Literature DB >> 17272718

Ultrafast bond softening in bismuth: mapping a solid's interatomic potential with X-rays.

D M Fritz1, D A Reis, B Adams, R A Akre, J Arthur, C Blome, P H Bucksbaum, A L Cavalieri, S Engemann, S Fahy, R W Falcone, P H Fuoss, K J Gaffney, M J George, J Hajdu, M P Hertlein, P B Hillyard, M Horn-von Hoegen, M Kammler, J Kaspar, R Kienberger, P Krejcik, S H Lee, A M Lindenberg, B McFarland, D Meyer, T Montagne, E D Murray, A J Nelson, M Nicoul, R Pahl, J Rudati, H Schlarb, D P Siddons, K Sokolowski-Tinten, Th Tschentscher, D von der Linde, J B Hastings.   

Abstract

Intense femtosecond laser excitation can produce transient states of matter that would otherwise be inaccessible to laboratory investigation. At high excitation densities, the interatomic forces that bind solids and determine many of their properties can be substantially altered. Here, we present the detailed mapping of the carrier density-dependent interatomic potential of bismuth approaching a solid-solid phase transition. Our experiments combine stroboscopic techniques that use a high-brightness linear electron accelerator-based x-ray source with pulse-by-pulse timing reconstruction for femtosecond resolution, allowing quantitative characterization of the interatomic potential energy surface of the highly excited solid.

Entities:  

Year:  2007        PMID: 17272718     DOI: 10.1126/science.1135009

Source DB:  PubMed          Journal:  Science        ISSN: 0036-8075            Impact factor:   47.728


  34 in total

1.  Ultrafast changes in lattice symmetry probed by coherent phonons.

Authors:  S Wall; D Wegkamp; L Foglia; K Appavoo; J Nag; R F Haglund; J Stähler; M Wolf
Journal:  Nat Commun       Date:  2012-03-06       Impact factor: 14.919

2.  Time-resolved structural dynamics of thin metal films heated with femtosecond optical pulses.

Authors:  Jie Chen; Wei-Kan Chen; Jau Tang; Peter M Rentzepis
Journal:  Proc Natl Acad Sci U S A       Date:  2011-11-07       Impact factor: 11.205

3.  Snapshots of cooperative atomic motions in the optical suppression of charge density waves.

Authors:  Maximilian Eichberger; Hanjo Schäfer; Marina Krumova; Markus Beyer; Jure Demsar; Helmuth Berger; Gustavo Moriena; Germán Sciaini; R J Dwayne Miller
Journal:  Nature       Date:  2010-11-24       Impact factor: 49.962

4.  Chemical physics: Melted in a flash.

Authors:  A Cavalleri
Journal:  Nature       Date:  2009-03-05       Impact factor: 49.962

5.  Electronic acceleration of atomic motions and disordering in bismuth.

Authors:  Germán Sciaini; Maher Harb; Sergei G Kruglik; Thomas Payer; Christoph T Hebeisen; Frank-J Meyer zu Heringdorf; Mariko Yamaguchi; Michael Horn-von Hoegen; Ralph Ernstorfer; R J Dwayne Miller
Journal:  Nature       Date:  2009-03-05       Impact factor: 49.962

6.  Coherent X-ray diffraction imaging of strain at the nanoscale.

Authors:  Ian Robinson; Ross Harder
Journal:  Nat Mater       Date:  2009-04       Impact factor: 43.841

7.  Direct observation of bond formation in solution with femtosecond X-ray scattering.

Authors:  Kyung Hwan Kim; Jong Goo Kim; Shunsuke Nozawa; Tokushi Sato; Key Young Oang; Tae Wu Kim; Hosung Ki; Junbeom Jo; Sungjun Park; Changyong Song; Takahiro Sato; Kanade Ogawa; Tadashi Togashi; Kensuke Tono; Makina Yabashi; Tetsuya Ishikawa; Joonghan Kim; Ryong Ryoo; Jeongho Kim; Hyotcherl Ihee; Shin-ichi Adachi
Journal:  Nature       Date:  2015-02-19       Impact factor: 49.962

8.  X-ray and optical wave mixing.

Authors:  T E Glover; D M Fritz; M Cammarata; T K Allison; Sinisa Coh; J M Feldkamp; H Lemke; D Zhu; Y Feng; R N Coffee; M Fuchs; S Ghimire; J Chen; S Shwartz; D A Reis; S E Harris; J B Hastings
Journal:  Nature       Date:  2012-08-30       Impact factor: 49.962

9.  Mapping molecular motions leading to charge delocalization with ultrabright electrons.

Authors:  Meng Gao; Cheng Lu; Hubert Jean-Ruel; Lai Chung Liu; Alexander Marx; Ken Onda; Shin-Ya Koshihara; Yoshiaki Nakano; Xiangfeng Shao; Takaaki Hiramatsu; Gunzi Saito; Hideki Yamochi; Ryan R Cooney; Gustavo Moriena; Germán Sciaini; R J Dwayne Miller
Journal:  Nature       Date:  2013-04-18       Impact factor: 49.962

Review 10.  Optical laser systems at the Linac Coherent Light Source.

Authors:  Michael P Minitti; Joseph S Robinson; Ryan N Coffee; Steve Edstrom; Sasha Gilevich; James M Glownia; Eduardo Granados; Philippe Hering; Matthias C Hoffmann; Alan Miahnahri; Despina Milathianaki; Wayne Polzin; Daniel Ratner; Franz Tavella; Sharon Vetter; Marc Welch; William E White; Alan R Fry
Journal:  J Synchrotron Radiat       Date:  2015-04-22       Impact factor: 2.616

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