Literature DB >> 32817545

Massively parallel classical logic via coherent dynamics of an ensemble of quantum systems with dispersion in size.

Hugo Gattuso1, R D Levine2,3,4, F Remacle1,5.   

Abstract

Quantum parallelism can be implemented on a classical ensemble of discrete level quantum systems. The nanosystems are not quite identical, and the ensemble represents their individual variability. An underlying Lie algebraic theory is developed using the closure of the algebra to demonstrate the parallel information processing at the level of the ensemble. The ensemble is addressed by a sequence of laser pulses. In the Heisenberg picture of quantum dynamics the coherence between the N levels of a given quantum system can be handled as an observable. Thereby there are N 2 logic variables per N level system. This is how massive parallelism is achieved in that there are N 2 potential outputs for a quantum system of N levels. The use of an ensemble allows simultaneous reading of such outputs. Due to size dispersion the expectation values of the observables can differ somewhat from system to system. We show that for a moderate variability of the systems one can average the N 2 expectation values over the ensemble while retaining closure and parallelism. This allows directly propagating in time the ensemble averaged values of the observables. Results of simulations of electronic excitonic dynamics in an ensemble of quantum dot (QD) dimers are presented. The QD size and interdot distance in the dimer are used to parametrize the Hamiltonian. The dimer N levels include local and charge transfer excitons within each dimer. The well-studied physics of semiconducting QDs suggests that the dimer coherences can be probed at room temperature.

Entities:  

Keywords:  2D electronic spectroscopy; Lie algebra; information quantal processing at room temperature; noise resilience; quantum dots

Year:  2020        PMID: 32817545      PMCID: PMC7474646          DOI: 10.1073/pnas.2008170117

Source DB:  PubMed          Journal:  Proc Natl Acad Sci U S A        ISSN: 0027-8424            Impact factor:   11.205


  25 in total

1.  Architecture with designer atoms: simple theoretical considerations.

Authors:  F Remacle; R D Levine
Journal:  Proc Natl Acad Sci U S A       Date:  2000-01-18       Impact factor: 11.205

2.  Luminescence polarization of CdSe microcrystals.

Authors: 
Journal:  Phys Rev B Condens Matter       Date:  1992-09-15

3.  Direct evidence of quantum transport in photosynthetic light-harvesting complexes.

Authors:  Gitt Panitchayangkoon; Dmitri V Voronine; Darius Abramavicius; Justin R Caram; Nicholas H C Lewis; Shaul Mukamel; Gregory S Engel
Journal:  Proc Natl Acad Sci U S A       Date:  2011-12-13       Impact factor: 11.205

4.  Information processing in parallel through directionally resolved molecular polarization components in coherent multidimensional spectroscopy.

Authors:  Tian-Min Yan; Barbara Fresch; R D Levine; F Remacle
Journal:  J Chem Phys       Date:  2015-08-14       Impact factor: 3.488

5.  Molecular decision trees realized by ultrafast electronic spectroscopy.

Authors:  Barbara Fresch; Dawit Hiluf; Elisabetta Collini; R D Levine; F Remacle
Journal:  Proc Natl Acad Sci U S A       Date:  2013-09-16       Impact factor: 11.205

6.  Exciton superposition states in CdSe nanocrystals measured using broadband two-dimensional electronic spectroscopy.

Authors:  Daniel B Turner; Yasser Hassan; Gregory D Scholes
Journal:  Nano Lett       Date:  2012-01-04       Impact factor: 11.189

7.  Room-temperature exciton coherence and dephasing in two-dimensional nanostructures.

Authors:  Elsa Cassette; Ryan D Pensack; Benoît Mahler; Gregory D Scholes
Journal:  Nat Commun       Date:  2015-01-19       Impact factor: 14.919

8.  Hot electron and hole dynamics in thiol-capped CdSe quantum dots revealed by 2D electronic spectroscopy.

Authors:  Nils Lenngren; Mohamed A Abdellah; Kaibo Zheng; Mohammed J Al-Marri; Donatas Zigmantas; Karel Žídek; Tõnu Pullerits
Journal:  Phys Chem Chem Phys       Date:  2016-09-21       Impact factor: 3.676

9.  Origin of Broad Emission Spectra in InP Quantum Dots: Contributions from Structural and Electronic Disorder.

Authors:  Eric M Janke; Nicholas E Williams; Chunxing She; Danylo Zherebetskyy; Margaret H Hudson; Lili Wang; David J Gosztola; Richard D Schaller; Byeongdu Lee; Chengjun Sun; Gregory S Engel; Dmitri V Talapin
Journal:  J Am Chem Soc       Date:  2018-11-07       Impact factor: 15.419

10.  Quantum machine learning for electronic structure calculations.

Authors:  Rongxin Xia; Sabre Kais
Journal:  Nat Commun       Date:  2018-10-10       Impact factor: 14.919

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  1 in total

1.  Scalable distributed gate-model quantum computers.

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Journal:  Sci Rep       Date:  2021-02-26       Impact factor: 4.379

  1 in total

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