Literature DB >> 33889817

Comparison of applied torque and energy conversion efficiency between rotational triboelectric nanogenerator and electromagnetic generator.

Shaohang Xu1,2, Xianpeng Fu1,2, Guoxu Liu1,2, Tong Tong1,2, Tianzhao Bu1,2, Zhong Lin Wang1,2,3, Chi Zhang1,2,4.   

Abstract

Triboelectric nanogenerator (TENG) is regarded as an equally important mechanical energy harvesting technology as electromagnetic generator (EMG). Here, the input mechanical torques and energy conversion efficiencies of the rotating EMG and TENG are systematically measured, respectively. At constant rotation rates, the input mechanical torque of EMG is balanced by the friction resisting torque and electromagnetic resisting torque, which increases with the increasing rotation rate due to Ampere force. While the input mechanical torque of TENG is balanced by the friction resisting torque and electrostatic resisting torque, which is nearly constant at different rotation rates. The energy conversion efficiency of EMG increases with the increasing input mechanical power, while that of the TENG remains nearly constant. Compared with the EMG, the TENG has a higher conversion efficiency at a low input mechanical power, which demonstrates a remarkable merit of the TENG for efficiently harvesting weak ambient mechanical energy.
© 2021 The Author(s).

Entities:  

Keywords:  Electromagnetic Field; Energy Resources; Energy Systems; Nanostructure

Year:  2021        PMID: 33889817      PMCID: PMC8050373          DOI: 10.1016/j.isci.2021.102318

Source DB:  PubMed          Journal:  iScience        ISSN: 2589-0042


Introduction

With the rapid development of the Internet of Things (Borgia, 2014; Roman et al., 2013), sustainable and long-life energy supply for billions of distributed electronics has become a major issue(Chu and Majumdar, 2012; Gielen et al., 2016). Compared with the traditional energy supply by using chemical battery, energy harvesting technology is a more effective way by converting ambient mechanical energy into electric power (Gao et al., 2020; Guo et al., 2016; Shao et al., 2018b; Xie et al., 2014; Xu et al., 2019). Nowadays, triboelectric nanogenerator (TENG) has attracted growing attention due to its simple structure(Wang et al., 2014; Ye et al., 2019; Zhang et al., 2019a, 2019b), high power density, low cost, high flexibility (Liu et al., 2020; Wang et al., 2020a), and abundant selection of materials (Li et al., 2020; Wang et al., 2020b; Yan et al., 2020; Zheng et al., 2020). Derived from the second term in Maxwell's displacement current (Akande and Lowell, 1985; Wang, 2017), the TENG has been widely used in micro/nanopower sources (Seung et al., 2015; Tayyab et al., 2020; Xiong et al., 2019), self-powered sensing (Jin et al., 2017; Khan et al., 2017; Wu et al., 2016), blue energy (Shao et al., 2018a; Wang et al., 2016), and high voltage sources (Bui et al., 2019; Li et al., 2017; Xia et al., 2019) since its first invention in 2012 (Fan et al., 2012). As a new energy technology, the TENG has an equally vital role in harvesting mechanical energy compare to the traditional electromagnetic generator (EMG). The TENG has demonstrated to be comparable and symmetrical with EMG in working mechanisms, governing equations, and output characteristics (Zhang et al., 2014), which has demonstrated that the TENG could be equivalently important as the EMG for harvesting mechanical energy. Moreover, the reports have demonstrated that the TENG has a better output performance than EMG at low frequency (Zi et al., 2016) and small amplitude (Zhao et al., 2019), which indicates a great advantages and possible killer applications of TENG in micromechanical energy harvesting and sensing. However, the applied force/torque and energy conversion efficiency of both generators have not systematically studied and compared yet, which are directly influenced by their different damping characteristics. So, it is extremely important to reveal the characteristics of applied force/torque for both generators and investigate the energy conversion efficiency dependence on input mechanical power. Here in this work, the input mechanical torque of the rotating EMG and TENG are systematically measured, respectively. At constant rotation rates, the input mechanical torque of EMG is balanced by the friction resisting torque and electromagnetic resisting torque, which increases with the increasing rotation rate due to Ampere force. While the input mechanical torque of TENG is balanced by the friction resisting torque and electrostatic resisting torque, which is nearly constant at different rotation rates. The energy conversion efficiencies of both generators are also quantified and compared. With the increase of the input mechanical power, the energy conversion efficiency of EMG is increasing, while that of the TENG remains nearly constant. The comparison results and demonstrations have shown that the TENG has a higher conversion efficiency than that of the EMG at a low input mechanical power. This work has demonstrated a remarkable merit of the TENG under a gentle-triggering, which has verified the possible applications for efficiently harvesting weak mechanical energy from human body and ambient environment.

Results

Figure 1 illustrates the schematic diagrams and working principles of the rotational EMG and TENG. Both EMG and TENG contain a rotator and a stator, which are based on the circular acrylic sheets with the same diameter of 280 mm and nine fixed power generation units, as shown in Figure 1A. For the EMG, the magnets and copper coils are embedded in the rotator and stator along the direction of circumference, respectively, as shown in Figure 1A (I). The magnetic poles of the magnet are in the same direction, while the winding direction of the copper coils are all counter clockwise, and the copper coils are connected in parallel. For the TENG, the fan-shaped fluorinated ethylene propylene (FEP) triboelectric layers are adhered to the rotator, while the corresponding fan-shaped copper electrodes are fabricated in the stator as the freestanding mode, which is shown in Figure 1A (II). The detailed fabrication processes of the two generators are described in the Experimental section.
Figure 1

Schematic illustrations and working principles of both fabricated generators

3D schematic diagram and photos of fabricated (A) EMG and TENG. Working principles of (B) EMG and (C) TENG.

Schematic illustrations and working principles of both fabricated generators 3D schematic diagram and photos of fabricated (A) EMG and TENG. Working principles of (B) EMG and (C) TENG. Figure 1B illustrates the working principle of the EMG based on the electromagnetic induction. At the initial state, as shown in Figure 1B (I), the magnets and copper coils are fully aligned. The magnetic flux through the copper coils achieves maximum value. When the magnets rotate away from the copper coils, the magnetic flux through the coil can be changed, which induces an electrodynamic potential and current in the coil, in the state II. The magnetic flux reduces to minimum when the magnets rotate to the final state III. The rotator part rotates continuously to the next initial state that can induce the current flow in the reversed direction. Thus, an alternating current (AC) can be generated for the periodically rotate of these magnets. By coupling of the contact electrification and the relative-sliding-induced charge transfer, the working principle of the freestanding mode TENG is shown in Figure 1C. To generate the equal negative and positive charges on the FEP and copper electrode, the two triboelectric layers are pre-contacted for electrification and then separate in a certain distance. In the process of relative rotation, the small gap is kept between the two triboelectric layers to eliminate the influence of friction. At the original state, the FEP layer is aligned with the left copper electrode. At this state, the TENG is in the electrostatic equilibrium state and no electron flows through the external circuit, as shown in Figure 1C (I). As shown in Figure 1C (II), when the FEP layer rotates under the excitation of input torque, the aligned area between FEP and left electrode is reduced. The produced potential difference will drive electrons to flow from the right to the left electrode. This electricity generation process will last until the FEP rotates to the position where the FEP is aligned with the right copper electrode, as shown in Figure 1C (III). In the following, the aligned area between FEP and left electrode starts to increase, which creates a reverse current. Electrons flow back and forth between the two copper electrodes, generating an AC signal. For the EMG, according to the Faraday's law, the open-circuit voltage and short-circuit current can be presented as:Where N1 is the number of the coil-magnet pairs and Ф is the total magnetic flux in each coil, r represents the internal resistance of the coil. Apparently, the rate of the magnetic flux variate is related to the rotation rate. Figures 2A and 2C shows the variety of open-circuit voltage and short-circuit current of the EMG at the rotation rate 200 r/min, the open-circuit voltage has the peak to peak values of 16.61V while the short-circuit current has the peak values of 71.48 mA. Considering the Equations (1) and (2), the peak to peak values of open-circuit voltage and the peak values of short-circuit current both increase proportionally with the increases of the rotation rate. The experimental results are given in the illustration of Figures 2A and 2C, respectively, which accord with the theoretical equations. The peak to peak values of open-circuit voltage increases from 0.86 V to 16.61 V, while the peak values of short-circuit current increase from 7.98 mA to 71.48 mA with the rotation rate increases from 10 r/min to 200 r/min.
Figure 2

The electric output performance comparison of the EMG and TENG

The open-circuit voltages of (A) EMG and (B) TENG with nine power generation units under a rotation rate of 200 r/min, the illustration is the peak to peak values open-circuit voltage of the EMG and TENG with increasing rotation rate from 10 r/min to 200 r/min respectively. The short-circuit currents of (C) EMG and (D) TENG with nine power generation units under a rotation rate of 200 r/min, the illustration is the peak values short-circuit current of the EMG and TENG with increasing rotation rate from 10 r/min to 200 r/min respectively. Impedance matchings of (E) EMG and (F) TENG with nine power generation units and increasing rotation rate from 10 r/min to 200 r/min. The maximum average output powers of (G) EMG and (H) TENG with different number of power generation units and rotation rates.

The electric output performance comparison of the EMG and TENG The open-circuit voltages of (A) EMG and (B) TENG with nine power generation units under a rotation rate of 200 r/min, the illustration is the peak to peak values open-circuit voltage of the EMG and TENG with increasing rotation rate from 10 r/min to 200 r/min respectively. The short-circuit currents of (C) EMG and (D) TENG with nine power generation units under a rotation rate of 200 r/min, the illustration is the peak values short-circuit current of the EMG and TENG with increasing rotation rate from 10 r/min to 200 r/min respectively. Impedance matchings of (E) EMG and (F) TENG with nine power generation units and increasing rotation rate from 10 r/min to 200 r/min. The maximum average output powers of (G) EMG and (H) TENG with different number of power generation units and rotation rates. For the TENG, according to the previous works, the open-circuit voltage and short-circuit current can be described as:where σ is the charge density on the FEP surface, S is the area of one electrode, C is the capacitance between the two electrodes, N2 is the number of segments of the electrode, ω is the rotational angular velocity (, where n is the rotation rate). Figures 2B and 2D shows the variety of open-circuit voltage and short-circuit current of the TENG at the rotation rate 200 r/min, the peak to peak values of open-circuit voltage can achieve 1064 V, and the peak values of short-circuit current can achieve 79.01 μA. Considering the Equations (3) and (4), with increasing the rotation rate, the peak values of short-circuit current can increases proportionally while the peak to peak values of open-circuit voltage can almost keep unchanged. As shown in the illustration of Figures 2B and 2D, when the rotation rate increases from 10 r/min to 200 r/min, the peak values of short-circuit current increases from 5.73 μA to 79.01 μA, while the peak values of open-circuit voltage remains almost stable around 1070 V. For the EMG, the average output power versus external load can be calculated as:where U is the voltage of the external load, R is the external resistance, t is the integral period. Under the different rotation rate, the average output power of the EMG first increased, and then decreased with increasing the external resistance, the maximum average output power always appears at the external resistance of 110 Ω regardless the rotation rate, which is shown in Figure 2E. Moreover, the average output power of the EMG with different number of power generation units at different rotation rate is shown in Figure S1. And the variety of the maximum average output powers of the EMG with rotation rate at different number of power generation units are summarized in Figure 2G, which are all nearly proportional to the square of the rotation rate. For the TENG, the average output power versus external load can be calculated as:where R is the external resistance, I is the current flowing through the external load, t is the integral period. With increase the external resistance, the variation trend of average output power of the TENG is similar to the EMG. However, the maximum average output power appears at the low external resistance when the rotation rate is high, while the maximum average output power appears at high external resistance when the rotation rate is low, with the increases of the rotation rate from 10 r/min to 200 r/min, the external resistance corresponding to the maximum average output power decreases from 80 MΩ to 5 MΩ, which is shown in Figure 2F. Furthermore, the average output power of the TENG with different number of power generation units at different rotation rate is shown in Figure S1. The variety of the maximum average output powers of the TENG with rotation rate at different number of power generation units are summarized in Figure 2H, which are all nearly proportional to the rotation rate. As shown in Figure 3A, the input mechanical torque needs to overcome the resisting torques for driving the rotator of the both generators to rotate during the operation. When the rotator rotates with a constant rotation rate, the torques are in equilibrium and can be described as:where T is the input mechanical torque, T is the field-induced resisting torque, and T is the friction resisting torque from mechanical bearing.
Figure 3

The input mechanical performance comparison of the EMG and TENG

The resisting force and torque analysis of the (A) EMG and TENG. The measured torque of (B) EMG and (C) TENG with different rotation rate. Average field-induced resisting torque of (D) EMG and (E) TENG with different rotation rate.

The input mechanical performance comparison of the EMG and TENG The resisting force and torque analysis of the (A) EMG and TENG. The measured torque of (B) EMG and (C) TENG with different rotation rate. Average field-induced resisting torque of (D) EMG and (E) TENG with different rotation rate. For the EMG, the field-induced resisting torque is the electromagnetic resisting torque which is caused by the ampere's force, as shown in Figure 3A (I). During the rotation, the induced current in the coils will generate an opposite ampere's force with rotating direction for hindering the rotator rotating. Therefore, the average electromagnetic resisting torque can be calculated as:where is the average ampere's force and is the equivalent arm of the Ampere's force. For the TENG, the field-induced resisting torque is the electrostatic resisting torque which is caused by the electrostatic force, as shown in Figure 3A (II). During the rotation, the static charge at the triboelectric films will generate an opposite electrostatic force with rotating direction for hindering the rotator rotating. Therefore, the average electrostatic resisting torque can be calculated as:where is the electrostatic force and is the equivalent arm of the electrostatic force. As shown in Figure S2, the input mechanical torque of the both generators can be measured by the torque sensor. Firstly, the input mechanical torques are measured at different rotation rates without field-induced resistances (T = 0). In these states, the friction resisting torque from mechanical bearing T can be acquired which is just counteracting the measured input mechanical torque T, as shown with black curves in Figures 3B and 3C. And then, the input mechanical torques T are measured with field-induced resistances, in the maximum average output power point at different rotation rates, as shown with color curves in Figures 3B and 3C. In addition, the input mechanical torques and friction resisting torque of both generators with different number of power generation units is shown in Figure S3. For both generators, the acquired friction resisting torque is fluctuating at each rotation rate, but the average value nearly keeps a constant with the increasing of rotation rate. The measured input mechanical torques are also fluctuating. For the EMG, the average value increases with the increasing of rotation rate. It is because that the increasing of rotation rate leads to the increase of induced current and ampere's force. Therefore, the electromagnetic resisting torque increases with the increasing of the rotation rate. While for the TENG, the average value nearly keeps constant with the increasing of rotating rate. It is because that the total amount of tribo-induced electrostatic charges is constant. Therefore, the electrostatic force and resisting torque is not influenced by the rotation rate. According to Equation (7), the field-induced resisting torque T can be calculated. Figures 3D and 3E summarize the acquired average electromagnetic and electrostatic resisting torques of the EMG and TENG with different number of power generation units versus the rotation rate, respectively. For the EMG, the average electromagnetic resisting torque increases with the increasing rotation rate for each different number of power generation units. Different from the EMG, the average electrostatic resisting torque of the TENG nearly keeps constant with the increasing rotation rate and linearly increases with the unit number, which is shown in the inset of Figure 3E. The average input mechanical power of the both generators can be described as:where is the average electromagnetic or electrostatic resisting torque of the both generators and ω is the rotating angular velocity. As shown in Figure 4A, the average input mechanical power of the EMG is nearly proportional to the square of the rotation rate for each different number of power generation units. While the average input power of the TENG is nearly proportional to the rotation rate for each different number of power generation units, as shown in Figure 4B.
Figure 4

The input power and efficiency comparison of the EMG and TENG

Average input power of (A) EMG and (B) TENG with different rotation rates. Max average output power (C) and energy conversion efficiency (D) comparison of EMG and TENG with different average input power. Dominant scope of TENG in average input power with different number of units (E).

The input power and efficiency comparison of the EMG and TENG Average input power of (A) EMG and (B) TENG with different rotation rates. Max average output power (C) and energy conversion efficiency (D) comparison of EMG and TENG with different average input power. Dominant scope of TENG in average input power with different number of units (E). The electrical energy conversion efficiency can be expressed as: Maximum average output power of the EMG and TENG with nine power generation units respectively at the different average input power is indicated in Figure 4C. With the increasing of the average input power, the maximum average output power of the EMG and TENG are both increase, but when the average input power is low, the maximum average output power of the TENG is high than that of the EMG, when the average input power exceeds 11.4 mW, the maximum average output power of the EMG will surpass that of the TENG. Each electrical energy conversion efficiency variation of the both generators versus average input mechanical powers are also shown in Figure 4D. With the increasing of the average input power from 1.05 mW to 18.61 mW, the electrical energy conversion efficiency of EMG rapidly grows and has a tendency to gradually become saturated. While the electrical energy conversion efficiency of the TENG nearly keeps unchanged but decrease slightly, crossing with the curve of EMG at average input power of 11.4 mW. The results indicate that the TENG is superior to the EMG with remarkable merits for harvesting mechanical energy in low input power (<11.4 mW). For the EMG, the reason for the efficiency characteristic curve which rapidly grows first and then remains virtually constant is that impact by the eddy current loss, copper loss, and other loss. When the average input power is low, the average output power is correspondingly low, the losses occupies a large proportion, which have a greater affection on average output power, and result in the low electrical energy conversion efficiency. With the increasing of the average input power, the average output power increases rapidly, the proportion of losses become lower, and the impact of losses on average output power would reduce and further increase the electrical energy conversion efficiency. For the TENG, the ideal conversion efficiency can keep constant with the increasing of the average input power; this is because the conversion efficiency of TENG is only related to electrostatic torque which can keep unchanged under different rotation rate. In fact, the conversion efficiency of TENG slightly decreases with the increasing of the average input power. It is because that the slight mechanical vibration will cause the energy loss when the average input power is high. The maximum average output power and electrical energy conversion efficiency of the both generators versus average input power at each different number of power generation units are shown in Figure S4, which all have similar variation tendency. For the eight, seven and six power generation units of both generators, the electrical energy conversion efficiency of EMG increases to the same value as that of the TENG when the average input power increases to 15.2 mW, 19 mW and 21.7 mW, respectively. The average input power at the intersection of electrical conversion efficiency increases with the decreasing unit number, as summarized in Figure 4E. The results show that the fewer the number of power generation units for both generators, the larger dominant power range for the TENG. As the applied torque of the TENG is proportional to the unit number, the results also demonstrate the remarkable merit of TENG in weak input force/torque. We have designed and demonstrated the merit of the TENG for harvesting weak mechanical energy with low input power, as shown in Figure 5A. The EMG and TENG work at the same input mechanical energy which is decided by the gravitational potential energy of the mass and can be tuned by changing the pre-input angle of the mass. An angle sensor is attached to the mass which is used to locate the pre-input angle of the mass and monitor the angle change in real time. The total working time under the same input energy of the both generators are also can achieve. Among them, both EMG and TENG with nine power generation units.
Figure 5

Demonstration for weak mechanical harvesting energy, which EMG and TENG with nine power generation units, respectively

Schematic of the EMG or TENG (A). The variety of swing angle of EMG (B) and TENG (C) at pre-input angle of 140 deg. Swing time of the EMG and TENG versus pre-input angle (D). Output energy of an LED driven by the EMG and TENG versus pre-input angle (E).

Demonstration for weak mechanical harvesting energy, which EMG and TENG with nine power generation units, respectively Schematic of the EMG or TENG (A). The variety of swing angle of EMG (B) and TENG (C) at pre-input angle of 140 deg. Swing time of the EMG and TENG versus pre-input angle (D). Output energy of an LED driven by the EMG and TENG versus pre-input angle (E). The oscillation curve of the swing angle for the EMG and TENG under pre-input angle 140 deg is shown in Figures 5B and 5C. The swing time of the EMG is 46 s while the TENG is 342 s. The oscillation curve of the swing angle for the EMG and TENG under pre-input angle 90 and 115 deg is shown in Figure S5. Changing the pre-input angle of the mass, the swing times of EMG and TENG also changes, which are summarized as shown in Figure 5D. The huge difference in the swing time between the both generators indicates that the TENG has much lower damping than the EMG. Figure 5E shows the output energy of the EMG and TENG across the LED with different pre-input angle, which can be calculated as:where t is the swing time, U and I is the voltage and current across the LED applied by the both generators, respectively. The output energy of the TENG across the LED rise slowly, while the EMG rise slowly and then rapidly rise, exceed TENG after 140°. The variation of the U and I at different pre-input angle are shown in Figures S6–S8. The visual demonstration is shown in Videos S1 and S2. The on/off state of the LED is determined by the input mechanical energy, which is tuned by changing the pre-input angle. When the pre-input angle exceeds 50 deg, the TENG can light up the LED, while the EMG cannot light up until the pre-input angle exceeds 90 deg. As the pre-input angle increases, the brightness of the LED lighted by TENG and EMG both gradually increases. The brightness of LED lighted by the EMG sharply increases and exceeds that of TENG after 115 deg. All these results demonstrate the remarkable merit of the TENG than the EMG in harvesting weak mechanical energy.

Discussion

In summary, this work has investigated the applied torque and energy conversion efficiency of the EMG and TENG, which proves that the TENG has a higher conversion efficiency than that of the EMG at the low input mechanical power. The input mechanical torques of the rotating EMG and TENG are systematically measured, respectively. At constant rotation rates, the input mechanical torque of EMG is balanced by the friction resisting torque and electromagnetic resisting torque, which increases with the increasing rotation rate due to Ampere force. While the input mechanical torque of TENG is balanced by the friction resisting torque and electrostatic resisting torque, which is nearly constant at different rotation rates. The energy conversion efficiencies of both generators are also quantified and compared. With the increase of the input mechanical power, the energy conversion efficiency of EMG is increasing, while that of the TENG remains nearly constant. The comparison results and demonstrations have shown that the TENG has a higher conversion efficiency than that of the EMG at a low input mechanical power. Moreover, the fewer the number of power generation units for both generators, the larger dominant power range for the TENG. In the energy conversion demonstration, an LED powered by the TENG and EMG in the same input mechanical energy has been exhibited. The TENG rather than the EMG can light up the LED by a small mechanical energy. This work has demonstrated a remarkable merit of the TENG under a gentle-triggering, which has verified the possible applications for efficiently harvesting weak mechanical energy from human body and ambient environment.

Limitations of the study

The applied torque, input mechanical power and energy conversion efficiencies of the rotational EMG and TENG are systematically investigated and compared. The results have demonstrated the triboelectric nanogenerator is more suitable for harvesting weak input mechanical energy. However, this method for measuring applied torque, input mechanical power and energy conversion efficiencies is only applicable to the rotational mode. For the TENGs in other modes such as contact-separation mode, further research on measurement methods are expected in the near future.

Resource availability

Lead contact

Further information and requests for resources and reagents should be directed to and will be fulfilled by the lead contact, Chi Zhang.

Materials availability

This study did not generate new unique reagents.

Data and code availability

We do not have any code and upon request we can provide the original data.

Methods

All methods can be found in the accompanying transparent methods supplemental file.
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