor:   15.419


  14 in total

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Journal:  Sci Rep       Date:  2013       Impact factor: 4.379

10.  Lewis basicity generated by localised charge imbalance in noble metal nanoparticle-embedded defective metal-organic frameworks.

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Journal:  Nat Commun       Date:  2018-10-18       Impact factor: 14.919
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