Literature DB >> 12513499

Three-dimensional director structures of defects in Grandjean-Cano wedges of cholesteric liquid crystals studied by fluorescence confocal polarizing microscopy.

I I Smalyukh1, O D Lavrentovich.   

Abstract

We use a nondestructive technique of fluorescence confocal polarizing microscopy to visualize three-dimensional director patterns of defects in Grandjean-Cano wedges filled with a cholesteric liquid crystal of pitch p=5 microm. Strong surface anchoring of the director causes a stable lattice of dislocations in the bulk. Optical slicing in the vertical cross sections of the wedges allows us to establish the detailed structure of dislocations and their kinks. Dislocations of Burgers vector b=p/2 are located in the thin part of the sample, very close to the bisector plane. Their cores are split into a pair of tau(-1/2) and lambda(+1/2) disclinations. Pairs of lambda(-1/2) and tau(+1/2) disclinations are observed when the b=p/2 dislocation forms a kink. The kinks along the b=p/2 dislocations change the level of dislocations by +/-p/4 and +/-p/2; these kinks are confined to the glide plane and are very long, (5-10) p. Above some critical thickness h(c) of the wedge sample, the dislocations are of Burgers vector b=p. They are often found away from the bisector plane. The core of b=p dislocations is split into a pair of nonsingular lambda(-1/2) and lambda(+1/2) disclinations. The kinks along the b=p dislocation are of a typical size p and form cusps in the direction perpendicular to the glide plane. At the cusp, lambda(-1/2) and lambda(+1/2) disclinations interchange ends. Other defect structures inlude "Lehmann clusters," i.e., dislocations of zero Burgers vector formed by two lambda(-1/2) and two lambda(+1/2) disclinations and dislocations of nonzero Burgers vector with a core split into more than two disclinations. We employ the coarse-grained Lubensky-de Gennes model of the cholesteric phase to describe some of the observed features. We calculate the elastic energy of a dislocation away from the core, estimate the energy of the core split into disclinations of different types, study the effect of finite sample thickness on the dislocations energy, and calculate the Peach-Koehler elastic forces that occur when a dislocation is shifted from its equilibrium position. Balance of the dilation/compression energy in the wedge and the energy of dislocations defines the value of h(c) and allows to estimate the core energy of the dislocations. Finally, we consider the Peierls-Nabarro mechanisms hindering glide of dislocations across the cholesteric layers. Because of the split disclination character of the core, glide is difficult as compared to climb, especially for b=p dislocations.

Entities:  

Year:  2002        PMID: 12513499     DOI: 10.1103/PhysRevE.66.051703

Source DB:  PubMed          Journal:  Phys Rev E Stat Nonlin Soft Matter Phys        ISSN: 1539-3755


  13 in total

1.  Reconfigurable interactions and three-dimensional patterning of colloidal particles and defects in lamellar soft media.

Authors:  Rahul P Trivedi; Ivan I Klevets; Bohdan Senyuk; Taewoo Lee; Ivan I Smalyukh
Journal:  Proc Natl Acad Sci U S A       Date:  2012-03-12       Impact factor: 11.205

2.  Selective imaging of 3D director fields and study of defects in biaxial smectic A liquid crystals.

Authors:  I I Smalyukh; R Pratibha; N V Madhusudana; O D Lavrentovich
Journal:  Eur Phys J E Soft Matter       Date:  2005-02-22       Impact factor: 1.890

3.  Light-induced rewiring and winding of Saturn ring defects in photosensitive chiral nematic colloids.

Authors:  I Gvozdovskyy; V S R Jampani; M Skarabot; I Muševič
Journal:  Eur Phys J E Soft Matter       Date:  2013-09-05       Impact factor: 1.890

4.  Spontaneous helielectric nematic liquid crystals: Electric analog to helimagnets.

Authors:  Xiuhu Zhao; Junchen Zhou; Jinxing Li; Junichi Kougo; Zhe Wan; Mingjun Huang; Satoshi Aya
Journal:  Proc Natl Acad Sci U S A       Date:  2021-10-19       Impact factor: 11.205

5.  Topological barriers to defect nucleation generate large mechanical forces in an ordered fluid.

Authors:  Bruno Zappone; Roberto Bartolino
Journal:  Proc Natl Acad Sci U S A       Date:  2021-11-02       Impact factor: 11.205

6.  Layering transitions and metastable structures of cholesteric liquid crystals in cylindrical confinement.

Authors:  Jonghee Eun; Joseph Pollard; Sung-Jo Kim; Thomas Machon; Joonwoo Jeong
Journal:  Proc Natl Acad Sci U S A       Date:  2021-08-17       Impact factor: 11.205

7.  Design of nematic liquid crystals to control microscale dynamics.

Authors:  Oleg D Lavrentovich
Journal:  Liq Cryst Rev       Date:  2021-05-26       Impact factor: 3.700

8.  Electrically tunable selective reflection of light from ultraviolet to visible and infrared by heliconical cholesterics.

Authors:  Jie Xiang; Yannian Li; Quan Li; Daniel A Paterson; John M D Storey; Corrie T Imrie; Oleg D Lavrentovich
Journal:  Adv Mater       Date:  2015-03-27       Impact factor: 30.849

9.  Topology-commanded optical properties of bistable electric-field-induced torons in cholesteric bubble domains.

Authors:  Andrii Varanytsia; Gregor Posnjak; Urban Mur; Vinay Joshi; Kelsey Darrah; Igor Muševič; Simon Čopar; Liang-Chy Chien
Journal:  Sci Rep       Date:  2017-11-23       Impact factor: 4.379

10.  Points, skyrmions and torons in chiral nematic droplets.

Authors:  Gregor Posnjak; Simon Čopar; Igor Muševič
Journal:  Sci Rep       Date:  2016-05-20       Impact factor: 4.379

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