| Literature DB >> 34881491 |
Kumar Dilip Ashtekar1, Hadi Gholami2, Mehdi Moemeni2, Ankush Chakraborty2, Lindsey Kiiskila2, Xinliang Ding2, Edmond Toma2, Christopher Rahn2, Babak Borhan2.
Abstract
Employing halenium affinity (HalA) as a guiding tool, the weak nucleophilic character of alkyl ketones was modulated by the templating effect of a tethered 2-tetrahydropyranyl(THP)-protected alcohol towards realizing a bromenium ion initiated spiroketalization cascade. Addition of ethanol aided an early termination of the cascade by scavenging the THP group after the halofunctionalization stage, furnishing monobromospiroketals. Alternatively, exclusion of ethanol from the reaction mixture biased the transient oxocarbenium towards α-deprotonation that precedes a second bromofunctionalization event thus, furnishing dibrominated spiroketals. The regio- and stereoselectivity exploited in the current methodology provides a novel and rapid access to the dibrominated spiroketal motifs exhibited by several natural products.Entities:
Keywords: Halenium affinity; Halocyclization; Reaction mechanisms; Spiroketalization
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Year: 2022 PMID: 34881491 PMCID: PMC9254888 DOI: 10.1002/anie.202115173
Source DB: PubMed Journal: Angew Chem Int Ed Engl ISSN: 1433-7851 Impact factor: 16.823