Consistent approach for electrical resistivity within Ziman's theory from solid state to hot dense plasma: Application to aluminum.

The approach presented in this work allows a consistent calculation of electrical conductivity of dense matter from the solid state to the hot plasma using the same procedure, consisting in dropping elastic scattering contributions to solid's and liquid's structure factors in the framework of the Ziman theory. The solid's structure factor was computed using a multiphonon expansion. The elastic part is the zero-phonon term and corresponds to Bragg peaks, thermally damped by Debye-Waller attenuation factors. For the liquid, a similar elastic contribution to the structure factor results from a long-range order persisting during the characteristic electron-ion scattering time. All the quantities required for the calculation of the resistivities are obtained from our average-atom model, including the total hypernetted-chain structure factor used from the liquid state to the plasma. No interpolation between two limiting structure factors is required. We derive the correction to apply to the resistivity in order to account for the transient long-range order in the liquid and show that it improves considerably the agreement with quantum-molecular dynamics simulations and experimental aluminum's isochoric and isobaric conductivities. Our results suggest that the long-range order in liquid aluminum could be a slightly compressed fcc one. Two series of ultrafast experiments performed on aluminum were also considered, the first one by Milchberg et al. using short laser pulses and the second one by Sperling et al. involving x-ray heating and carried out on the Linac Coherent Light Source facility. Our attempts to explain the latter assuming an initial liquid state at an ion temperature much smaller than the electron one suggest that the actual initial state before main heating is neither perfectly solid nor a normal liquid.