Literature DB >> 15245100

Collective nature of the boson peak and universal transboson dynamics of glasses.

A I Chumakov1, I Sergueev, U van Bürck, W Schirmacher, T Asthalter, R Rüffer, O Leupold, W Petry.   

Abstract

Using probe molecules with resonant nuclei and nuclear inelastic scattering, we are able to measure the density of states exclusively for collective motions with a correlation length of more than approximately 20 A. Such spectra exhibit an excess of low-energy modes (boson peak). This peak behaves in the same way as that observed by conventional methods. This shows that a significant part of the modes constituting the boson peak is of collective character. At energies above the boson peak, the reduced density of states of the collective motions universally exhibits an exponential decrease.

Entities:  

Year:  2004        PMID: 15245100     DOI: 10.1103/PhysRevLett.92.245508

Source DB:  PubMed          Journal:  Phys Rev Lett        ISSN: 0031-9007            Impact factor:   9.161


  4 in total

1.  Probing vibrational anisotropy with nuclear resonance vibrational spectroscopy.

Authors:  Jeffrey W Pavlik; Alexander Barabanschikov; Allen G Oliver; E Ercan Alp; Wolfgang Sturhahn; Jiyong Zhao; J Timothy Sage; W Robert Scheidt
Journal:  Angew Chem Int Ed Engl       Date:  2010-06-14       Impact factor: 15.336

2.  Quantitative vibrational dynamics of iron in carbonyl porphyrins.

Authors:  Bogdan M Leu; Nathan J Silvernail; Marek Z Zgierski; Graeme R A Wyllie; Mary K Ellison; W Robert Scheidt; Jiyong Zhao; Wolfgang Sturhahn; E Ercan Alp; J Timothy Sage
Journal:  Biophys J       Date:  2007-03-09       Impact factor: 4.033

3.  Recent advances in biosynthetic modeling of nitric oxide reductases and insights gained from nuclear resonance vibrational and other spectroscopic studies.

Authors:  Saumen Chakraborty; Julian Reed; J Timothy Sage; Nicole C Branagan; Igor D Petrik; Kyle D Miner; Michael Y Hu; Jiyong Zhao; E Ercan Alp; Yi Lu
Journal:  Inorg Chem       Date:  2015-08-14       Impact factor: 5.165

4.  Universal law for the vibrational density of states of liquids.

Authors:  Alessio Zaccone; Matteo Baggioli
Journal:  Proc Natl Acad Sci U S A       Date:  2021-02-02       Impact factor: 11.205

  4 in total

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