| Literature DB >> 15089216 |
Abstract
Nearly logarithmic decay of correlations, which was observed for several supercooled liquids in optical-Kerr-effect experiments [Phys. Rev. Lett. 84, 2437 (2000)]; Phys. Rev. Lett. 90, 197401 (2003)]], is explained within the mode-coupling theory for ideal glass transitions as a manifestation of the beta-peak phenomenon. A schematic model, which describes the dynamics by only two correlators, one referring to density fluctuations and the other to the reorientational fluctuations of the molecules, yields for strong rotation-translation coupling response functions in agreement with those measured for benzophenone and Salol for the time interval extending from 2 ps to about 20 and 200 ns, respectively.Entities:
Year: 2004 PMID: 15089216 DOI: 10.1103/PhysRevLett.92.105701
Source DB: PubMed Journal: Phys Rev Lett ISSN: 0031-9007 Impact factor: 9.161