Literature DB >> 32567893

Depletion of Two-Level Systems in Ultrastable Computer-Generated Glasses.

Dmytro Khomenko1,2, Camille Scalliet3, Ludovic Berthier4,5, David R Reichman2, Francesco Zamponi1.   

Abstract

Amorphous solids exhibit quasiuniversal low temperature anomalies whose origin has been ascribed to localized tunneling defects. Using an advanced Monte Carlo procedure, we create in silico glasses spanning from hyperquenched to ultrastable glasses. Using a multidimensional path-finding protocol, we locate tunneling defects with energy splittings smaller than k_{B}T_{Q}, with T_{Q} the temperature below which quantum effects are relevant (T_{Q}≈1  K in most experiments). We find that as the stability of a glass increases, its energy landscape as well as the manner in which it is probed tend to deplete the density of tunneling defects, as observed in recent experiments. We explore the real-space nature of tunneling defects, and find that they are mostly localized to a few atoms, but are occasionally dramatically delocalized.

Entities:  

Year:  2020        PMID: 32567893     DOI: 10.1103/PhysRevLett.124.225901

Source DB:  PubMed          Journal:  Phys Rev Lett        ISSN: 0031-9007            Impact factor:   9.161


  1 in total

1.  Nuclear quantum effects on the dynamics and glass behavior of a monatomic liquid with two liquid states.

Authors:  Ali Eltareb; Gustavo E Lopez; Nicolas Giovambattista
Journal:  J Chem Phys       Date:  2022-05-28       Impact factor: 4.304

  1 in total

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