Mohammed AlAloul1, Mahmoud Rasras1. 1. Photonics Research Lab, Department of Electrical and Computer Engineering, PO Box 129188, New York University Abu Dhabi, Abu Dhabi, UAE.
Abstract
Graphene has emerged as an ultrafast optoelectronic material for all-optical modulators. However, because of its atomic thickness, it absorbs a limited amount of light. For that reason, graphene-based all-optical modulators suffer from either low modulation efficiencies or high switching energies. Through plasmonic means, these modulators can overcome the aforementioned challenges, yet the insertion loss (IL) of plasmon-enhanced modulators can be a major drawback. Herein, we propose a plasmon-enhanced graphene all-optical modulator that can be integrated into the silicon-on-insulator platform. The device performance is quantified by investigating its switching energy, extinction ratio (ER), IL, and operation speed. Theoretically, it achieves ultrafast (<120 fs) and energy-efficient (<0.6 pJ) switching. In addition, it can operate with an ultra-high bandwidth beyond 100 GHz. Simulation results reveal that a high ER of 3.5 dB can be realized for a 12 μm long modulator, yielding a modulation efficiency of ∼0.28 dB/μm. Moreover, it is characterized by a 6.2 dB IL, which is the lowest IL reported for a plasmon-enhanced graphene all-optical modulator.
Graphene has emerged as an ultrafast optoelectronic material for all-optical modulators. However, because of its atomic thickness, it absorbs a limited amount of light. For that reason, graphene-based all-optical modulators suffer from either low modulation efficiencies or high switching energies. Through plasmonic means, these modulators can overcome the aforementioned challenges, yet the insertion loss (IL) of plasmon-enhanced modulators can be a major drawback. Herein, we propose a plasmon-enhanced graphene all-optical modulator that can be integrated into the silicon-on-insulator platform. The device performance is quantified by investigating its switching energy, extinction ratio (ER), IL, and operation speed. Theoretically, it achieves ultrafast (<120 fs) and energy-efficient (<0.6 pJ) switching. In addition, it can operate with an ultra-high bandwidth beyond 100 GHz. Simulation results reveal that a highER of 3.5 dB can be realized for a 12 μm long modulator, yielding a modulation efficiency of ∼0.28 dB/μm. Moreover, it is characterized by a 6.2 dB IL, which is the lowest IL reported for a plasmon-enhanced graphene all-optical modulator.
The
incessant demand for bandwidth-intensive applications necessitates
the quest for ultrahigh-speed optoelectronic devices. Global data
center traffic is growing faster by more than 25% a year.[1] To sustain this enormous growth, ultrafast and
energy-efficient integrated optical transceivers are indispensable.[2] In these data centers, integrated silicon-based
photonic interconnects serve as the communication link between servers,
racks, and digital logic chips, where the transmission loss in Si
waveguides can be as low as 0.1 dB/cm using the silicon-on-insulator
(SOI) platform.[3] Integrated optical interconnects
consist of a transmitter, a waveguide, and a receiver. The modulator
imposes a data stream on the optical waveguide mode.Most modulators
employed in silicon photonics (SiPh) are based
on silicon.[4] These high-speed modulators
operate based on the plasma dispersion effect and are limited by an
intrinsic bandwidth of ∼60 GHz.[5,6] Plasma dispersion
modulators with bit rates exceeding 100 Gbps have been demonstrated
by introducing additional fabrication steps or incorporating reactive
components in the driver circuit.[7,8] Nevertheless,
these devices are based on large-footprint Mach–Zehnder modulator
structures, and their energy consumption is on the order of pJ/bit
or more. Modulators based on thin-film lithium niobate (LiNbO3) which is heterogeneously integrated into silicon waveguides
were demonstrated with a bandwidth of up to 110 GHz.[5,9] However, these devices operate with stringent phase-matching conditions
which complicate their design and require unconventional fabrication
processes, making them unfavorable for mass production. Two-dimensional
materials on silicon recently emerged as active materials for electro-optic
modulation, with graphene on the lead due to its exceptionally fast
response.[10−13] These materials are characterized by a favorable set of inherent
features, which include high-speed, small footprint, low-cost manufacturing,
low-power consumption, and compatibility with complementary metal–oxide
semiconductor processes.[4,14] Nonetheless, the bandwidth
of graphene-based electro-optic modulators is limited by device parasitics
to a few tens of GHz, which hinders the adoption of these devices
in ultrahigh-speed transceiver links.In recent years, on-chip
all-optical modulators stood out for their
extraordinary high-speed performance.[15−19] These modulators exhibit ultrafast switching speeds
(<1 ps) but consume picojoules of energy.[18,20] Low-energy all-optical switching (<1 pJ) has been demonstrated
in refs,[21−23] yet the operation speed of these
devices is limited to tens of GHz. On-chip all-optical graphene modulators
were lately investigated in refs.[17,24] These modulators
suffered from relatively high switching energies or low modulation
efficiencies, and both limitations can be attributed to the intrinsically
low optical absorption of graphene. Introducing plasmonic metals to
these modulators to plasmonically enhance the effective absorption
of graphene is a promising solution to overcome these limitations.
Indeed, plasmonic all-optical graphene switches and modulators were
experimentally studied in refs,[25,26] where an
ultrafast switching time (260 fs) at an ultra-low energy (35 fJ) was
reported in ref (25). Both plasmonic devices utilized plasmonic gap waveguides, which
in addition to their high Ohmic losses require plasmonic mode converters
to achieve decent coupling efficiencies with Si waveguides. Therefore,
despite the remarkable performance of these devices, they are characterized
by an excessive insertion loss (IL), for example, 19 dB in ref (25), making them impractical
for future communication links.Here, we propose a plasmon-enhanced
graphene all-optical modulator
featuring a low IL, an ultrafast operation, a low-energy switching,
and a high modulation efficiency. The device structure is based on
a silicon rib waveguide, which facilitates its integration into the
SOI platform. The device structure is presented, and its operation
principle is explained. Its performance is quantified by investigating
its switching energy, modulation efficiency, IL, and operation speed.
Following that, a comparison is made with state-of-the-art devices.
Finally, this report is concluded by pointing out the major findings
of this study.
Results and Discussion
Device Structure
The structure of
the on-chip modulator is illustrated in Figure a. A silicon rib waveguide on top of a bottom
oxide (BOX) layer guides the incoming light to the modulator section.
Silicon dioxide (SiO2) is placed on the silicon ridge sides
to facilitate the placement of the graphene monolayer on top of the
waveguide. A gold (Au) stripe is placed on top of graphene to plasmonically
enhance its interaction with the optical mode, which in turn boosts
its effective optical absorption. The waveguide supports a quasi-transverse
magnetic (quasi-TM) mode, which is chosen for its superior interaction
with the graphene sheet (see Supporting Information Section 1).
Figure 1
(a) All-optical modulator based on a silicon rib waveguide
structure.
(b) Electric field profile of the propagating quasi-TM mode in the
waveguide-integrated modulator. The dashed white line represents the
graphene sheet plane. λ = 1550 nm. Si: silicon, SiO2: silicon dioxide, BOX: bottom oxide, Gr: graphene, and Au: gold.
(a) All-optical modulator based on a silicon rib waveguide
structure.
(b) Electric field profile of the propagating quasi-TM mode in the
waveguide-integrated modulator. The dashed white line represents the
graphene sheet plane. λ = 1550 nm. Si: silicon, SiO2: silicon dioxide, BOX: bottom oxide, Gr: graphene, and Au: gold.Figure a presents
the coupling efficiency between the SOI waveguide and the modulator
section. The coupling efficiency is taken as the power overlap between
the fundamental waveguide and modulator TM modes that yield the highest
coupling efficiency, at each waveguide height and width, for a fixed
160 nm thick slab and 2 μm BOX layer. The Au stripe is 20 nm
thick, and its width was initially set equal to the waveguide width.
A commercially available 500 nm SOI waveguide height was chosen to
achieve a decent coupling efficiency (70%). For heights below 340
nm, the coupling efficiency is <30%, which results in a high IL.
On the other hand, the coupling efficiency increases for heights beyond
500 nm, yet these heights are not common in SOI-based SiPh. The waveguide
width was chosen to be 460 nm, which is a standard width in SiPh.
All-optical modulators are employed for ultrafast information processing
and photonic computing systems.[15,16] These systems are likely
to contain heterogeneously integrated III–V lasers on Si. In
such a case, a 500 nm thick waveguide would be a favorable choice
because thick SOI waveguides are essential to achieve decent coupling
efficiencies with III–V lasers.[27−30]
Figure 2
(a) Coupling efficiency between the SOI
waveguide and the modulator
section as a function of the waveguide height and width and (b) coupling
efficiency as a function of the taper length. λ = 1550 nm.
(a) Coupling efficiency between the SOI
waveguide and the modulator
section as a function of the waveguide height and width and (b) coupling
efficiency as a function of the taper length. λ = 1550 nm.The Au stripe width was later changed from its
initial 460 nm width
to 380 nm, in order to achieve high absorption efficiency in graphene
(see Supporting Information Section 2).
The coupling efficiency was also improved as a result of this modification
to become ∼77%. Furthermore, tapered Au stripes that are 600
nm long were incorporated into the design, which boosted the coupling
efficiency to ∼88% (see Figure b). For longer taper lengths, the coupling efficiency
is limited by the Ohmic losses induced by the Au stripe. The power
overlap between the two modes was computed using Lumerical MODE.[31,32] The coupling efficiency with a taper was computed using the mode
expansion monitor,[33,34] where the fundamental SOI TM-mode
was imported into Lumerical FDTD to compute its power overlap with
the modulator waveguide after tapering the Au stripe.The waveguide
satisfies the single-mode condition for a deep-etched
sub-micron SOI rib at λ = 1550 nm, which is determined by the
following relations[35]where W is the waveguide
width, H is the waveguide height, and h is the slab thickness. A deep-etched silicon waveguide is one, where h < H/2 is satisfied. We propose some
fabrication methods and discuss the impact of some potential variations
on the device performance in Supporting Information Section 5. In the next section, we explore the operation principle
of the device.
Operation Principle
Graphene can
be utilized to build extinction or phase modulators. In ref (36), it was reported that
graphene-based phase all-optical modulators exhibit a higher modulation
efficiency than extinction modulators. However, this conclusion is
only applicable for graphene modulators that are based on a Mach–Zehnder
structure. In another report,[37] it was
concluded that higher modulation efficiencies can be achieved based
on extinction modulators, and for a smaller device footprint. These
modulators operate based on the principle of Pauli-blocking,[38−40] which occurs when photogenerated electrons fill the conduction band
states of graphene following a sufficiently intense pump excitation,
thereby blocking the interband transition of other electrons.Graphene is unintentionally doped when placed on a substrate, giving
a chemical potential (μ) in the range of 0.1–0.2 eV.[37,41] For telecom wavelengths, a photon has an energy ℏω
> 2μ, which induces an interband transition following its
absorption
by graphene, thereby creating an electron–hole pair.[42]Figure a illustrates the interband absorption of a pump photon with
an energy ℏωpump > 2μ. Upon absorbing
a sufficiently intense pump excitation, electrons fill up the conduction
band states, resulting in a chemical potential μ′. Consequently,
incoming pump photons cannot induce an interband transition because
ℏωpump ≤ 2μ′ and are thus
transmitted through graphene (see Figure b). Similarly, a probe photon with an energy
ℏωprobe ≤ ℏωpump is also transmitted because ℏωprobe ≤
2μ′. As such, all-optical amplitude modulation can be
realized; the probe signal is transmitted when the pump signal is
HIGH, or absorbed when the pump signal is LOW.
Figure 3
(a) Interband absorption
of a pump photon with energy ℏωpump. (b) Pump
photon Pauli-blocked (transmitted) after applying
a sufficiently high pump intensity. (c) Transmission of the probe
signal, as determined by the pump signal amplitude. Black and white
circles represent electrons and holes, respectively. Filled energy
states are represented by darker shades.
(a) Interband absorption
of a pump photon with energy ℏωpump. (b) Pump
photon Pauli-blocked (transmitted) after applying
a sufficiently high pump intensity. (c) Transmission of the probe
signal, as determined by the pump signal amplitude. Black and white
circles represent electrons and holes, respectively. Filled energy
states are represented by darker shades.From Figure b,
it can be inferred that μ′ = ℏωpump/2.[25] The chemical potential of graphene
is related to the carrier density (n0)
by the following relation[42]where vF is the
Fermi velocity. The interband absorption is Pauli-blocked when graphene
gains a chemical potential energy that is given byΔn can be calculated by reordering eqFor a graphene
sheet with an area A = WL, the number
of carriers that are needed to reach μ′
is m = ΔnWL. Because each
absorbed photon generates an electron–hole pair, the energy
that is required to saturate the absorption of graphene (Usw) can be expressed as[25]where Usw is the
switching energy, and ℏω is the pump photon energy. We
are interested in the graphene area that interacts with the optical
mode. For the modulator structure of Figure a, the interaction area is the waveguide
width (W) times the modulator length (L). Figure a shows
the calculated switching energy for a 1550 nm pump signal. The switching
energy increases at low chemical potentials and is maximized when
the charge neutrality point coincides with the Dirac point (μ
= 0). As illustrated in Figure , more electrons are needed to fill the conduction band states
up to μ′ when μ is low and that necessitates higher
switching energies. Similarly, longer modulators require a higher
pump energy to saturate the absorption of graphene, which is expected
because the number of carriers (m) is proportional
to L. The modulation efficiency is also a function
of the modulator length, as is going to be elaborated in the next
section. Because graphene is effectively doped by the substrate, the
switching energy is practically considered for chemical potentials
in the range of 0.1–0.2 eV. In that range, the switching process
is inherently efficient, where the optical absorption saturates when
graphene absorbs energies <60 fJ. However, in reality, the optical
mode experiences coupling and Ohmic losses as it propagates in the
modulator waveguide. In addition, graphene absorbs only a small fraction
(AGr) of the total mode energy (see Methods). Moreover, a part of graphene absorption
is nonsaturable and does not contribute to the modulation function.[25,43−45] Thus, the power fraction that is effectively absorbed
by graphene (AGr) can be expressed aswhere As and Ans are the saturable and nonsaturable fractions
of AGr. For the all-optical modulator
that is presented in ref (44), it has been reported that monolayer graphene absorbs 69.12%
of light, of which 65.88% is saturable and 3.24% is nonsaturable.
Based on these experimental values, the nonsaturable absorption of
monolayer graphene is ∼5% of the total effective absorption:
(3.24/69.12) × 100%, which is used to quantify Ans in this study. Monolayer graphene has the least nonsaturable
absorption; Ans is higher for thicker
graphene.[44−46] The higherAns reduces
the modulation efficiency and contributes to a higher IL. In addition
to graphene thickness, surface defects, for example, wrinkles, result
in a higherAns.[44] To calculate the effective switching energy (Ueff), we consider the limited absorption of graphene and compensate
for the coupling, Ohmic, and nonsaturable absorption losseswhere Γ is the coupling
loss and AAu is the Ohmic loss that is
induced by the Au stripe (see Methods). On
the left hand side of eq , we added the amount of switching energy that is lost to coupling
and ohmic losses. On the right hand side, we subtracted the nonsaturable
component of the effective absorption of graphene because it does
not contribute to the modulation function. Γ is accounted for
only once in eq because
the optical mode couples out of the modulator after switching takes
place. The calculated effective switching energy for λpump = 1550 nm is shown in Figure b. As expected, Ueff is higher
than Usw, and by a factor of ∼11×.
Despite that, energy-efficient switching is attainable, where pump
signals with energies <600 fJ can saturate the absorption of graphene
for λpump = 1550 nm, considering the aforementioned
practical range of μ. It is possible to tune the chemical potential
of graphene on a substrate by thermal annealing.[41,47,48] For a reasonable μ = 0.2 eV and 12
μm long modulator, Ueff is as low
as 242 fJ for a 1550 nm pump signal. In the next section, we investigate
the modulation efficiency and the IL of the device.
Figure 4
(a) Switching energy
(Usw) and (b)
effective switching energy (Ueff) as a
function of the chemical potential (μ) and modulator length
(L). λ = 1550 nm.
(a) Switching energy
(Usw) and (b)
effective switching energy (Ueff) as a
function of the chemical potential (μ) and modulator length
(L). λ = 1550 nm.
Modulation Efficiency
The modulation
efficiency of the modulator is quantified by its extinction ratio
(ER),[24−26,39,40] which is given bywhere Ton and Toff represent the transmitted power of the probe
signal when the pump signal is turned on and off, respectively. Graphene’s
absorption is maximized when the pump signal is turned off. By considering
the fractions of the power absorbed by Au and graphene, and the coupling
losses that the guided mode experiences as it couples in and out of
the modulator, Toff can be expressed asGraphene is transparent
when the pump
signal is turned on, except for the nonsaturable fraction (Ans) of AGr, as was
explained in the previous section. The maximum graphene transparency
and, consequently, the maximum ER of the modulator are obtained when
the pump signal has an energy U ≥ Ueff. By considering the nonsaturable fraction
of AGr, the maximum transmitted power
of the probe signal (Tmax) can be expressed
asThe IL is given by[49]Figure a presents
the maximum ER and Tmax, and Figure b shows the corresponding
IL and ER/IL ratio as a function of the modulator length. By linearly
fitting the ER curve that is shown in Figure a, we obtain a modulation efficiency of ∼0.28
dB/μm. To maximize the ER and the ER/IL ratio, we set the modulator
length to 12 μm. At this length, a 3.5 dB ER is achievable for
a relatively low IL (6.2 dB). The slight offset in ER that is seen
at L = 0 is due to the graphene portion that is placed
beneath the taper, where its effective absorption has been incorporated
into the calculations (see Supporting Information Section 3).
Figure 5
(a) Maximum transmitted power of the probe signal (Tmax) and the maximum ER (ERmax) as
a function
of the modulator length (L). (b) IL and ER/IL ratio
as a function of the modulator length (L). λ
= 1550 nm.
(a) Maximum transmitted power of the probe signal (Tmax) and the maximum ER (ERmax) as
a function
of the modulator length (L). (b) IL and ER/IL ratio
as a function of the modulator length (L). λ
= 1550 nm.The energy of a pulse is a function
of the pulse duration and power: U = tpulseP. Considering a constant pulse
duration, the saturable absorption
of graphene can be expressed as a function of the pump signal energy[25]where Usat is
the energy at which As is equal to half
of its maximum value, that is, As(Usat) = AGr(1 – Ans)/2. By incorporating eqs into 12 and 13, the transmitted power of the probe signal (Ton) can be expressed as a function of the pump
signal energyWe estimate Usat by setting it
equal
to Usw/2 because the losses are incorporated
into Ton. Figure shows Ton as
a function of the pump energy. The modulator length and the chemical
potential are varied in Figure a,b, respectively. It can be seen in both figures that Ton is minimized when U = 0,
where it is equal to Toff. Ton rises as the pump energy increases and becomes nearly
flat as U → Ueff, indicating the onset of saturable absorption. A higher Ton/Toff ratio, and
hence, a higherER, is achieved for longer modulators. This is consistent
with the results that are presented in Figure a. A greater pump energy is required to saturate
the absorption of graphene at lower μ (see Figure b). This observation is consistent
with the calculated Ueff, as is presented
in Figure b.
Figure 6
(a) Transmitted
power of the probe signal (Ton) as a function
of the pump signal energy at multiple modulator
lengths for a fixed μ = 0.2 eV. (b) Transmitted power of the
probe signal (Ton) as a function of the
pump energy (U) at multiple chemical potential (μ)
values and fixed L = 12 μm.
(a) Transmitted
power of the probe signal (Ton) as a function
of the pump signal energy at multiple modulator
lengths for a fixed μ = 0.2 eV. (b) Transmitted power of the
probe signal (Ton) as a function of the
pump energy (U) at multiple chemical potential (μ)
values and fixed L = 12 μm.Atotal, AAu, and Γ are functions of the wavelength (see Supporting Information Secion 4). Consequently,
ER, IL, and Ueff are also functions of
the wavelength. Figure a shows the ER and
the IL of the modulator as a function of the probe signal wavelength.
The IL follows the trend of the coupling efficiency, which decreases
at longer wavelengths, whereas the ER is more affected by the propagation
loss as a function of wavelength (see Supporting ). In Figure a, we assume that a pump signal with an energy U ≥ Ueff has been applied
with a wavelength λpump < λprobe. Figure b presents
the calculated Usw and Ueff as a function of the pump signal wavelength at a fixed
μ = 0.2 eV. Interestingly, Usw is
higher for pump signals of shorter wavelengths (see eq ). This result agrees with previous
experimental studies, where it has been reported in ref[45,50] that a
lower pump intensity is required to saturate graphene at longer pump
wavelengths. This can be explained by the unique conical dispersion
of graphene, which becomes wider at higher energies. Consequently,
a greater number of high-energy photons would be needed to fill the
high-energy states in the conduction band with photoexcited electrons,
which results in a higher overall switching energy. Therefore, a higher
pump energy would be required to saturate the absorption of graphene,
so that a probe signal with a wavelength λprobe >
λpump would be transmitted through graphene. We also
observe that Ueff is minimized at longer
wavelengths. However, it is noted that this trend is not as linear
as it is the case for Usw at shorter wavelengths
because for this device, external factors such as the coupling efficiency,
Ohmic losses, and the effective absorption of graphene dominate the
trend of Ueff at shorter wavelengths.
More specifically, the absorption efficiency of graphene and the coupling
efficiency are both maximized at shorter wavelengths (see Supporting Information Section 4), and therefore,
both contribute to a smaller Ueff based
on eq . The resultant Usw and Ueff at other
chemical potentials are presented in Supporting Information Section 4. In the next section, we calculate the
device bandwidth and switching speed.
Figure 7
(a) Maximum ER (ERmax) of the
modulator and its IL as
a function of the probe signal wavelength (λprobe). (b) Switching energy (Usw) and effective
switching energy (Ueff) as a function
of the pump signal wavelength (λpump) for fixed L = 12 μm and μ = 0.2 eV.
(a) Maximum ER (ERmax) of the
modulator and its IL as
a function of the probe signal wavelength (λprobe). (b) Switching energy (Usw) and effective
switching energy (Ueff) as a function
of the pump signal wavelength (λpump) for fixed L = 12 μm and μ = 0.2 eV.
Operation Speed
The operation speed
of the modulator is determined by the carrier cooling dynamics in
monolayer graphene. Graphene has a unique conical dispersion, where
its density of states fades away at the Dirac point. As a result,
electrons in the vicinity of the Dirac point have a relatively low
heat capacity. Upon photoexcitation, these electrons immediately scatter
with one another, creating a fleeting Fermi–Dirac distribution
of hot thermalized electrons within a few tens to 150 fs.[51,52] As such, photon energy is converted to electron heat. Eventually,
hot electrons cool down in a few picoseconds by emitting optical and
acoustic phonons, coupling with surface optical phonons, and most
importantly through disorder-assisted scattering which dominates at
room temperature.[47,53−55] Hence, electrons
first heat up through intraband electron–electron scattering,
then they cool down through phonon- and disorder-assisted scattering.The Boltzmann transport theory can be used to calculate the timescale
in which electron–electron scattering events take place.[56] First, the electrical conductivity of graphene
can be expressed as[57−59]where σ0 is the minimum conductivity
taken from,[57]h is the
Planck’s constant, and Δ is the minimum conductivity
plateau. Δ is a parameter that quantifies the amount of disorder
in a graphene sample. For graphene-on-SiO2, the minimum
conductivity plateau can be as low as Δ ≈ 55 meV,[57,60] or as high as Δ ≈ 100 meV.[58] The Drude mobility (η) of graphene is given by[61]Now the electron–electron scattering time (τscat) is calculated according to the Boltzmann transport theory[62]The electron cooling time (τcool) is the inverse
of the electron cooling rate (γcool), which can be
expressed as[53,57,63]where Tk = 300
K is the temperature, g is the electron–phonon
coupling constant, ϱ is the density of states, kF is the Fermi wave vector, is the mean free path, TBG is the Bloch–Grüneisen temperature, D = 20 eV is the deformation potential constant,[47] ρ = 7.6 × 10–7 kg/m2 is the mass density of graphene, and s =
2 × 104 m/s is the speed of longitudinal acoustic
phonons.[42]Figure a shows
τscat and Figure b shows τcool for low-disorder (Δ
= 55 meV) and high-disorder (Δ = 100 meV) graphene. It is observed
that electron–electron scattering occurs in 30–120 fs,
which is consistent with the experimentally reported electron heating
times.[51,52] The electron cooling time is 4–10
ps, which is similar to what has been reported in the literature.[47,53] Moreover, the scattering and cooling events occur on a shorter timescale
for the highly disordered graphene, which is consistent with experimental
findings.[64] The calculated τscat and τcool significantly increase as μ
→ 0 and thus were not shown in its vicinity. As was previously
explained, graphene is effectively doped by the substrate, and the
μ → 0 case is therefore not applicable. For graphene,
the time evolution of the electron temperature, that is, ΔTe(t), can be described by a
two-exponential function[51,64,65]where τ1 and τ2 are analytically
fitted time constants. Based on the calculated
τscat and τcool values, we consider
the case of 100 fs heating time and 4 ps cooling time, which are taken
as the rise (τr) and fall (τf) times
of ΔTe, respectively. For the same
τr and τf, the resultant ΔTe is shown in Figure , where the corresponding time constants
are τ1 = 0.06 ps and τ2 = 1.8 ps
(see Supporting Information Section 7);
both are in agreement with experimentally fitted time constants.[44,51,64−66] As seen in Figure , electrons heat
up within a sub-ps duration and subsequently cool down in a few picoseconds.
Therefore, this device can operate as an ultrafast switch, with a
switching time that is determined by electron–electron scattering
events, that is, 30–120 fs. As a modulator, this device is
limited by the electron cooling time, that is, <10 ps, depending
on the chemical potential and sample disorder. This corresponds to
an ultra-high bandwidth beyond 100 GHz.
Figure 8
(a) Electron–electron
scattering time (τscat) and (b) electron cooling
time (τcool) for low-disorder
(Δ = 55 meV) and high-disorder (Δ = 100 meV) graphene
as a function of chemical potential (μ).
Figure 9
Time evolution
of the electron temperature (ΔTe) in graphene following a pumping event, and the corresponding
normalized transmittance of the probe signal as a function of time.
(a) Electron–electron
scattering time (τscat) and (b) electron cooling
time (τcool) for low-disorder
(Δ = 55 meV) and high-disorder (Δ = 100 meV) graphene
as a function of chemical potential (μ).Time evolution
of the electron temperature (ΔTe) in graphene following a pumping event, and the corresponding
normalized transmittance of the probe signal as a function of time.In practice, the modulator can impose a pump pulse
on the probe
signal, even if electrons are not totally cooled down. However, this
comes at the cost of a lower modulation efficiency. A high ΔTe indicates that many electrons are photoexcited
and are thus occupying the conduction band states. When ΔTe → 0, graphene is reverted to its steady
state, where electrons occupy the valence band states. Consequently,
the transmittance of the probe signal (Ton) increases with the increase of ΔTe (see Figure ). Based
on eq , a higher Ton/Toff ratio results
in a higherER. Thus, the modulation efficiency is also a function
of the time delay between two consecutive pump pulses; it is possible
to modulate a probe signal when the time delay between two consecutive
pulses is less than τcool, but this may result in
a poor ER because the Ton/Toff ratio would be reduced.Table presents
the performance metrics of on-chip graphene all-optical switches and
modulators that were previously reported. The device presented in
this work achieves the fastest switching speed because it is based
on monolayer graphene. Besides offering a higher modulation efficiency,
fewer layer graphene is characterized by faster carrier heating and
cooling mechanisms.[44,65] The device presented in ref (25) is based on bilayer graphene
and has demonstrated a switching time of 260 fs. It is noted in Table that plasmonic devices
achieve a decent performance at a small footprint, with the most compact
footprint reported in ref (25). For scenarios where the device footprint and the switching
energy are not a concern, nonplasmonic devices are the favorable choice
for their negligible IL, for example refs (17) and (24). Though this device is longer than other plasmonic ones
reported in literature, it can achieve a similar modulation efficiency
at a significantly lower IL.
Table 1
Performance Metrics
of On-Chip Graphene
All-Optical Switches/Modulators
structure
IL
ER (dB)
L (μm)
ER/μm
IL/μm
tswitch
Ueff
dielectric WG[24]
negligible
2.75
100
0.0275 dB/μm
negligible
n/a
n/aa
SOI WG[17]
negligible
1.1b
30
0.0367 dB/μm
negligible
1.2 psc
2.1 pJ
plasmonic WG[26]
n/a
2.1
10
0.21 dB/μm
n/a
n/a
n/ad
plasmonic WG[25]
19 dB
3.5
4
0.875 dB/μm
4.75 dB/μm
260 fs
35 fJ
this work
6.2 dB
3.5
12
0.28 dB/μm
0.517 dB/μm
30–120 fs
<0.6 pJ
Input light power
is 60 mW.
Modulation depth
is 22.7%.
Limited by the
resolution time of
the asynchronous pump–probe system.
Input light power is 46 mW. n/a:
not available (not reported).
Input light power
is 60 mW.Modulation depth
is 22.7%.Limited by the
resolution time of
the asynchronous pump–probe system.Input light power is 46 mW. n/a:
not available (not reported).
Conclusions
To sum up, a waveguide-integrated
plasmon-enhanced graphene all-optical
modulator is proposed. The device structure is based on a thick Si
rib waveguide, which enables its integration into the SOI platform.
It operates based on the principle of Pauli-blocking, where the optical
absorption of graphene saturates by absorbing sufficiently intense
pump radiation. A plasmonic gold (Au) stripe was incorporated into
the modulator waveguide to enhance the effective absorption of graphene
by a factor of ∼4×. Furthermore, the Au stripe was tapered
to improve the coupling efficiency between the SOI and modulator waveguides
to be as high as 88%. We investigated the effective switching energy,
modulation efficiency, and IL of the device as a function of the modulator
length. The modulator length was set to 12 μm to achieve a highER (3.5 dB) at a relatively low IL (6.2 dB), which is the lowest IL
reported for a plasmon-enhanced graphene all-optical modulator. The
modulator achieves efficient sub-picojoule switching, where the effective
switching energy is <600 fJ for λpump = 1550 nm.
The switching time of the device is limited by intraband electron–electron
scattering, where the switching time was calculated to be 30–120
fs. As a modulator, its operation bandwidth is determined by the hot
carrier cooling dynamics, leading to ultrahigh bandwidths beyond 100
GHz. This device is characterized by very promising performance metrics
that are expected to serve the needs of ultrahigh-speed links in next-generation
data centers.
Methods
The total
propagation loss of the computed mode that is shown in Figure b is αtotal = 0.43 dB/μm (see Figure a). Removing graphene yields a propagation
loss αAu = 0.34 dB/μm (see Figure b), which is attributed to
Au. The propagation loss (α) is defined as[67]where Ei and Ef represent the electric
field intensity before
and after propagating a distance L in the modulator
waveguide, respectively. The total fraction of power absorbed in the
waveguide (Atotal) can be calculated using
the Beer–Lambert law
Figure 10
(a) Propagation loss of the waveguide mode
with graphene and (b)
without graphene. The white line represents the graphene sheet plane.
λ = 1550 nm.
(a) Propagation loss of the waveguide mode
with graphene and (b)
without graphene. The white line represents the graphene sheet plane.
λ = 1550 nm.The propagation loss
that is related to graphene is given bywhich results in αGr = 0.09
dB/μm. Thus, the Au stripe enhances the absorption of graphene
by a factor of ∼4× (see Supporting Information Section 2). The fraction of power that is absorbed
by graphene (AGr) can be taken as[68]Then, the remainder constitutes the Ohmic absorption that
is introduced
by Au
Authors: Hugo E Romero; Ning Shen; Prasoon Joshi; Humberto R Gutierrez; Srinivas A Tadigadapa; Jorge O Sofo; Peter C Eklund Journal: ACS Nano Date: 2008-10-28 Impact factor: 15.881
Authors: Dong Sun; Zong-Kwei Wu; Charles Divin; Xuebin Li; Claire Berger; Walt A de Heer; Phillip N First; Theodore B Norris Journal: Phys Rev Lett Date: 2008-10-06 Impact factor: 9.161
Authors: K J Tielrooij; L Piatkowski; M Massicotte; A Woessner; Q Ma; Y Lee; K S Myhro; C N Lau; P Jarillo-Herrero; N F van Hulst; F H L Koppens Journal: Nat Nanotechnol Date: 2015-04-13 Impact factor: 39.213