Paul C V Thrane1,2, Chao Meng1, Fei Ding1, Sergey I Bozhevolnyi1. 1. Centre for Nano Optics, University of Southern Denmark, Campusvej 55, Odense DK-5230, Denmark. 2. SINTEF Smart Sensors and Microsystems, Gaustadalleen 23C, 0737 Oslo, Norway.
Abstract
Tunable metasurfaces promise to enable adaptive optical systems with complex functionalities. Among possible realizations, a recent platform combining microelectromechanical systems (MEMS) with gap-surface plasmon (GSP) metasurfaces offers high modulation efficiency, broadband operation, and fast response. We compare tunable metasurfaces operating in GSP and Fabry-Pérot (FP) regions by investigating polarization-independent blazed gratings both numerically and experimentally. Peak efficiency is calculated to be ∼75% in both cases (∼40% in measurements), while the operation bandwidth is found larger when operating in the GSP region. Advantages of operating in the FP region include relaxed assembly requirements and operation tolerances. Additionally, simulation and experimental results show that coupling between neighboring unit cells increases for larger air gaps, resulting in deteriorated efficiency. We believe the presented analysis provides important guidelines for designing tunable metasurfaces for diverse applications in miniaturized adaptive optical systems.
Tunable metasurfaces promise to enable adaptive optical systems with complex functionalities. Among possible realizations, a recent platform combining microelectromechanical systems (MEMS) with gap-surface plasmon (GSP) metasurfaces offers high modulation efficiency, broadband operation, and fast response. We compare tunable metasurfaces operating in GSP and Fabry-Pérot (FP) regions by investigating polarization-independent blazed gratings both numerically and experimentally. Peak efficiency is calculated to be ∼75% in both cases (∼40% in measurements), while the operation bandwidth is found larger when operating in the GSP region. Advantages of operating in the FP region include relaxed assembly requirements and operation tolerances. Additionally, simulation and experimental results show that coupling between neighboring unit cells increases for larger air gaps, resulting in deteriorated efficiency. We believe the presented analysis provides important guidelines for designing tunable metasurfaces for diverse applications in miniaturized adaptive optical systems.
Metasurfaces have successfully demonstrated
a wide range of optical
effects and components,[1−5] with a lot of recent research focusing on developing metasurfaces
with tunable properties to enable adaptive optical components and
with several different techniques being followed, each having their
own advantages and disadvantages.[6−9] One method to achieve this tunability is,
for instance, to include materials that undergo a phase change. GeSbTe
can, for example, change from having a crystal structure to an amorphous
state depending on the temperature, with the two states having very
different permittivity.[10] By incorporating
resistive heaters, it is thus possible to make metasurface elements
that can change their resonances quite significantly with a drawback
being that demonstrated devices have slow switching time.[11] Faster responses have been demonstrated using
the electro-optic effect in lithium niobate[12,13] or by modulating the free carrier density using electric[14] or optical[15] signals,
with an issue being that the permittivity changes are limited to thin
accumulation or depletion layers giving low modulation ranges.[7] The effect can be enhanced by using ε-near-zero
materials[16] or by using 2D materials such
as graphene[17] or black phosphorus.[18] Liquid crystals enable larger and more efficient
modulation by changing the refractive index around the nanostructures[7] but again have slower responses due to the time
it takes to rotate the molecules.[19] Metasurfaces
can also be adjusted through mechanically altering the system, with
demonstrated concepts including embedding the nanostructures in a
stretchable polymer[20] or incorporating
the metasurface with MEMS.[21] MEMS based
tunable metasurfaces can achieve high efficiency modulation while
still switching fast enough for many applications depending on the
specific mechanical implementation, with most systems being able to
operate in the range from one kHz up to several hundred kHz.[22] For visible and near-IR frequencies the individual
meta-atoms are so small that individual actuation by MEMS is challenging,
while collective modulation of all meta-atoms is more straightforward.One such recently demonstrated platform[23] consists of a gold MEMS mirror[24] and
a glass substrate with gold nanostructures, where the air gap between
the nanostructures and mirror can be controlled accurately. The system
is designed to function as a reflective optical metasurface (OMS)
for light with wavelength λ = 800 nm when the air gap is less
than 50 nm. For these small separations there are GSP resonances[25] due to the near field coupling of the nanostructures
and mirror. By moving the mirror away, these GSP resonances disappear,
switching off the metasurface functionality and replacing it with
that of a standard mirror. The experimentally demonstrated efficiency
of this system was 50%, with switching times less than 0.4 ms. In
this work we describe how the same MEMS-OMS platform can function
also for larger air gaps owing to hybrid plasmonic FP resonances.[26,27] This configuration has recently been used to achieve efficient and
fast 0–2π birefringence control in reflection.[28] Not only is fabrication easier at larger air
gaps since any particle or unevenness may obstruct the MEMS mirror
from getting close enough for the GSP resonances, but larger gaps
could also help reduce the trade-off between aperture size and switching
speed by alleviating squeeze film air damping in the system.[29] Additionally, the amount of simulations required
for design is reduced through the use of the analytic FP equation,
removing the need to simulate the response for every air gap separately.
We show also that the simulated peak efficiency is around 75% for
metasurfaces working in both GSP and FP regions, while the bandwidth
is larger for the GSP metasurface with around 2 times the bandwidth
when comparing with the metasurface working at the first FP resonance.
For larger air gaps there is progressively more coupling/cross-talk
between neighboring nanostructures due to scattering and multiple
reflections in the FP cavity, resulting in a gradual decrease in metasurface
efficiency. This is a result of the metasurface design being based
on simulations where the unit cells are placed in arrays of identical
structures, whereas the actual metasurface may generally consist of
varying meta-atoms. We verify this effect both numerically and experimentally.
Results and Discussion
To compare plasmonic metasurfaces
designed to work in the GSP and
FP regions, we first calculate the complex reflection coefficient
for different nanostructure geometries at two nanostructure–substrate
separations corresponding to the two regions. Figure a and Figure b illustrate the MEMS-OMS and its constituent unit
cells used in this work. Specifically, the periodically repeated unit
cell has a side length Λ and consists of a gold nanobrick with
thickness t and side
lengths L and L and separated from a gold
substrate by an air gap Ta. In physical
implementations there needs to be a dielectric substrate supporting
the nanobricks; this has been omitted in the simulations except when
comparing with the experimental measurements discussed later. To design
the dynamic MEMS-OMS, we set the working wavelength at λ = 800
nm and choose the unit cell size of 250 nm to avoid any high-order
diffraction and excitation of surface waves. Meanwhile, the optimal
nanobrick thickness t is found to be 50 nm, ensuring large reflection amplitudes and wide
phase coverage.[23,30]Figure c and Figure d show electric field plots for two configurations
of the unit cell, while Figure e and Figure f show the reflection coefficients as a function of L and L for two different values of Ta for normally incident x-polarized excitation
at λ = 800 nm. At Ta = 20 nm, there
is a GSP resonance around L = 150 nm with near field coupling between the substrate and
nanobrick as can be seen in the plot of the electric field in Figure c. At Ta = 430 nm, there is a less sharp resonance centered around L = 160 nm, due to a hybrid
plasmonic/FP resonance between the substrate and the layer of nanobricks
since the near-field coupling between the nanobricks and substrate
is negligible, as shown in Figure d. As can be seen by comparing the phase contours in Figure e and Figure f, the range of available reflection
phases are slightly larger for the case where Ta = 20 nm; however the difference is not significant enough
to give larger efficiencies for the blazed grating designs presented
later. The phase profiles for these gratings are shown in Figure S1.
Figure 1
MEMS-OMS unit cell design within respective
GSP and FP regions.
(a, b) Schematic illustration of the MEMS-OMS metasurface and unit
cell. A gold brick with side lengths L and L and thickness t of
50 nm is situated a distance Ta away from
a gold substrate. The unit cell has a square footprint with side lengths
Λ = 250 nm. (c, d) The norm of the electric field in the xz plane at the center of the nanobricks for x-polarized excitation at normal incidence with separation distances
of Ta = 20 nm and Ta = 430 nm, respectively. The nanobrick geometries are indicated
as black squares in (e) and (f). (e, f) Absolute value of the complex
reflection coefficients calculated as a function of nanobrick dimensions L and L at the wavelength of λ = 800 nm for
(e) Ta = 20 nm and (f) Ta = 430 nm. The color maps represent the reflection amplitude
for x-polarized excitation at normal incidence, while
the blue and black contour lines indicate the reflection phases acquired
for x- and y-polarized excitations,
respectively. Blue circles indicate nanobrick geometries for composing
the polarization independent MEMS-OMS blazed gratings optimized in
respective GSP and FP regions. The phase and reflection amplitudes
of these nanobricks are shown in Figure S1.
MEMS-OMS unit cell design within respective
GSP and FP regions.
(a, b) Schematic illustration of the MEMS-OMS metasurface and unit
cell. A gold brick with side lengths L and L and thickness t of
50 nm is situated a distance Ta away from
a gold substrate. The unit cell has a square footprint with side lengths
Λ = 250 nm. (c, d) The norm of the electric field in the xz plane at the center of the nanobricks for x-polarized excitation at normal incidence with separation distances
of Ta = 20 nm and Ta = 430 nm, respectively. The nanobrick geometries are indicated
as black squares in (e) and (f). (e, f) Absolute value of the complex
reflection coefficients calculated as a function of nanobrick dimensions L and L at the wavelength of λ = 800 nm for
(e) Ta = 20 nm and (f) Ta = 430 nm. The color maps represent the reflection amplitude
for x-polarized excitation at normal incidence, while
the blue and black contour lines indicate the reflection phases acquired
for x- and y-polarized excitations,
respectively. Blue circles indicate nanobrick geometries for composing
the polarization independent MEMS-OMS blazed gratings optimized in
respective GSP and FP regions. The phase and reflection amplitudes
of these nanobricks are shown in Figure S1.The transition between these GSP and FP regions
is displayed in Figure , where the reflection
coefficients for different brick sizes are shown as a function of Ta. The first FP resonance is located around Ta = 350 nm with Ta + T/2 close to λ/2,
with a difference corresponding to the phase change upon reflection
on the gold mirror. At this separation the system acts as a gold mirror
with the reflection coefficient being independent of L and L, since at this separation distance the nanostructures
are centered in the interference minimum from the superposition of
incident and relected fields. For slightly larger air gaps the reflection
is very dependent on the nanobrick dimensions (e.g., Ta = 430 nm as shown in Figure f) and then gradually returns to mirror-like
behavior at the second FP resonance located around Ta + T/2
close to λ, with the pattern repeating for subsequent FP apart
by a spaced separation of λ/2, again with a small correction
due to the phase change upon multiple reflections on the gold mirror.
This can be accurately described with the FP equation:[26]where the total reflection coefficient rtot is given as a function of the reflection
and transmission coefficients r and t, with
the light incident on region j from region i and the subscripts 1, 2, and 3 respectively referring
to the regions above the nanobricks, between the nanobricks and substrate,
and the substrate. Note that the reflection and transmission coefficients
in general are dependent on the polarization and incidence angle of
the light. With mirror-symmetric nanostructures and both regions 1
and 2 consisting of the same material (e.g., air), we have r12 = r21, t12 = t21, and n2 = 1. Ta cos(θ2) is the effective air gap for light traversing the gap with
an angle θ2 and can be simplified as Ta for normal incidence. By simulating the structures without
any gold substrate, the reflection and transmission coefficients r and t are determined for each nanobrick geometry. Equation is then used to
calculate the total reflection coefficient as a function of Ta, thus avoiding the requirement of simulating
the full structure for every air gap separation. This method gives
correct results except for very small air gaps, in this case Ta < 80 nm = λ/10, where near-field
coupling and corresponding GSP excitation must be taken into account.
The difference between the results from eq and full-wave simulations including the substrate
can be clearly observed for small gap sizes in Figure S2.
Figure 2
Complex reflection coefficients as a function of air gap
and nanobrick
dimensions. The color map represents the reflection amplitudes for
normally incident x-polarized light, while the contour
lines indicate the reflection phases. The three subfigures represent
three different cases of the nanobrick dimensions, namely, (a) square
bricks (L = L), (b) constant L = 100 nm, and (c) constant L = 100 nm. The light is normally
incident and with wavelength 800 nm.
Complex reflection coefficients as a function of air gap
and nanobrick
dimensions. The color map represents the reflection amplitudes for
normally incident x-polarized light, while the contour
lines indicate the reflection phases. The three subfigures represent
three different cases of the nanobrick dimensions, namely, (a) square
bricks (L = L), (b) constant L = 100 nm, and (c) constant L = 100 nm. The light is normally
incident and with wavelength 800 nm.After analyzing the polarization-dependent responses
of the unit
cell in both GSP and FP regions, we start to implement functional
metasurfaces. Figure compares the performance of two blazed metasurface gratings, one
optimized for Ta = 20 nm and the other
for Ta = 430 nm. As illustrated in Figure a, the metasurface
gratings consist of a periodic array of 12 elements, with the first
2 elements empty while the other dimensions are chosen and marked
with blue circles in Figure e and Figure f to provide large reflection amplitudes and an approximately linear
phase gradient along the x-direction.
Figure 3
Dynamic MEMS-OMS blazed
gratings designed for respective GSP and
FP regions. (a) Supercell sketches of the 12-element polarization-independent
dynamic MEMS-OMS blazed gratings. Outlines of the nanobrick dimensions
optimized for Ta = 20 nm and Ta = 430 nm are indicated with black squares and orange
dashed lines, respectively. (b, c) Calculated diffraction efficiencies
into the specular (m = 0) and first diffraction order
(m = +1) as a function of wavelength with the optimal
air gap for each grating, for x- and y-polarized excitations. (d, e) Calculated diffraction efficiencies
as a function of air gap Ta at λ
= 800 nm for x- and y-polarized
excitations.
Dynamic MEMS-OMS blazed
gratings designed for respective GSP and
FP regions. (a) Supercell sketches of the 12-element polarization-independent
dynamic MEMS-OMS blazed gratings. Outlines of the nanobrick dimensions
optimized for Ta = 20 nm and Ta = 430 nm are indicated with black squares and orange
dashed lines, respectively. (b, c) Calculated diffraction efficiencies
into the specular (m = 0) and first diffraction order
(m = +1) as a function of wavelength with the optimal
air gap for each grating, for x- and y-polarized excitations. (d, e) Calculated diffraction efficiencies
as a function of air gap Ta at λ
= 800 nm for x- and y-polarized
excitations.In general the metasurface can be designed to control
two orthogonal
polarization states independently by using anisotropic elements, but
the blazed grating is made polarization independent by choosing isotropic
elements with L = L. Figure b and Figure c show the diffraction efficiencies of the two gratings
for x- and y-polarized light as
a function of wavelength, where the polarization independent behavior
can be observed. The efficiencies of the +1 diffraction order at the
design wavelength of λ = 800 nm are similar for both gratings,
with the values approaching 75%. However, the operating bandwidth
is different. The grating working at Ta = 20 nm has an efficiency above 60% in the wavelength range between
760 and 900 nm, while for the grating working at Ta = 430 nm the corresponding wavelength range is only
spanning from 770 to 825 nm. This reduced bandwidth is due to the
fact that the FP resonance is narrower than the GSP resonance. At
higher order FP resonances, the bandwidth will be reduced even further
as the resonance requires the air gap to be an integer multiple of
half wavelengths. Conversely, this effect might be used to design
highly chromatic metasurfaces by choosing a large air gap. Figure d and Figure e compare the diffraction efficiencies
of two metasurface gratings for x- and y-polarized light as a function of Ta at
the design wavelength of 800 nm. Impressively, both metasurface gratings
achieve more than 65% reflection in the +1 diffraction order when
the air gap is Ta = 20 nm and Ta = 430 nm due to the similarity of the meta-atoms.
But there is a clear gain in efficiency by tailoring the meta-atoms
for the relevant air gap, which is true for both polarization states.One may expect the same responses for metasurface blazed gratings
with repeating FP regions. However, in our simulations and experimental
results we observe a decrease in the +1 order efficiency at higher
order FP resonances in combination with more reflection into other
diffraction orders, which can be understood as increased coupling
or cross-talk between neighboring nanostructures via reflections in
the gold substrate. Figure a shows another 12-element blazed grating optimized for Ta = 20 nm. As earlier, the choice of nanobrick
dimensions is based on simulations where the nanobricks are placed
in an array of identical neighbors, while in practical applications
the neighbors may have any geometry. This has been shown to not significantly
affect the performance of GSP metasurfaces as long as the phase gradient
is not too large.[25] However, as can be
seen in the reflection amplitude for the diffraction orders plotted
in Figure b, the efficiency
of the grating degrades as Ta increases,
with light going into unwanted diffraction modes other than the desired
+1 diffraction order, falling from 72% at Ta = 430 nm to 66% at the fourth FP resonance due to increased coupling
between elements within the supercell via the mirror substrate. In Figure S3, the same effect is visible for a grating
made of 8 unit cells. With fewer meta-atoms the neighboring nanobricks
are less similar in size, resulting in a larger drop in efficiency
going from around 70% at Ta = 430 nm to
less than 50% at the fourth FP resonance. The reflected field distributions
for a blazed grating at several different air gap separations are
shown in Figure S4. Figure c and Figure d show experimental measurements of a fabricated metasurface
paired with a piezoelectric MEMS mirror, showing the same gradual
decrease of the maximum diffraction efficiency from around 38% at
the first FP resonance to 30% at the fourth FP resonance for both
polarization states, together with increased intensity in the +2 diffraction
order. This coupling issue is especially important when making high
NA lenses or other components requiring large deflection angles, where
the large phase gradient will require nanobricks that differ significantly
from their neighbors. Details and some discussion of the fabrication
and optical characterization can be found in Figures S5 and S6, while Figure S7 describes
the measurements done to determine the relationship between air gap
and voltage applied to the MEMS mirror. It should be noted that the
minimal air gap achieved with the measured sample was ∼150
nm, sufficient for FP operation but not optimal for GSP operation.
Closer separations can be achieved[23] but
likely requires significantly more effort to be produced with high
yield and might be harder to realize with larger apertures. To conclude,
we show how the recently developed MEMS-OMS platform is not limited
to working in the GSP region. For larger air gaps the FP resonances
enable the system to still function as a metasurface, with slightly
smaller phase range and similar efficiencies if the nanostructure
geometries are optimized to work at the relevant air gap. The main
advantage of allowing for larger air gaps is alleviating issues with
thin film damping for high speed operation, as well as simplifying
fabrication tolerances as decreasing the air gap below 50 nm is a
very challenging problem, requiring flat parallel surfaces free from
any particles or irregularities that may obstruct the MEMS movement.
Meanwhile, working in the GSP region gives better bandwidth and fewer
issues with coupling between meta-atoms, which causes the system to
change behavior between different FP periods when having metasurfaces
comprised of nonidentical meta-atoms. Ultimately, the choice between
two different, albeit similar, operation regimes of the considered
MEMS-OMS platform should be made by carefully considering all implications
of their advantages and drawbacks, highlighted in this work, to targeted
functionalities and particular applications in optical systems.
Figure 4
Effect of coupling
via mirror substrate on grating efficiency:
comparison of simulations and experimental measurements. (a) Supercell
of a MEMS-OMS dynamic blazed grating with 12 meta-atoms optimized
for the GSP region. (b) Diffraction efficiencies as a function of
air gap Ta. For these simulations the
gold nanobricks are placed on a glass substrate, which is the case
for the fabricated OMS shown in (c). The OMS is placed in close proximity
(<3 μm) to a piezoelectric MEMS gold mirror. The air gap
can then be changed by applying voltages on the MEMS. The measured
diffraction efficiencies are shown in (d). The air gap values in (d)
have been added by measuring the approximate relationship between
air gap and voltage as described in Figure S7. In both (b) and (d) the upper (lower) plot is for x-polarized (y-polarized) excitation. The nanobrick
thickness is 50 nm, and the wavelength is 800 nm.
Effect of coupling
via mirror substrate on grating efficiency:
comparison of simulations and experimental measurements. (a) Supercell
of a MEMS-OMS dynamic blazed grating with 12 meta-atoms optimized
for the GSP region. (b) Diffraction efficiencies as a function of
air gap Ta. For these simulations the
gold nanobricks are placed on a glass substrate, which is the case
for the fabricated OMS shown in (c). The OMS is placed in close proximity
(<3 μm) to a piezoelectric MEMS gold mirror. The air gap
can then be changed by applying voltages on the MEMS. The measured
diffraction efficiencies are shown in (d). The air gap values in (d)
have been added by measuring the approximate relationship between
air gap and voltage as described in Figure S7. In both (b) and (d) the upper (lower) plot is for x-polarized (y-polarized) excitation. The nanobrick
thickness is 50 nm, and the wavelength is 800 nm.
Methods
The simulations were done using COMSOL Multiphysics
5.6 with the
Wave Optics module. The refractive index for gold was interpolated
from experimental values[31] for both the
gold substrate and gold nanobricks. When simulating individual nanobricks,
the unit cell is set to have periodic conditions in both x- and y-directions, while the gold substrate is
backed by a perfect electrical conductor condition and the air region
is padded with a perfectly matched layer. When using eq the coefficients r12, r21, t12, and t21 are determined
by simulating the nanobricks without the gold substrate, with perfectly
matched layers backing the domains on both sides of the nanostructure
in the z-direction. r23, the reflection coefficient for the gold substrate for light with
normal incidence, is determined byn2 being the refractive
index of the layer above the substrate (in this case air, n2 = 1) and n3 the
refractive index of gold. The light was set to be normally incident
for all simulations, and the results were calculated independently
for light linearly polarized in the x- and y-directions. When simulating gratings with large air gaps
and many nanobricks, the simulation volume was reduced by simulating
half the unit cell and replacing the periodic boundary conditions
in the y-direction by perfectly magnetic or electric
conductors depending on the incident polarization state. For the simulations
in Figure , the nanobricks
were placed on a lossless dielectric material with refractive index
1.46.Fabrication of the MEMS metasurface devices is done by
individually
manufacturing MEMS micromirrors and glass substrates containing the
metasurfaces, before manually gluing the MEMS chips and glass substrates
together in a cleanroom environment. A description and discussion
of this process can be found in Figure S5. Additional details can also be found in refs (24) and (32) for MEMS fabrication and
refs (23) and (28) for the MEMS–metasurface
combination.Optical characterization is done by sending laser
light with wavelength
800 nm through a linear polarizer, half wave plate (used to switch
between two linear polarization states), and beam splitter and then
focusing onto the sample using a microscope objective. The light is
reflected back into the objective and is redirected by the beam splitter,
before tube lens, iris (in image plane for spatial filtering), and
two lenses that relay the light onto a CMOS camera. The last lens
can be flipped in and out of the optical path to switch between capturing
the direct and Fourier images. The direct object image is used to
ensure the signal is collected from only the metasurface area, while
the intensity in the different diffraction orders is measured by integrating
the intensity of the corresponding areas in the Fourier plane image.
Details on the equipment and a diagram of the setup can be found in Figure S6.
Authors: Yao-Wei Huang; Ho Wai Howard Lee; Ruzan Sokhoyan; Ragip A Pala; Krishnan Thyagarajan; Seunghoon Han; Din Ping Tsai; Harry A Atwater Journal: Nano Lett Date: 2016-09-02 Impact factor: 11.189