Literature DB >> 15544413

Ground-state clusters for short-range attractive and long-range repulsive potentials.

S Mossa1, F Sciortino, P Tartaglia, E Zaccarelli.   

Abstract

We report calculations of the ground-state energies and geometries for clusters of different sizes (up to 80 particles), where individual particles interact simultaneously via a short-ranged attractive potential, modeled with a generalization of the Lennard-Jones potential, and a long-ranged repulsive Yukawa potential. We show that for specific choices of the parameters of the repulsive potential, the ground-state energy per particle has a minimum at a finite cluster size. For these values of the parameters in the thermodynamic limit, at low temperatures and small packing fractions, where clustering is favored and cluster-cluster interactions can be neglected, thermodynamically stable cluster phases can be formed. The analysis of the ground-state geometries shows that the spherical shape is marginally stable. In the majority of the studied cases, we find that above a certain size, ground-state clusters preferentially grow almost in one dimension.

Mesh:

Year:  2004        PMID: 15544413     DOI: 10.1021/la048554t

Source DB:  PubMed          Journal:  Langmuir        ISSN: 0743-7463            Impact factor:   3.882


  16 in total

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Review 7.  Nucleation precursors in protein crystallization.

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Journal:  Cryst Growth Des       Date:  2010-11-15       Impact factor: 4.076

9.  Colloidal systems with a short-range attraction and long-range repulsion: Phase diagrams, structures, and dynamics.

Authors:  Yun Liu; Yuyin Xi
Journal:  Curr Opin Colloid Interface Sci       Date:  2019-02       Impact factor: 6.448

10.  Negative normal stress differences N1-N2 in a low concentration capillary suspension.

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Journal:  Soft Matter       Date:  2018-05-02       Impact factor: 3.679

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