Literature DB >> 34591623

Achieving net-zero greenhouse gas emission plastics by a circular carbon economy.

Raoul Meys1,2, Arne Kätelhön1,2, Marvin Bachmann1, Benedikt Winter1,3, Christian Zibunas1, Sangwon Suh4, André Bardow1,3,5.   

Abstract

Mitigating life-cycle greenhouse gas emissions of plastics is perceived as energy intensive and costly. We developed a bottom-up model that represents the life cycle of 90% of global plastics to examine pathways to net-zero emission plastics. Our results show that net-zero emission plastics can be achieved by combining biomass and carbon dioxide (CO2) utilization with an effective recycling rate of 70% while saving 34 to 53% of energy. Operational costs for net-zero emission plastics are in the same range as those for linear fossil-based production with carbon capture and storage and could even be substantially reduced. Realizing the full cost-saving potential of 288 billion US dollars requires low-cost supply of biomass and CO2, high-cost supply of oil, and incentivizing large-scale recycling and lowering investment barriers for all technologies that use renewable carbon feedstock.

Entities:  

Year:  2021        PMID: 34591623     DOI: 10.1126/science.abg9853

Source DB:  PubMed          Journal:  Science        ISSN: 0036-8075            Impact factor:   47.728


  10 in total

Review 1.  Mechanism-Based Design of Efficient PET Hydrolases.

Authors:  Ren Wei; Gerlis von Haugwitz; Lara Pfaff; Jan Mican; Christoffel P S Badenhorst; Weidong Liu; Gert Weber; Harry P Austin; David Bednar; Jiri Damborsky; Uwe T Bornscheuer
Journal:  ACS Catal       Date:  2022-02-28       Impact factor: 13.084

2.  Cascade degradation and upcycling of polystyrene waste to high-value chemicals.

Authors:  Zhen Xu; Fuping Pan; Mengqi Sun; Jianjun Xu; Nuwayo Eric Munyaneza; Zacary L Croft; Gangshu George Cai; Guoliang Liu
Journal:  Proc Natl Acad Sci U S A       Date:  2022-08-15       Impact factor: 12.779

3.  Biosensor and chemo-enzymatic one-pot cascade applications to detect and transform PET-derived terephthalic acid in living cells.

Authors:  Thomas Bayer; Lara Pfaff; Yannick Branson; Aileen Becker; Shuke Wu; Uwe T Bornscheuer; Ren Wei
Journal:  iScience       Date:  2022-04-29

4.  Closed-loop additive manufacturing of upcycled commodity plastic through dynamic cross-linking.

Authors:  Sungjin Kim; Md Anisur Rahman; Md Arifuzzaman; Dustin B Gilmer; Bingrui Li; Jackson K Wilt; Edgar Lara-Curzio; Tomonori Saito
Journal:  Sci Adv       Date:  2022-06-03       Impact factor: 14.957

Review 5.  Opportunities and challenges for the application of post-consumer plastic waste pyrolysis oils as steam cracker feedstocks: To decontaminate or not to decontaminate?

Authors:  Marvin Kusenberg; Andreas Eschenbacher; Marko R Djokic; Azd Zayoud; Kim Ragaert; Steven De Meester; Kevin M Van Geem
Journal:  Waste Manag       Date:  2021-12-03       Impact factor: 7.145

6.  Chemically recyclable polyesters from CO2, H2, and 1,3-butadiene.

Authors:  Yongjia Lou; Luyan Xu; Ninglin Gan; Yunyan Sun; Bo-Lin Lin
Journal:  Innovation (Camb)       Date:  2022-02-05

7.  Chemical Recycling of Poly(Cyclohexene Carbonate) Using a Di-MgII Catalyst.

Authors:  Frances N Singer; Arron C Deacy; Thomas M McGuire; Charlotte K Williams; Antoine Buchard
Journal:  Angew Chem Int Ed Engl       Date:  2022-05-05       Impact factor: 16.823

8.  Anaerobic Digested Wastewater CO2 Sequestration Using a Biophotocatalytic System with a Magnetized Photocatalyst (Fe-TiO2).

Authors:  Emmanuel Kweinor Tetteh; Gloria Amo-Duodu; Sudesh Rathilal
Journal:  Molecules       Date:  2022-08-16       Impact factor: 4.927

9.  A Bio-Based Supramolecular Adhesive: Ultra-High Adhesion Strengths at both Ambient and Cryogenic Temperatures and Excellent Multi-Reusability.

Authors:  Peng Sun; Shan Mei; Jiang-Fei Xu; Xi Zhang
Journal:  Adv Sci (Weinh)       Date:  2022-08-09       Impact factor: 17.521

10.  Knowledge Mapping and Institutional Prospects on Circular Carbon Economy Based on Scientometric Analysis.

Authors:  Zhengai Dong; Lichen Zhang; Houjian Li; Yanhui Gong; Yue Jiang; Qiumei Peng
Journal:  Int J Environ Res Public Health       Date:  2022-09-30       Impact factor: 4.614

  10 in total

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