Literature DB >> 33401378

Characterization of Lignin Compounds at the Molecular Level: Mass Spectrometry Analysis and Raw Data Processing.

Ruochun Zhang1,2, Yulin Qi1,2, Chao Ma1, Jinfeng Ge1, Qiaozhuan Hu1, Fu-Jun Yue1,2, Si-Liang Li1,2, Dietrich A Volmer3.   

Abstract

Lignin is the second most abundant natural biopolymer, which is a potential alternative to conventional fossil fuels. It is also a promising material for the recovery of valuable chemicals such as aromatic compounds as well as an important biomarker for terrestrial organic matter. Lignin is currently produced in large quantities as a by-product of chemical pulping and cellulosic ethanol processes. Consequently, analytical methods are required to assess the content of valuable chemicals contained in these complex lignin wastes. This review is devoted to the application of mass spectrometry, including data analysis strategies, for the elemental and structural elucidation of lignin products. We describe and critically evaluate how these methods have contributed to progress and trends in the utilization of lignin in chemical synthesis, materials, energy, and geochemistry.

Entities:  

Keywords:  data processing; ionization; lignin; mass spectrometry; structural information

Mesh:

Substances:

Year:  2021        PMID: 33401378      PMCID: PMC7795929          DOI: 10.3390/molecules26010178

Source DB:  PubMed          Journal:  Molecules        ISSN: 1420-3049            Impact factor:   4.411


  46 in total

1.  High-performance liquid chromatography/high-resolution multiple stage tandem mass spectrometry using negative-ion-mode hydroxide-doped electrospray ionization for the characterization of lignin degradation products.

Authors:  Benjamin C Owen; Laura J Haupert; Tiffany M Jarrell; Christopher L Marcum; Trenton H Parsell; Mahdi M Abu-Omar; Joseph J Bozell; Stuart K Black; Hilkka I Kenttämaa
Journal:  Anal Chem       Date:  2012-06-29       Impact factor: 6.986

Review 2.  Structural analysis of small to medium-sized molecules by mass spectrometry after electron-ion fragmentation (ExD) reactions.

Authors:  Yulin Qi; Dietrich A Volmer
Journal:  Analyst       Date:  2016-01-04       Impact factor: 4.616

3.  Enhanced Mass Defect Filtering To Simplify and Classify Complex Mixtures of Lignin Degradation Products.

Authors:  Tobias K F Dier; Kerstin Egele; Verlaine Fossog; Rolf Hempelmann; Dietrich A Volmer
Journal:  Anal Chem       Date:  2015-12-23       Impact factor: 6.986

4.  Characterization of Miscanthus giganteus lignin isolated by ethanol organosolv process under reflux condition.

Authors:  Stefan Bauer; Hagit Sorek; Valerie D Mitchell; Ana B Ibáñez; David E Wemmer
Journal:  J Agric Food Chem       Date:  2012-08-10       Impact factor: 5.279

5.  Detailed study of cyanobacterial microcystins using high performance tandem mass spectrometry.

Authors:  Yulin Qi; Stella Bortoli; Dietrich A Volmer
Journal:  J Am Soc Mass Spectrom       Date:  2014-04-30       Impact factor: 3.109

6.  Shedding light on the structures of lignin compounds: photo-oxidation under artificial UV light and characterization by high resolution mass spectrometry.

Authors:  Yulin Qi; Rolf Hempelmann; Dietrich A Volmer
Journal:  Anal Bioanal Chem       Date:  2016-09-17       Impact factor: 4.142

7.  Identification of the Phenol Functionality in Deprotonated Monomeric and Dimeric Lignin Degradation Products via Tandem Mass Spectrometry Based on Ion-Molecule Reactions with Diethylmethoxyborane.

Authors:  Hanyu Zhu; Tiffany M Jarrell; Nathaniel Louden; Joann P Max; Christopher L Marcum; Hao Luo; James S Riedeman; Mahdi M Abu-Omar; Hilkka I Kenttämaa
Journal:  J Am Soc Mass Spectrom       Date:  2016-08-23       Impact factor: 3.109

8.  Negative ion mode atmospheric pressure ionization methods in lignin mass spectrometry: A comparative study.

Authors:  Dmitry S Kosyakov; Nikolay V Ul'yanovskii; Elena A Anikeenko; Natalia S Gorbova
Journal:  Rapid Commun Mass Spectrom       Date:  2016-10-15       Impact factor: 2.419

Review 9.  Analysis of natural organic matter via fourier transform ion cyclotron resonance mass spectrometry: an overview of recent non-petroleum applications.

Authors:  Yulin Qi; Pingqing Fu; Dietrich A Volmer
Journal:  Mass Spectrom Rev       Date:  2020-05-15       Impact factor: 9.011

10.  Divergent accumulation of microbial necromass and plant lignin components in grassland soils.

Authors:  Tian Ma; Shanshan Zhu; Zhiheng Wang; Dima Chen; Guohua Dai; Bowei Feng; Xiangyan Su; Huifeng Hu; Kaihui Li; Wenxuan Han; Chao Liang; Yongfei Bai; Xiaojuan Feng
Journal:  Nat Commun       Date:  2018-08-28       Impact factor: 14.919

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  1 in total

1.  Solid-State Nuclear Magnetic Resonance as a Tool to Probe the Impact of Mechanical Preprocessing on the Structure and Arrangement of Plant Cell Wall Polymers.

Authors:  Coyla R Munson; Yu Gao; Jenny C Mortimer; Dylan T Murray
Journal:  Front Plant Sci       Date:  2022-01-12       Impact factor: 5.753

  1 in total

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