Literature DB >> 16712373

Predicting the long-time dynamic heterogeneity in a supercooled liquid on the basis of short-time heterogeneities.

Asaph Widmer-Cooper1, Peter Harrowell.   

Abstract

We report that the local Debye-Waller factor in a simulated 2D glass-forming mixture exhibits significant spatial heterogeneities and that these short-time fluctuations provide an excellent predictor of the spatial distribution of the long-time dynamic propensities. In contrast, the potential energy per particle of the inherent structure does not correlate well with the spatially distributed dynamics.

Year:  2006        PMID: 16712373     DOI: 10.1103/PhysRevLett.96.185701

Source DB:  PubMed          Journal:  Phys Rev Lett        ISSN: 0031-9007            Impact factor:   9.161


  19 in total

1.  Temperature behavior of the Kohlrausch exponent for a series of vinylic polymers modelled by an all-atomistic approach.

Authors:  S Palato; N Metatla; A Soldera
Journal:  Eur Phys J E Soft Matter       Date:  2011-09-22       Impact factor: 1.890

2.  Correlation between dynamical heterogeneities, structure and potential-energy distribution in a 2D amorphous solid.

Authors:  S Mazoyer; F Ebert; G Maret; P Keim
Journal:  Eur Phys J E Soft Matter       Date:  2011-09-26       Impact factor: 1.890

3.  Field theory of fluctuations in glasses.

Authors:  S Franz; G Parisi; F Ricci-Tersenghi; T Rizzo
Journal:  Eur Phys J E Soft Matter       Date:  2011-09-26       Impact factor: 1.890

4.  Avalanches mediate crystallization in a hard-sphere glass.

Authors:  Eduardo Sanz; Chantal Valeriani; Emanuela Zaccarelli; Wilson C K Poon; Michael E Cates; Peter N Pusey
Journal:  Proc Natl Acad Sci U S A       Date:  2013-12-04       Impact factor: 11.205

5.  Critical-like behaviour of glass-forming liquids.

Authors:  Hajime Tanaka; Takeshi Kawasaki; Hiroshi Shintani; Keiji Watanabe
Journal:  Nat Mater       Date:  2010-02-21       Impact factor: 43.841

6.  Local thermal energy as a structural indicator in glasses.

Authors:  Jacques Zylberg; Edan Lerner; Yohai Bar-Sinai; Eran Bouchbinder
Journal:  Proc Natl Acad Sci U S A       Date:  2017-06-27       Impact factor: 11.205

7.  Bond orientational order in liquids: Towards a unified description of water-like anomalies, liquid-liquid transition, glass transition, and crystallization: Bond orientational order in liquids.

Authors:  Hajime Tanaka
Journal:  Eur Phys J E Soft Matter       Date:  2012-10-31       Impact factor: 1.890

8.  New conserved structural fields for supercooled liquids.

Authors:  Jean Farago; Alexander Semenov; Stefan Frey; Jörg Baschnagel
Journal:  Eur Phys J E Soft Matter       Date:  2014-06-06       Impact factor: 1.890

9.  Vibrational scaling of the heterogeneous dynamics detected by mutual information.

Authors:  Antonio Tripodo; Francesco Puosi; Marco Malvaldi; Dino Leporini
Journal:  Eur Phys J E Soft Matter       Date:  2019-11-22       Impact factor: 1.890

10.  Mutual information reveals multiple structural relaxation mechanisms in a model glass former.

Authors:  Andrew J Dunleavy; Karoline Wiesner; Ryoichi Yamamoto; C Patrick Royall
Journal:  Nat Commun       Date:  2015-01-22       Impact factor: 14.919

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