Literature DB >> 35858305

Ultrahigh efficient emulsification with drag-reducing liquid gating interfacial behavior.

Shijie Yu1, Yuan Jing2, Yi Fan1, Linghu Xiong3, Huimeng Wang1, Jinmei Lei1, Yunmao Zhang1, Jing Liu1, Shuli Wang1,4, Xinyu Chen5, Hao Sun3,6, Xu Hou1,2,7.   

Abstract

Emulsification is a crucial technique for mixing immiscible liquids into droplets in numerous areas ranging from food to medicine to chemical synthesis. Commercial emulsification methods are promising for high production, but suffer from high energy input. Here, we report a very simple and scalable emulsification method that employs the drag-reducing liquid gating structure to create a smooth liquid-liquid interface for the reduction of resistance and tunable generation of droplets with good uniformity. Theoretical modeling and experimental results demonstrate that our method exhibits ultrahigh efficiency, which can reach up to more than 4 orders of magnitude greater energy-saving compared to commercial methods. For temperature-sensitive biological components, such as enzymes, proteins, and bacteria, it can offer a comfortable environment to avoid exposure to high temperatures during emulsifying, and the interface also enables the suppression of fouling. This unique drag-reducing liquid gating interfacial emulsification mechanism promotes the efficiency of droplet generation and provides fresh insight into the innovation of emulsifications that can be applied in many fields, including the food industry, the daily chemical industry, biomedicine, material fabrication, the petrochemical industry, and beyond.

Entities:  

Keywords:  drag-reducing interfacial behavior; droplet; efficient emulsification; liquid gating; liquid structure

Year:  2022        PMID: 35858305      PMCID: PMC9304007          DOI: 10.1073/pnas.2206462119

Source DB:  PubMed          Journal:  Proc Natl Acad Sci U S A        ISSN: 0027-8424            Impact factor:   12.779


  29 in total

1.  Liquid-based gating mechanism with tunable multiphase selectivity and antifouling behaviour.

Authors:  Xu Hou; Yuhang Hu; Alison Grinthal; Mughees Khan; Joanna Aizenberg
Journal:  Nature       Date:  2015-03-05       Impact factor: 49.962

2.  Multichannel Dynamic Interfacial Printing: An Alternative Multicomponent Droplet Generation Technique for Lab in a Drop.

Authors:  Shenglong Liao; Xinglei Tao; Yingjiao Ju; Jie Feng; Wenbin Du; Yapei Wang
Journal:  ACS Appl Mater Interfaces       Date:  2017-12-06       Impact factor: 9.229

3.  Sustained release of dexamethasone from hydrophilic matrices using PLGA nanoparticles for neural drug delivery.

Authors:  Dong-Hwan Kim; David C Martin
Journal:  Biomaterials       Date:  2006-01-27       Impact factor: 12.479

4.  Electrospun Liquid-Infused Membranes for Emulsified Oil/Water Separation.

Authors:  Chen Song; Gregory C Rutledge
Journal:  Langmuir       Date:  2022-02-07       Impact factor: 3.882

5.  Synchronized Reagent Delivery in Double Emulsions for Triggering Chemical Reactions and Gene Expression.

Authors:  Ariane Stucki; Petra Jusková; Nicola Nuti; Steven Schmitt; Petra S Dittrich
Journal:  Small Methods       Date:  2021-06-25

6.  Prediction of dexamethasone release from PLGA microspheres prepared with polymer blends using a design of experiment approach.

Authors:  Bing Gu; Diane J Burgess
Journal:  Int J Pharm       Date:  2015-09-15       Impact factor: 5.875

7.  On-demand modulation of 3D-printed elastomers using programmable droplet inclusions.

Authors:  Hing Jii Mea; Luis Delgadillo; Jiandi Wan
Journal:  Proc Natl Acad Sci U S A       Date:  2020-06-15       Impact factor: 11.205

8.  Fluorescent Janus emulsions for biosensing of Listeria monocytogenes.

Authors:  Jie Li; Suchol Savagatrup; Zachary Nelson; Kosuke Yoshinaga; Timothy M Swager
Journal:  Proc Natl Acad Sci U S A       Date:  2020-05-15       Impact factor: 11.205

9.  Engineering the Deformability of Albumin-Stabilized Emulsions for Lymph-Node Vaccine Delivery.

Authors:  Tiantian Song; Yufei Xia; Yiqun Du; Michael W Chen; Hong Qing; Guanghui Ma
Journal:  Adv Mater       Date:  2021-05-19       Impact factor: 30.849

10.  Host-guest liquid gating mechanism with specific recognition interface behavior for universal quantitative chemical detection.

Authors:  Huimeng Wang; Yi Fan; Yaqi Hou; Baiyi Chen; Jinmei Lei; Shijie Yu; Xinyu Chen; Xu Hou
Journal:  Nat Commun       Date:  2022-04-07       Impact factor: 17.694

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