Literature DB >> 34301938

Proximate ferromagnetic state in the Kitaev model material α-RuCl3.

H Suzuki1, H Liu2, J Bertinshaw3, K Ueda3,4, H Kim3,5,6, S Laha3, D Weber3,7, Z Yang3, L Wang3, H Takahashi3, K Fürsich3, M Minola3, B V Lotsch3,8, B J Kim3,5,6, H Yavaş9,10, M Daghofer11,12, J Chaloupka13,14, G Khaliullin3, H Gretarsson3,9, B Keimer15.   

Abstract

α-RuCl3 is a major candidate for the realization of the Kitaev quantum spin liquid, but its zigzag antiferromagnetic order at low temperatures indicates deviations from the Kitaev model. We have quantified the spin Hamiltonian of α-RuCl3 by a resonant inelastic x-ray scattering study at the Ru L3 absorption edge. In the paramagnetic state, the quasi-elastic intensity of magnetic excitations has a broad maximum around the zone center without any local maxima at the zigzag magnetic Bragg wavevectors. This finding implies that the zigzag order is fragile and readily destabilized by competing ferromagnetic correlations. The classical ground state of the experimentally determined Hamiltonian is actually ferromagnetic. The zigzag state is stabilized by quantum fluctuations, leaving ferromagnetism - along with the Kitaev spin liquid - as energetically proximate metastable states. The three closely competing states and their collective excitations hold the key to the theoretical understanding of the unusual properties of α-RuCl3 in magnetic fields.
© 2021. The Author(s).

Entities:  

Year:  2021        PMID: 34301938     DOI: 10.1038/s41467-021-24722-4

Source DB:  PubMed          Journal:  Nat Commun        ISSN: 2041-1723            Impact factor:   14.919


  31 in total

1.  Kitaev-Heisenberg model on a honeycomb lattice: possible exotic phases in iridium oxides A2IrO3.

Authors:  Jirí Chaloupka; George Jackeli; Giniyat Khaliullin
Journal:  Phys Rev Lett       Date:  2010-07-09       Impact factor: 9.161

2.  Mott insulators in the strong spin-orbit coupling limit: from Heisenberg to a quantum compass and Kitaev models.

Authors:  G Jackeli; G Khaliullin
Journal:  Phys Rev Lett       Date:  2009-01-06       Impact factor: 9.161

3.  Quantum spin liquids: a review.

Authors:  Lucile Savary; Leon Balents
Journal:  Rep Prog Phys       Date:  2016-11-08

Review 4.  Magnetism in two-dimensional van der Waals materials.

Authors:  Kenneth S Burch; David Mandrus; Je-Geun Park
Journal:  Nature       Date:  2018-10-31       Impact factor: 49.962

5.  Zigzag magnetic order in the iridium oxide Na2IrO3.

Authors:  Jiří Chaloupka; George Jackeli; Giniyat Khaliullin
Journal:  Phys Rev Lett       Date:  2013-02-28       Impact factor: 9.161

6.  Models and materials for generalized Kitaev magnetism.

Authors:  Stephen M Winter; Alexander A Tsirlin; Maria Daghofer; Jeroen van den Brink; Yogesh Singh; Philipp Gegenwart; Roser Valentí
Journal:  J Phys Condens Matter       Date:  2017-12-13       Impact factor: 2.333

7.  Magnetic Properties of Restacked 2D Spin 1/2 honeycomb RuCl3 Nanosheets.

Authors:  Daniel Weber; Leslie M Schoop; Viola Duppel; Judith M Lippmann; Jürgen Nuss; Bettina V Lotsch
Journal:  Nano Lett       Date:  2016-05-19       Impact factor: 11.189

8.  Spin liquids in frustrated magnets.

Authors:  Leon Balents
Journal:  Nature       Date:  2010-03-11       Impact factor: 49.962

9.  Generic spin model for the honeycomb iridates beyond the Kitaev limit.

Authors:  Jeffrey G Rau; Eric Kin-Ho Lee; Hae-Young Kee
Journal:  Phys Rev Lett       Date:  2014-02-20       Impact factor: 9.161

10.  Novel Jeff=1/2 Mott state induced by relativistic spin-orbit coupling in Sr2IrO4.

Authors:  B J Kim; Hosub Jin; S J Moon; J-Y Kim; B-G Park; C S Leem; Jaejun Yu; T W Noh; C Kim; S-J Oh; J-H Park; V Durairaj; G Cao; E Rotenberg
Journal:  Phys Rev Lett       Date:  2008-08-15       Impact factor: 9.161

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