Literature DB >> 34417307

Droplet tilings for rapid exploration of spatially constrained many-body systems.

Anton Molina1,2, Shailabh Kumar2, Stefan Karpitschka2, Manu Prakash3.   

Abstract

Geometry in materials is a key concept which can determine material behavior in ordering, frustration, and fragmentation. More specifically, the behavior of interacting degrees of freedom subject to arbitrary geometric constraints has the potential to be used for engineering materials with exotic phase behavior. While advances in lithography have allowed for an experimental exploration of geometry on ordering that has no precedent in nature, many of these methods are low throughput or the underlying dynamics remain difficult to observe directly. Here, we introduce an experimental system that enables the study of interacting many-body dynamics by exploiting the physics of multidroplet evaporation subject to two-dimensional spatial constraints. We find that a high-energy initial state of this system settles into frustrated, metastable states with relaxation on two timescales. We understand this process using a minimal dynamical model that simulates the overdamped dynamics of motile droplets by identifying the force exerted on a given droplet as being proportional to the two-dimensional vapor gradients established by its neighbors. Finally, we demonstrate the flexibility of this platform by presenting experimental realizations of droplet-lattice systems representing different spin degrees of freedom and lattice geometries. Our platform enables a rapid and low-cost means to directly visualize dynamics associated with complex many-body systems interacting via long-range interactions. More generally, this platform opens up the rich design space between geometry and interactions for rapid exploration with minimal resources.

Entities:  

Keywords:  droplets; evaporation; geometric frustration; metastability; self-assembly

Year:  2021        PMID: 34417307      PMCID: PMC8403944          DOI: 10.1073/pnas.2020014118

Source DB:  PubMed          Journal:  Proc Natl Acad Sci U S A        ISSN: 0027-8424            Impact factor:   11.205


  25 in total

1.  Contact line deposits in an evaporating drop

Authors: 
Journal:  Phys Rev E Stat Phys Plasmas Fluids Relat Interdiscip Topics       Date:  2000-07

2.  Collective behavior of thermally active colloids.

Authors:  Ramin Golestanian
Journal:  Phys Rev Lett       Date:  2012-01-20       Impact factor: 9.161

3.  Breaking of ergodicity and long relaxation times in systems with long-range interactions.

Authors:  D Mukamel; S Ruffo; N Schreiber
Journal:  Phys Rev Lett       Date:  2005-12-09       Impact factor: 9.161

4.  Rapid prototyping of paper-based microfluidics with wax for low-cost, portable bioassay.

Authors:  Yao Lu; Weiwei Shi; Lei Jiang; Jianhua Qin; Bingcheng Lin
Journal:  Electrophoresis       Date:  2009-05       Impact factor: 3.535

5.  Potential energy landscapes for the 2D XY model: minima, transition states, and pathways.

Authors:  Dhagash Mehta; Ciaran Hughes; Mario Schröck; David J Wales
Journal:  J Chem Phys       Date:  2013-11-21       Impact factor: 3.488

6.  Direct observation of thermal relaxation in artificial spin ice.

Authors:  A Farhan; P M Derlet; A Kleibert; A Balan; R V Chopdekar; M Wyss; J Perron; A Scholl; F Nolting; L J Heyderman
Journal:  Phys Rev Lett       Date:  2013-08-02       Impact factor: 9.161

Review 7.  Additivity principles in biochemistry.

Authors:  K A Dill
Journal:  J Biol Chem       Date:  1997-01-10       Impact factor: 5.157

8.  Two-component marangoni-contracted droplets: friction and shape.

Authors:  Adrien Benusiglio; Nate J Cira; Manu Prakash
Journal:  Soft Matter       Date:  2018-09-26       Impact factor: 3.679

9.  Thermal fluctuations in artificial spin ice.

Authors:  Vassilios Kapaklis; Unnar B Arnalds; Alan Farhan; Rajesh V Chopdekar; Ana Balan; Andreas Scholl; Laura J Heyderman; Björgvin Hjörvarsson
Journal:  Nat Nanotechnol       Date:  2014-06-08       Impact factor: 39.213

10.  Predator-prey interactions between droplets driven by non-reciprocal oil exchange.

Authors:  Caleb H Meredith; Pepijn G Moerman; Jan Groenewold; Yu-Jen Chiu; Willem K Kegel; Alfons van Blaaderen; Lauren D Zarzar
Journal:  Nat Chem       Date:  2020-11-16       Impact factor: 24.427

View more
  1 in total

1.  How liquid-liquid phase separation induces active spreading.

Authors:  Youchuang Chao; Olinka Ramírez-Soto; Christian Bahr; Stefan Karpitschka
Journal:  Proc Natl Acad Sci U S A       Date:  2022-07-22       Impact factor: 12.779

  1 in total

北京卡尤迪生物科技股份有限公司 © 2022-2023.