Literature DB >> 19997962

ATP chemosensitivity testing of new antitumor duplex drugs linking 3`-C-ethynylycytidine (ECyd) and 2´-deoxy-5-fluorouridine (5-FdU) in comparison to standard cytostatica and combinations thereof.

Sarah Schott1, Markus Wallwiener, Beate Kootz, Harald Seeger, Tanja Fehm, Hans Neubauer.   

Abstract

BACKGROUND: 2´-Deoxy-5-fluorouridylyl-(5´-5´)-3´-C-ethynylcytidine [5-FdU(5´-5´)ECyd] and 3´-C-ethynylcytidinylyl-(5´->1-O)-2-O-octadecyl-sn-glycerylyl-(3-Ο->5´)-2´-deoxy-5-fluorouridine [ECyd-lipid-5-FdU] are antitumor active duplex drugs and these heterodinucleoside phosphate analogues could be cleaved in vivo by wide-spread phosphodiesterases into different antitumor active antimetabolites.
METHODS: We cultured breast MCF-7, MDA-MB-231 and ovarian OVCAR-29 and OAW-42 cancer cell lines and used the luminometric measuring of the ATP tumor chemosensitivity assay to assess the in vitro activity of 5-FdU(5´-5´)ECyd and ECyd-lipid-5-FdU in comparison to standard single cytostatic agents and combinations thereof currently used in anticancer therapies. To allow comparison between samples and different regimens IndexSUM was determined based on the percentage tumor cell growth inhibition at each test drug concentration. Additionally, the cytostatic efficacy of 5-FdU(5´-5´)ECyd and ECyd-lipid-5-FdU was evaluated at a minimum of five concentrations at 10 fold dilutions using 60 human tumor cell lines including ovarian and breast cancer cell lines from the National Cancer Institute (USA).
RESULTS: 5-FdU(5´-5´)ECyd and ECyd-lipid-5-FdU have a high cytostatic efficacy reaching 50% tumor cell growth inhibition at concentrations ranging between nano- and micomolar. IndexSum values for broad range efficacy in MCF-7 breast cancer cells were comparable to values obtained for standard drug combinations. Higher cytostatic efficacy was observed in MDA-MB-231 cells.
CONCLUSION: The duplex drugs 5-FdU(5´-5´)ECyd and ECyd-lipid-5-FdU represent potential new chemotherapeutic drugs for breast and ovarian cancer cells which are comparable to currently used drug combinations and more potent in comparison to some monocytostatica used in cancer therapy.

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Year:  2009        PMID: 19997962     DOI: 10.1007/s10637-009-9355-0

Source DB:  PubMed          Journal:  Invest New Drugs        ISSN: 0167-6997            Impact factor:   3.850


  29 in total

1.  A crucial role of uridine/cytidine kinase 2 in antitumor activity of 3'-ethynyl nucleosides.

Authors:  Daigo Murata; Yoshio Endo; Tohru Obata; Kazuki Sakamoto; Yasuhiro Syouji; Masakazu Kadohira; Akira Matsuda; Takuma Sasaki
Journal:  Drug Metab Dispos       Date:  2004-07-27       Impact factor: 3.922

2.  In vitro activity and mechanism of action of a duplex and multidrug of ethynylcytidine and 5-fluorodeoxyuridine.

Authors:  I V Bijnsdorp; R A Schwendener; H Schott; S Schott; I Fichtner; R J Honeywell; N Losekoot; A C Laan; G J Peters
Journal:  Nucleic Acids Symp Ser (Oxf)       Date:  2008

3.  Cytotoxicity, cell-cycle perturbations and apoptosis in human tumor cells by lipophilic N4-alkyl-1-beta-D-arabinofuranosylcytosine derivatives and the new heteronucleoside phosphate dimer arabinocytidylyl-(5'-->5')-N4-octadecyl-1-beta-D-arabinofuranosylcytosi ne.

Authors:  D H Horber; R M Cattaneo-Pangrazzi; P von Ballmoos; H Schott; P S Ludwig; S Eriksson; I Fichtner; R A Schwendener
Journal:  J Cancer Res Clin Oncol       Date:  2000-06       Impact factor: 4.553

4.  The ex vivo characterization of XR5944 (MLN944) against a panel of human clinical tumor samples.

Authors:  Federica Di Nicolantonio; Louise A Knight; Pauline A Whitehouse; Stuart J Mercer; Sanjay Sharma; Peter A Charlton; David Norris; Ian A Cree
Journal:  Mol Cancer Ther       Date:  2004-12       Impact factor: 6.261

5.  The novel heterodinucleoside dimer 5-FdU-NOAC is a potent cytotoxic drug and a p53-independent inducer of apoptosis in the androgen-independent human prostate cancer cell lines PC-3 and DU-145.

Authors:  R M Cattaneo-Pangrazzi; H Schott; R A Schwendener
Journal:  Prostate       Date:  2000-09-15       Impact factor: 4.104

6.  A novel apoptotic pathway of 3'-Ethynylcytidine(ECyd) involving the inhibition of RNA synthesis--the possibility of RNase L activated pathway as a target of ECyd.

Authors:  Tomoharu Naito; Tatsushi Yokogawa; Hye-Sook Kim; Akira Matsuda; Takuma Sasaki; Masakazu Fukushima; Yukio Kitade; Yusuke Wataya
Journal:  Nucleic Acids Symp Ser (Oxf)       Date:  2007

7.  Bioluminescence of cellular ATP: a new method for evaluating cytotoxic agents in vitro.

Authors:  L Kangas; M Grönroos; A L Nieminen
Journal:  Med Biol       Date:  1984

8.  In vivo and in vitro activity and mechanism of action of the multidrug cytarabine-L-glycerylyl-fluorodeoxyuridine.

Authors:  Irene V Bijnsdorp; Reto A Schwendener; Herbert Schott; Iduna Fichtner; Kees Smid; Sarah Schott; Adrie C Laan; Godefridus J Peters
Journal:  Nucleosides Nucleotides Nucleic Acids       Date:  2007       Impact factor: 1.381

9.  Predicting resistance to platinum-containing chemotherapy with the ATP tumor chemosensitivity assay in primary ovarian cancer.

Authors:  Hans Neubauer; Maya Stefanova; Erich Solomayer; Christoph Meisner; Manfred Zwirner; Diethelm Wallwiener; Tanja Fehm
Journal:  Anticancer Res       Date:  2008 Mar-Apr       Impact factor: 2.480

10.  Chemosensitivity testing of human tumors using a microplate adenosine triphosphate luminescence assay: clinical correlation for cisplatin resistance of ovarian carcinoma.

Authors:  P E Andreotti; I A Cree; C M Kurbacher; D M Hartmann; D Linder; G Harel; I Gleiberman; P A Caruso; S H Ricks; M Untch
Journal:  Cancer Res       Date:  1995-11-15       Impact factor: 12.701

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  5 in total

1.  Cytotoxicity of the new antimetabolite-bisphosphonate (5-FdU-alendronate) in comparison to standard therapeutics on breast and ovarian cancer cell lines in the ATP tumor chemosensitivity assay.

Authors:  Sarah Schott; Markus Wallwiener; Beate Kootz; Harald Seeger; Tanja Fehm; Hans Neubauer
Journal:  Invest New Drugs       Date:  2011-05-21       Impact factor: 3.850

2.  Cytostatic activity of the duplex drug linking 2'-deoxy-5-fluorouridine (5FdU) with 3'-C-ethynylcytidine (ECyd) against gastric adenocarcinoma cell lines.

Authors:  Jürgen Weinreich; Sarah Schott; Ingmar Königsrainer; Derek Zieker; Alfred Königsrainer; Herbert Schott
Journal:  Invest New Drugs       Date:  2010-07-02       Impact factor: 3.850

3.  Effect of duplex drugs linking 2'-deoxy-5-fluorouridine (5-FdU) with 3'-C-ethynylcytidine (ECyd) on hepatoblastoma cell lines.

Authors:  Carmen Eicher; Alexander Dewerth; Verena Ellerkamp; Joerg Fuchs; Sarah Schott; Sorin Armeanu-Ebinger
Journal:  Pediatr Surg Int       Date:  2013-02       Impact factor: 1.827

4.  Synthesis of a 3'-C-ethynyl-β-d-ribofuranose purine nucleoside library: Discovery of C7-deazapurine analogs as potent antiproliferative nucleosides.

Authors:  Fabian Hulpia; Sam Noppen; Dominique Schols; Graciela Andrei; Robert Snoeck; Sandra Liekens; Peter Vervaeke; Serge Van Calenbergh
Journal:  Eur J Med Chem       Date:  2018-07-29       Impact factor: 6.514

5.  The conjugated antimetabolite 5-FdU-ECyd and its cellular and molecular effects on platinum-sensitive vs. -resistant ovarian cancer cells in vitro.

Authors:  Sarah Schott; Pauline Wimberger; Barbara Klink; Konrad Grützmann; Julian Puppe; Ulrike Sophie Wauer; Daniel Martin Klotz; Evelin Schröck; Jan Dominik Kuhlmann
Journal:  Oncotarget       Date:  2017-08-14
  5 in total

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