Liqiang Qi1, Mengmeng Liu1, Xu Wang1, Jingxin Li1, Fang Zeng1. 1. Hebei Key Laboratory of Power Plant Flue Gas Multi-Pollutants Control, Department of Environmental Science and Engineering, North China Electric Power University-Baoding Campus, Baoding 071003, P. R. China.
Abstract
For particles that escape from electrostatic precipitators (ESPs), inertial recapture is used to improve the efficiency of dust removal. A rod-grid inertial separator was designed. The electrostatic and fluid flow particle tracking modules were selected in the model established by the COMSOL software, and the dust removal efficiency of the proposed dust separator was evaluated. When the flue gas velocity was 20 m·s-1, the diameter of the round rod was 8 mm, and the spacing of the pipes was 15 mm, the removal efficiency of PM2.5 and PM10 reached 27.8 and 84.6%, respectively. Experiments were performed under laboratory conditions and actual working conditions in a coal-fired power plant flue. Results showed that an inertial separator can achieve more than 60% efficiency in recapturing fly ashes that have escaped from ESPs. It can effectively remove fine particles and aerosol pollutants represented by PM2.5 and PM10.
For particles that escape from electrostatic precipitators (ESPs), inertial recapture is used to improve the efficiency of dust removal. A rod-grid inertial separator was designed. The electrostatic and fluid flow particle tracking modules were selected in the model established by the COMSOL software, and the dust removal efficiency of the proposed dust separator was evaluated. When the flue gas velocity was 20 m·s-1, the diameter of the round rod was 8 mm, and the spacing of the pipes was 15 mm, the removal efficiency of PM2.5 and PM10 reached 27.8 and 84.6%, respectively. Experiments were performed under laboratory conditions and actual working conditions in a coal-fired power plant flue. Results showed that an inertial separator can achieve more than 60% efficiency in recapturing fly ashes that have escaped from ESPs. It can effectively remove fine particles and aerosol pollutants represented by PM2.5 and PM10.
China’s environmental
protection standards are becoming
increasingly strict. The ultralow emission standard of coal-fired
power plants has reduced dust emission concentration to 10 mg/Nm.[1,3] Electrostatic precipitators (ESPs) have been widely applied as a
particle collection system for industrial fumes. The fine particle
removal characteristics of ESPs have been extensively evaluated and
analyzed.[2,3] Some strict guidelines and particle emission
standards have been implemented for controlling fine particle emissions
in recent years, especially in China. However, conventional dust removal
devices, such as ESPs, cannot meet the new standards.ESP technology
is currently widely used in power plants in China;
many cutting-edge technologies have been developed.[4] A low–low temperature (LLT) ESP system has better
particle capture efficiency than traditional ESPs.[5−7] Lower flue gas
temperature can increase the breakdown field strength and gas density
and reduce the specific resistance of fly ash and flow velocity. Electrostatic
agglomeration is one of the effective solutions to improve the collecting
efficiency of fine particles.[8] Agglomeration
can connect two or more particles and convert them into a larger particle,
which can be removed from the flue gas by conventional dust removal
technology.[9] Moreover, turbulent agglomeration
relies on fluid flow and interparticle collision to prompt the growth
and removal of fine particles,[10−12] and it is a convenient and economical
way owing to the simple structures, low cost, reliable operation,
and easy retrofitting and maintenance.Inertial separation of
dust escaped from ESPs is a worthwhile means.[13] In inertial adhesion, dust collection happens
when dust hits and adheres to the collecting surface,[14,15] and a dust layer is formed by adhering the dust particles to one
another under the collision of a high flow velocity and then impacting
the dust collector.For particles of a certain size, a critical
velocity exists beyond
which the particles will bounce back from the surface and not adhere.
This velocity depends on the elasticity of the particles and the surface
and is inversely proportional to the particle size. When airflow velocity
is high, large particles collide with a large elastic force and do
not easily adhere. However, a high airflow velocity is advantageous
for capturing fine particles. When particles bounce, the sedimentation
coefficient increases.[16]Dunbar[17] studied cascade impact samplers
and found that the main factor affecting the collection efficiency
of such samplers is particle rebound, which can be reduced by applying
a thin layer of grease on the impact plate. Demokritou[18] experimented with the use of polyurethane foam
impingement plates and found that even if the surface of the plates
is not coated with grease and other adhesive substances, particles
rarely rebound into the air stream.A related research indicates
that inertial adhesion is limited
to the application of a sampler and has yet to be studied as a dust
removal device. Research results reveal that a sampler cannot be used
as a dust collector directly in industrial dust removal. Therefore,
a dust removal technology based on inertial adhesion theory must be
developed.[19−21]Inertial separators are characterized by simple
designs, low investment
and operating costs, and a high reliability. The inertial particle
separator is widely used as an important gas–solid separation
device to protect the core engine in a severely polluted environment.[22−24] The separation efficiency of the IPS is not only affected by the
single geometrical or aerodynamic parameter but also apparently influenced
by the interaction effects between different parameters. In the inertial
separator, the trajectories of particles with small size are dominated
by the flow direction while the paths of particles with larger size
are dominated by the individual particle inertia and bounce characteristics
from the walls. In general, a high flow velocity is conducive to the
inertial separation of particles, while a slower flow velocity increases
the collection efficiency of ESPs. The inertial separator and ESPs
are connected in series, and high collection efficiency will be acquired
at low and high velocities. Thus, the topic of inertial separation
of particles from ESPs is new and can fill the knowledge gap on this
subject. This work focuses on particles that have escaped from the
tail of ESPs of thermal power plants. The objective is to find a new
solution to meet the national emission standards by capturing particles
through an inertial adhesion mechanism under a high flow rate condition
and to further reduce the dust emission concentration. Due to low
pressure drop and high efficiency, air cleaners based on ESPs have
also been widely applied to remove fine particles and improve indoor
and outdoor air quality.[25−27] Thus, this study can be used
to guide the removal of indoor and outdoor particles by joint electrostatic
inertial separators.
Results and Discussion
Computational Modeling Results
Simulated
Pressure Field
Figure shows the pressure
loss of the rod-grid inertial separator. The velocity is 15 m·s–1.
Figure 1
Flow diagram of internal pressure change of the rod-grid
inertial
separator.
Flow diagram of internal pressure change of the rod-grid
inertial
separator.The cloud diagram in Figure and the graph in Figure show that the pressure
drop from the inlet to outlet
is about 200 Pa, much lower than that of the particle filter. Moreover,
after the airflow passes through a row of impact rods, the pressure
is greatly reduced, and the pressure between the two rows of plates
is relatively stable. This result is attributed to the sudden contraction
and expansion that occur when the airflow passes the impact rods,
thus causing a sudden change in the velocity of the airflow. This
change in airflow velocity causes a change in pressure, which is the
impact after each row.
Figure 2
Pressure curve of the rod-grid inertial separator.
Pressure curve of the rod-grid inertial separator.
Simulated Velocity Field
The simulated
velocity field of the rod-grid inertial separator is shown in Figure .
Figure 3
Simulated velocity field
of the rod-grid inertial separator.
Simulated velocity field
of the rod-grid inertial separator.Figure illustrates
that when the circular rod is hit, the area of the fluid flow suddenly
shrinks and expands, increasing the flow velocity at the gap between
the round rods in each row of rods. On the side of the round pipe
facing the airflow, the gas velocity is low, that is, only ∼9
m·s–1. Meanwhile, the flow rate on the back
side of the rod is low, and eddy currents are generated. In a turbulent
flow field, fine particles collide and agglomerate with each other
under the influence of vortexes, which can improve the removal efficiency
of fine particles.
Changes in the Flow Field
The flow
field variation inside the rod-grid inertial separator is shown in Figure .
Figure 4
Flow field variation
inside the rod-grid inertial separator.
Flow field variation
inside the rod-grid inertial separator.Airflow impinges on the collecting round bar at a certain velocity.
The velocity of the airflow is higher around the round rod, which
is favorable for the inertial adhesion of dust. Then, the airflow
flows around the collecting round bar, exhibiting an acceleration
process. A low-speed vortex area is formed on the back convection
surface of the round bar, and some dust can also be collected, which
improves the dust removal efficiency.
Simulated
Dust Concentration Cloud Map
The concentration distribution
of dust in the rod-grid inertial
separator was simulated. The dust concentration at the inlet of the
device is 2200 mg/m3, the particle size is 10 μm,
and the velocity is 15 m·s–1.Figure shows that the concentration
of dust in the entire flow field is relatively uniform. On the upstream
surface of the trapping rod, dust concentration reaches the maximum
owing to the adhesion and trapping of dust.
Figure 5
Concentration distribution
of dust in the rod-grid inertial separator.
Concentration distribution
of dust in the rod-grid inertial separator.
Simulated Particle Trajectory Map
The
rod-grid inertial separator has a gas–solid two-phase
flow field. In addition to the distribution of the gas flow field,
the trajectory of the particle phase is also a research focus. Figure illustrates the
particle trajectories in the rod-grid inertial separator under different
velocities. Figure shows the trajectories of 2.5 and 10 μm particles in the rod-grid
inertial separator at 18 m/s velocity. The figure indicates that the
trajectory of the particle phase in the flow field away from the trapping
rod is relatively regular, that is, the flow field can be regarded
as being in a laminar flow state. Impact, flow, acceleration, and
deceleration occur in the vicinity of the trapping rod, and some eddy
currents appear. Small-scale vortexes were more conducive to the removal
of fine particles.
Figure 6
Particle trajectories in the rod-grid inertial separator
under
different velocities: (a) 15 m/s and (b) 18 m/s.
Figure 7
Trajectories
of (a) 2.5 and (b) 10 μm particles at 18 m/s.
Particle trajectories in the rod-grid inertial separator
under
different velocities: (a) 15 m/s and (b) 18 m/s.Trajectories
of (a) 2.5 and (b) 10 μm particles at 18 m/s.In the case of different velocities, the particle trajectory
does
not change significantly and only affects the internal turbulence.
Simulated Dust Removal Efficiency
Evaluating the removal efficiency of particles in flue gas is important
for engineering practice.Figure presents the simulation results for the collection
efficiencies of particles with diameters of 0.1, 0.5, 1, 2.5, 5, and
10 μm at flow velocities of 10–20 m·s–1. The collection efficiency increased with the increase of flow velocity
and particle size. The particle trajectories with small particle size,
because of the relatively smaller inertia, are dominated by the flow
direction, while paths with larger particle size are dominated by
the individual particle inertia and bounce characteristics from the
rods. The inertial forces acting on particles are larger with higher
velocities. When the particles flow around the rod, large inertial
forces make it more difficult for the particles to change their direction
of motion.
Figure 8
Simulated collection efficiencies of the inertial separator according
to flow velocity.
Simulated collection efficiencies of the inertial separator according
to flow velocity.Figures and 10 show the collection
efficiencies of particles
with round rod diameters of 3, 5, and 8 mm, and rod distances of 10,
15, and 20 mm. When the particle size was larger than 2.5 μm,
the collection efficiency of the inertial separator increased as the
rod diameter increased (Figure ). Because large particles have larger inertial forces and
the blocking area increases with the increase of rod diameter, the
probability of particle capture increases accordingly. Small particles
have a relatively smaller inertia, and it is easier to get around
the rod with the flow. For all particle sizes, the collection efficiency
decreased with the increase of rod distance (Figure ). Combination of the electrostatic precipitator
and inertial separator is more effective for collecting large particles
than turbulent agglomeration. The collection efficiency of PM2.5 and
PM10 can reach 27.8 and 84.6%, respectively. For PM2.5, the capture
efficiency of 27.8% combined with the fractional PM removal efficiency
of the WFGD after ESP will meet the ultralow emission standard.
Figure 9
Simulated collection
efficiencies of the inertial separator with
different rod diameters.
Figure 10
Simulated collection
efficiencies of the inertial separator with
different rod distances.
Simulated collection
efficiencies of the inertial separator with
different rod diameters.Simulated collection
efficiencies of the inertial separator with
different rod distances.A slower flow velocity
can increase the collection efficiency of
ESPs, while a faster flow velocity can increase the collection efficiency
of inertial dust separators. When these types of dust collectors are
connected in series, a high collection efficiency can be expected
at both low and high velocities. Moreover, both the precharge of the
ESP and the turbulence of the inertial separator can improve the collection
efficiency of particles.
Laboratory Experiments
According
to the simulation results, rods with a diameter of 8 mm and a distance
of 10 mm were selected in the laboratory experiment.Table indicates that, for
10 g of ash fed at different gas velocities for 60 min, the amount
of ash collected by the trap increases with increasing velocity. The
total removal efficiency of the experimental and simulation results
matches well under all flow velocity conditions, but its value found
in the experiment is lower than the simulation predictions. One reason
is that a large amount of ash samples is present at the bottom of
the pipeline because this area is small, the distance from the feed
port to the trap gate is short, and the airflow velocity is low. Thus,
the ash sample cannot be completely suspended after it comes down
from the feed port and a large part falls at the bottom of the pipe.
Moreover, because the feed port is too close to the trap, the ash
sample coming down from the feed port is not evenly dispersed in the
gas stream.
Table 1
Efficiency of Dust Collection at Different
Gas Velocities
wind speed (m/s)
10
12
15
18
dust
collection (g)
1.604
2.356
2.842
3.648
collection efficiency (%)
16.04
23.56
28.42
36.48
standard deviation (%)
1.10
1.42
0.99
1.26
With the 18 m·s–1 gas velocity, the change
of ash collection on the round rod with time (10, 20, 30, and 60 min)
is observed. The ash samples from the surfaces are weighed. The results
are shown in Table .
Table 2
Amount of Dust Collected over Time
time (min)
10
20
30
60
rod (Φ = 5 mm)
0.793
1.886
2.662
2.726
rod (Φ = 8 mm)
1.321
2.609
3.586
3.648
standard deviation (%)
1.15
1.20
1.01
1.05
According to the amount of dust collected,
as dust collection time
increases, the dust collected from the round pipe also increases but
the flow area of the round pipe remains constant. Moreover, the amount
of dust carried by the round pipe has a maximum value, which is impossible
to increase without limit.When the stainless steel rod is placed
in the flue for 10 min,
a thin layer of dust adheres to the surface of the rod, which is evenly
distributed along the surface of the pipe facing the airflow. The
dust that adheres on the rod for 20 min increases compared to that
on the rod for 10 min, and the dust collected in the middle portion
of the round rod facing the airflow surface increases. After adherence
for 30 min, the dust on the round rod increases further and the accumulated
dust forms a cone shape. After standing for 60 min, the dust collected
by the round rod continues to increase further but only slightly.
Therefore, after 30 min of dust collection, the dust collected on
the round pipe is near the maximum load of the round pipe. Increasing
the dust collection time does not improve dust collection greatly.
Field Experiments
Field tests are
conducted in a thermal power plant in North China.The dust
concentration of flue gas from the outlet of ESP is 56.8 mg/Nm3, flue gas moisture content is 4.5%, flue gas flow velocity
is 20.4 m·s–1, flue gas temperature is ∼145
°C, and SO2 concentration is 1.02%. The pipeline negative
pressure is −2670 Pa.The rod-grid inertial separator
was placed in the flue behind the
outlet of ESP. The image of the rod after particle collection for
30 min is shown in Figure .
Figure 11
Image of the rod after dust collection for 30 min.
Image of the rod after dust collection for 30 min.After 30 min, the dust concentration at the outlet of flue
was
21.3 mg/m3. Thus, the collection efficiency of the rod-grid
inertial separator can reach 62.5%. It is an effective way to reduce
particulate emissions and does not require a major overhaul.
Conclusions
A rod-grid inertial separator after ESPs
was designed. An analysis
of pressure change in the rod-grid inertial separator indicates that
the change in flow velocity, trajectory of the dust particles, and
some rules about the operation of the rod-grid inertial separator
have been obtained. The dust removal efficiency of the proposed dust
separator was evaluated. When the flue gas velocity was 20 m·s–1, the diameter of the round rod was 8 mm, and the
spacing of the pipes was 15 mm, the removal efficiency of PM2.5 and
PM10 reached 27.8 and 84.6%, respectively. Experiments were performed
under laboratory conditions and field working conditions in a coal-fired
power plant flue. The law of experimental and simulation results matched
well under all flow velocity conditions. Field experiments showed
that the inertial separator can achieve 62.5% efficiency in recapturing
fly ashes that have escaped from ESPs. Inertial separation of particles
escaped from ESPs is a new solution to meet national emission standards
and to reduce the dust emission concentration.
Materials
and Methods
Experimental Setup and Instrumentation
Experimental System
A schematic
diagram of the flue retrofit used in the laboratory is shown in Figure . The diameter
of the flue in the laboratory is 400 mm, and the flow rate of the
regulated airflow can only reach ∼8 m·s–1, which is extremely low. Therefore, another small tube is designed,
fabricated, and installed. This tube is connected to the small rectangular
observation hole on the side of the dust removal tube and blocks the
inlet of this tube. Owing to the reduced airflow area, the gas flow
rate in the small tube can be increased up to 18 m·s–1.
Figure 12
Diagram of the flue retrofit used in the laboratory: ①,
flange; ②, trapping grate segment; ③, side wall openings;
④, open pore; and ⑤, hopper.
Diagram of the flue retrofit used in the laboratory: ①,
flange; ②, trapping grate segment; ③, side wall openings;
④, open pore; and ⑤, hopper.After the test rig is connected to the dust removal tube, the collecting
rod is arranged in the trapping grid section. There are two rows of
collecting rods interlaced in the direction of vertical airflow (Figure , top view).
Figure 13
Arrangement
of the collecting rods in the trapping grid section: w, the width of the trapping grid section; L, the
length of the trapping grid section; b, distance
between collecting rods; and d, rod diameter.
Arrangement
of the collecting rods in the trapping grid section: w, the width of the trapping grid section; L, the
length of the trapping grid section; b, distance
between collecting rods; and d, rod diameter.
Laboratory Experiments
The dust
removal efficiency of the precipitator is tested in the laboratory.The angle of the wind deflector is adjusted to change the gas velocity,
which is measured with a hot-ball anemometer. Experimental gas velocities
of 10, 12, 15, and 18 m·s–1 for 10 g of ash
fed into the flue in front of the inertial separator by the automatic
feeder are recorded. The experiment lasts for 30 min, and the amount
of ash collected on the surface of the rod is weighed.Fly ashes
have been obtained from the dust hopper of ESP in the
Tuoketuo Power Plant, China. A YFJ Bahco centrifuge (Chengde Instrument
and Meter Factory) was used to measure the size distributions of fly
ashes. The dispersity of fly ash is shown in Figure .
Figure 14
Dispersity of the fly ash.
Dispersity of the fly ash.The collection efficiencies have been calculated as followswhere Mpassed is
the mass concentration of particles leaving the inertial separator
through the outlet, Mtrapped is the mass
concentration of particles trapped by rods, and Mtotal is the mass concentration of particles fed at the
inlet. An isokinetic sampling method was used for the measurement
of the mass concentration of particles.
Test
under Real Conditions
Field
tests were performed in a power plant.Boilers (410 tons) of
50 MW capacity were running in the thermal power plant in North China.
The dust concentration of flue gas is 216 mg/Nm3, dust
collector efficiency is 99.54%, flue gas moisture content is 4.5%,
flue gas flow rate is 15.4 m·s–1, flue gas
temperature is ∼145 °C, and SO2 concentration
is 1.02%. The pipeline negative pressure is −2670 Pa.In the field experiment of power plant A#5, sample devices are
inserted into the holes at the side of the downstream flue and left
for 10, 20, 30, and 60 min. The ash on the round rod is observed.
In the field test, owing to the high flow rate in the flue gas pipeline
and the lower pressure in the flue in comparison with the atmospheric
pressure, measures must be taken to prevent air from leaking out from
the measuring hole. Such measures, which include washing the stainless
steel pipe, affect the dust collection efficiency.The dust
collected from the stainless steel rods is brought back
to the laboratory for weighing.Total mass concentrations of
particles at the entrance and exit
of the ESP were simultaneously measured, and an isochronic sampling
method was used for the particulate matter sample (Methods of Performance
Tests for Electrostatic Precipitators, GB/T13931-2002 of China).
Simulation Approach and Numeric Computation
Theoretical Model
Given that the
diameter of the particles used for calculations is larger than the
average free path of gas molecules, the particles must not be treated
as “quasifluid”. In the present study, the influence
of the electric field on the flow field is usually neglected in the
numerical simulation. The airflow through the ESP channel is modeled
as steady and turbulent while assuming constant density and viscosity.[28] Therefore, the discrete phase model (DPM) (i.e.,
Euler–Lagrange model) is adopted to simulate particle flow
in the transverse-plate ESP.In calculating the single-phase
flow field, the gas is assumed to be complete, with a constant specific
heat coefficient that ignores mass force and viscosity.Gas-phase control
equation: For the
3-D compressible two-phase flow field of the transverse-plate ESP,
the general form of the conservation equations of the gas phase in
the Euler coordinate system iswhere u is the gas
velocity, ν is the velocity of the particle,
ϕ is any
independent variable, Γϕ is the transport coefficient, Sϕ is the gas source term, and S is the source term
for the interaction of gas and particles.Particle-phase control equation: The
equation of the particle phase in the Lagrangian coordinate system
iswhere A is the cross-sectional
area of the channel and υ is the
particle flow rate perpendicular to the component of the flow rod
cross section.When only the fluid resistance
and gravity of the particles are
considered and other forces and mass loss rates are ignored, the momentum
equation of the particle phase in the i direction
iswhere
τ is the particle relaxation time
and g is the gravitational
acceleration.
Flow Field Performance
The COMSOL5.4
software was used in this study to measure and calculate the electrostatic
and flow field models of 3-D gas–solid two-phase flow of a
rod-grid inertial separator. The collecting rods are round with diameters
of 3, 5, and 8 mm, and the distances between the rods are set as 10,
15, and 20 mm, respectively. The gas velocity is controlled at 10,
12, 15, 18, and 20 m·s–1, and the gas velocity
data curve is plotted.In this study, the discrete phase model
(DPM) is used to simulate the two-phase flow field of a rod-grid inertial
separator. The mesh division is shown in Figure .
Figure 15
Mesh division of the rod-grid inertial separator.
Mesh division of the rod-grid inertial separator.Initial conditions and boundary conditions: operating
pressure:
101 325 Pa; entrance conditions: V = 15 m·s–1 (the tail flue gas velocity after the outlet of the
ESP); and wall condition: fixed heat flow is 0, no slip wall surface
is used, pressure is extrapolated from the value in the flow field,
and the velocity of particles near the wall is 0, that is, the dust
reaches the plate and is completely collected.
Evaluation of Dust Removal Efficiency
The rod-grid
inertial separator is designed to remove the particles
in the flue gas at the end of ESPs of the coal-fired power plant to
realize deep purification of the flue gas.The electrostatic
and fluid flow particle tracking modules are selected in the model
established by the COMSOL software. The particles flow with the flow
field, and the particle diameter, density, stress (gravity, drag,
and electric field), and charging characteristics are set (hypothesis
for the saturation charge). The internal wall surface characteristics
of the dust collector are also set.The number and frequency
of particle placement are also set. One
thousand particles are delivered once every 0.01 s with a delivery
time of 1 s. The gas velocity at the inlet of the precipitator is
set, and the internal flow field of the precipitator is calculated.
Finally, the dust removal efficiency of the precipitator can be obtained
according to the number of frozen particles on the flue gas outlet
surface of the precipitator combined with the number of particles
placed in the flue gas inlet.